Atmospheric trace gases and global climate: a seasonal model study | Tellus B: Chemical and Physical Meteorology (original) (raw)
Atmospheric trace gases and global climate: a seasonal model study
Original Research Papers
Abstract
Observations have shown that concentrations of atmospheric trace gases CO2, CFCs, CH4 and N2O have been increasing and the trend of increases will most likely continue. Increases of these radiatively and chemically important trace gases may have implications for global climate both directly by modifying the earth’s radiation budget and indirectly by changing atmospheric O3 distribution. Here, we use atmospheric models with seasonal cycles to study the changes in latitudinal and vertical distributions of atmospheric O3 and temperature caused by increases of trace gases in the next few decades. It is found that increases of CFCs, CH4, and N2O may augment the surface warming expected from CO2 increases. Using projected trends of CO2, N2O, CH4 and CFCs, our calculations showed that the annual mean and global mean surface temperature could warm by as much as 2.5 °C with larger warming at high latitudes by the middle of the next century. The calculations also suggest that the warming in the lower stratosphere and upper troposphere is much larger than that at the surface, especially during the summertime. Large stratosphere cooling is calculated with maximum cooling of ~ 12 °C around 45 km, where O3 depletion caused by increases of trace gases contributes substantially to the total cooling. However, the effects of O3 changes on the temperatures below 40 km appear to be small because of the small changes calculated in the O3 distribution.
Submitted on Nov 19, 2022
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References
Blake , D. R. and Rowland , F. S . 1988. Continuing worldwide increase in tropospheric methane, 1978 to 1987. Science 239, 1129 - 1131 .
Bowman , K. P. and Krueger , A. J . 1985 . A global climatology of total ozone from the Nimbus 7 Total Ozone Mapping Spectrometer. J . Geophys. Res. 90 , D5 , 7967 – 7976 .
Chemical Manufacturers Association (CMA), 1986. Production, sales and calculated release of CFC-11 and CFC-12 through 1985. Chemical Manufacturers Association, 2501 M Street NW, Washington DC, October, 1986.
Cunnold , D. M. , Prinn , R. G. , Rasmussen , R. A. , Simmonds , P. G. , Alyea , F. N. , Cardelino , C. A. , Crawford , A. J. , Fraser , P. J. and Rosen , R. D . 1986 . Atmospheric lifetime and annual release estimates for CFC13 and CF2C12 from 5 years of ALE data . J. Geophys. Res. 91 , 10797 – 10817 .
**DOE.**1985a . Atmospheric carbon dioxide and global carbon cycle (eds. M. C. MacCracken and F. M. Luther ). Report ER-0239, US Department of Energy , Washington DC , 315 pp .
DOE. 1985b . Projecting the climatic effects of increasing carbon dioxide (eds. M. C. MacCracken and F. M. Luther ). Report ER-0237, US Department of Energy , Washington DC , 381 pp .
Eckman , R. S. , Haigh , J. D. and Pyle , J. A . 1987 . An important uncertainty in coupled chlorine-carbon dioxide studies of atmospheric ozone modification . _Nature_329 , 616 – 619 .
Gutowski , W. J. , Wang , W.-C. and Stone , P. H . 1985 . Effects of dynamic heat fluxes on model climate sensitivity: meridional sensible and latent heat fluxes . J. Geophys. Res. 90 , 13081 – 13086 .
Haigh , J. D . 1984 . Radiative heating in the lower stratosphere and the distribution of ozone in a two-dimensional model . Quart. J. R. Met. Soc. 110 , 167 – 185 .
Haigh , J. D. and Pyle , J. A . 1982 . Ozone perturbation experiments in a two-dimensional circulation model . Quart. J. R. Met. Soc. 108 , 551 – 574 .
Hansen , J. , Lacis , A. , Rind , D. , Russell , G. , Stone , P. , Fung , I. , Ruedy , R. and Lerner , J . 1984. Climate sensitivity: Analysis of feedback mechanisms. In: Climate processes and climate sensitivity,Geophys. Monogr. Ser., vol. 29 (eds. J. E. Hansen and T. Takahashi ). Washington, DC: AGU, 130 – 163.
Hansen , J. and Lebedeff , S . 1987 . Global trends of measured surface air temperature . J. Geophys. Res. 92 , 13345 – 13372 .
Khalil , M. A. K. and Rasmussen , R. A . 1986 . Interannual variability of atmospheric methane: possible effects of the El Nifio-Southern Oscillation . _Science_232 , 56 – 58 .
Khalil , M. A. K. and Rasmussen , R. A . 1989 . Climate-induced feedbacks for the global cycles of methane and nitrous oxide . Tellus , in press .
Ko , M. K. W. , Sze , N. D. , Livshits , M. , McElroy , M. B. and Pyle , J. A . 1984 . The seasonal and lati-tudinal behavior of trace gases and 03 as simulated by a two-dimensional model of the atmosphere . J. Atmos. Sci. 41 , 2381 – 2408 .
Ko , M. K. W. , Tung , K. K. , Weisenstein , D. K. and Sze , N. D . 1985a . A zonal-mean model of strato-spheric tracer transport in isentropic coordinates : Numerical simulations for nitrous oxide and nitric acid. J. Geophys. Res. 90 , 2313 – 2329 .
Ko , M. K. W. , Weisenstein , D. K. , Sze , N. D. and Tung , K. K . 1985b. Simulation of 03 distribution using a two-dimensional zonal-mean model in isentropic coordinate. In: Atmospheric ozone (eds. C. S. Zerofos and A. Ghazi ). _Dordrecht/Boston/ Lancaster: D. Reidel Publ. Co.,_19 – 23.
Lacis , A. and Hansen , J . 1974 . A parameterization for the absorption of solar radiation in the earth's atmosphere . J. Atmos. Sci. 31 , 118 – 133 .
Logan , J. A . 1985 . Tropospheric ozone: seasonal behaviour, trends and anthropogenic influence . J. Geophys. Res. 90 , 10463 – 10482 .
Luther , F. , Wuebbles , D. J. and Chang , J. S . 1977 . Temperature feedback in a stratospheric model . J. Geophys. Res. 82 , 4935 – 4942 .
Murgatroyd , R. J. and Singleton , F . 1961 . Possible meridional circulation in the stratosphere and mesophere . Quart. J. Roy. Meteor. Soc. 87 , 125 – 135 .
NASA/JPL. 1985 . Chemical Kinetics and Photo-chemical Data for Use in Stratospheric Modeling, Evaluation Number 7. NASA Panel for Data Evaluation, JPL Publication, 85-37, Jet Propulsion Laboratory, Pasadena, California.
Oort , A. H . 1971 . The observed annual cycle in the meridional transport of atmospheric energy . J. Atmos. Sci. 28 , 235 – 339 .
Oort , A. G. , Yonder Haar , T. H . 1976 . On the observed annual cycle in the ocean-atmosphere heat balance over the northern hemisphere . J. Phys. Oceanogr. 6 , 781 – 800 .
Pearman , G. I. , Etheridge , D ., deSilva , F. and Fraser , P. 1986. Evidence of changing concentrations of atmospheric CO2, N20 and CH4 from air bubbles in Antarctic ice. Nature 320 , 248 – 250
Ramanathan , V. , Callis , L. , Cess , R. , Hansen , J. , Isaksen , I. , Kuhn , W. , Luther , F. , Mahlman , J. , Reck , R. and Schlesinger , M . 1987 . Climate-chemical interactions and effects of changing atmospheric trace gases . Rev. Geophys. 25 , 1441 – 1482 .
Rinsland , C. P. , Levine , J. S. and Miles , T . 1985 . Concentration of methane in the troposphere deduced from 1951 infrared solar spectra . _Nature_318 , 245 – 249 .
Stone , P. H . 1984. Feedbacks between dynamical heat fluxes and temperature in the atmosphere. In: Climate processes and climate sensitivity, Geophys., Monogr. Ser., vol. 29 (eds. J. Hansen and T. Takahashi ). Washington, DC: AGU, 6 – 17.
UN EP. 1987 . Montreal Protocol on substances that deplete the ozone layer. The United Nations Environmental Programme . Final Act. UN : New York .
Wang , W.-C. and Molnar , G . 1985 . A model study of the greenhouse effects due to increasing atmospheric CH4, N20, CF2C12 and CFC13 . J. Geophys. Res. 90 , 12971 – 12980 .
Wang , W.-C. , Molnar , G. , Mitchell , T. P. and Stone , P. H . 1984 . Effects of dynamical heat fluxes on model climate sensitivity . J. Geophys. Res. 89 , 4699 – 4711 .
Wang , W.-C. and Ryan , P. B . 1983 . Overlapping effect of atmospheric H20, CO2, and 03 on the CO2 radiative effect . _Tellus_35B , 81 – 91 .
Wang , W.-C. and Sze , N. D . 1980 . Coupled effects of atmospheric N20 and 03 on the earth's climate . _Nature_286 , 589 – 590 .
Wang , W.-C. , Wuebbles , D. , Washington , W. M. , Isaacs , R. G. and Molnar , G . 1986 . Trace gases and other potential perturbations to global climate . Rev. Geophys. 24 , 110 – 140 .
Washington , W. M. and Meehl , G. A . 1984 . Seasonal cycle experiments on the climate sensitivity due to a doubling of CO2 with an atmospheric general circu-lation model coupled to a simple mixed layer ocean model . J. Geophys. Res. 89 , 9475 – 9503 .
Wetherald , R. T. and Manabe , S . 1981 . Influence of seasonal variation upon the sensitivity of a model climate . J. Geophys. Res. 88 , 6600 – 6610 .
WMO. 1986 . Atmospheric ozone 1985. Global Ozone Research and Monitoring Project, Report No. 16, World Meteorological Organization, Geneva, 1095 pp.