Ice IX: An Antiferroelectric Phase Related to Ice III (original) (raw)

Skip Nav Destination

Article navigation

Issue Cover

Research Article| March 01 1968

E. Whalley;

Division of Applied Chemistry, National Research Council, of Canada, Ottawa, Canada

Search for other works by this author on:

J. B. R. Heath;

Division of Applied Chemistry, National Research Council, of Canada, Ottawa, Canada

Search for other works by this author on:

D. W. Davidson

Division of Applied Chemistry, National Research Council, of Canada, Ottawa, Canada

Search for other works by this author on:

Crossmark: Check for Updates

J. Chem. Phys. 48, 2362–2370 (1968)

The dielectric properties of ice III in the frequency range 10−1 to 105 cps have been measured down to − 160°C. There is a gradual transition from the orientationally disordered III to an orientationally ordered and probably antiferroelectric phase, which is designated IX, starting at about − 65°C and reaching completion at about − 108°C. An arrangement of the hydrogen atoms in ice IX is proposed. The amplitude of the orientational polarization decreases continuously through the transformation region although the relaxation time is close to the value extrapolated from previous measurements in the disordered phase. The limiting high‐frequency dielectric constant of the dispersion decreases with decreasing temperature. The cause of this behavior, which is unusual for molecular crystals, is undoubtedly that the polarization of the lattice vibrations contributes a large part of the high‐frequency dielectric constant. This contribution decreases with decreasing temperature because the decreasing anharmonic interaction increases the absorption frequencies. The high‐frequency dielectric constant decreases by about 5.7% at the III‐IX transition although there is little volume change; this decrease might be a valuable way of detecting order‐disorder transitions, particularly if they proceed slowly. The infrared polarizabilities of the various phases are briefly discussed. Ice IX could not be warmed into III because it always transforms to the more stable ice II.

REFERENCES

G. J.

Wilson

,

R. K.

Chan

,

D. W.

Davidson

, and

E.

Whalley

,

J. Chem. Phys.

43

,

2384

(

1965

).

B.

Kamb

,

Acta Cryst.

17

,

1437

(

1964

).

E.

Whalley

and

D. W.

Davidson

,

J. Chem. Phys.

43

,

2148

(

1965

).

J. E.

Bertie

and

E.

Whalley

,

J. Chem. Phys.

40

,

1637

(

1964

).

J. E.

Bertie

,

L. D.

Calvert

, and

E.

Whalley

,

J. Chem. Phys.

38

,

840

(

1963

).

W. B.

Kamb

and

S. K.

Datta

,

Nature

187

,

140

(

1960

).

G.

Tammann

,

Ann. Physik

2

,

1

(

1900

).

P. W.

Bridgman

,

Proc. Am. Acad. Arts Sci.

47

,

441

(

1912

).

G. S.

Kell

and

E.

Whalley

,

J. Chem. Phys.

48

,

2359

(

1968

).

S. R. Gough and D. W. Davidson (private communication).

E.

Whalley

,

D. W.

Davidson

, and

J. B. R.

Heath

,

J. Chem. Phys.

45

,

3976

(

1966

).

R. K.

Chan

,

D. W.

Davidson

, and

E.

Whalley

,

J. Chem. Phys.

43

,

2376

(

1965

).

R. H. Cole, Ann. Rept. 1958, Conf. Electrical Insulation, Natl. Acad. Sci.‐Natl. Res. Council, Washington, D.C., 1959.

This can be proved bv a simple extension of arguments given in

E.

Whalley

,

Advan. High Pressure Res.

1

,

143

(

1966

).

K. Vonnegut, Cat’s Cradle (Holt, Rinehart and Winston, Inc., New York, 1963).

L. D. Calvert and E. Whalley (unpublished results).

A. J.

Brown

and

E.

Whalley

,

J. Chem. Phys.

45

,

4360

(

1966

).

See, for example, H. Fröhlich, Theory of Dielectrics (Oxford University Press, New York, 1958), 2nd ed., Chap. II.

E.

Whalley

and

J. E.

Bertie

,

J. Chem. Phys.

46

,

1264

(

1967

).

J. E.

Bertie

and

E.

Whalley

,

J. Chem. Phys.

46

,

1271

(

1967

).

J. E. Bertie H. J. Labte, and E. Whalley, J. Chem. Phys. (to be published).

E. Whalley (unpublished).

This content is only available via PDF.

© 1968 American Institute of Physics.

1968

American Institute of Physics

You do not currently have access to this content.

Sign in

Sign In

You could not be signed in. Please check your credentials and make sure you have an active account and try again.

Username ?

Password

Pay-Per-View Access

$40.00