Raffaele Lamanna | ENEA, Italian National Agency for New Technologies, Energy and Sustainable Economic Development (original) (raw)
Papers by Raffaele Lamanna
IEEE Transactions on Applied Superconductivity, 2016
Annual Reports on NMR Spectroscopy, 2013
J Amer Oil Chem Soc, 2002
In order to differentiate milks from different species, we carried out a comparative analysis of ... more In order to differentiate milks from different species, we carried out a comparative analysis of TAG from cow, buffalo, goat, and sheep milk fat based on 13 C NMR experiments. NMR spectroscopy, although less sensitive than other techniques, does not require an extensive chemical manipulation of samples and can easily highlight the differences in the content of short-chain acyl groups in the four milk species. The resonances were assigned and quantified, and by using only three NMR parameters in data clustering with fuzzy logic analysis, we were able to distinguish goats' milk from sheep's milk, and both of these milks from cows' and buffaloes' milks. This appears to be an important result, considering the ease and rapidity with which milk identification can be obtained. From 13 C NMR spectra of TAG, the positional distribution of FA chains on the glycerol backbone can also be easily evaluated.
Chemical Physics, 1996
Density and water self-diffusion in ethanol-water mixtures are measured as a function of the temp... more Density and water self-diffusion in ethanol-water mixtures are measured as a function of the temperature and for several alcohol concentrations in the water rich region. An extension of the five species model for liquid water, in which H bond cooperativity is taken into account, is proposed to interpret the temperature and concentration trends of the mixture density, solvent self-diffusion and near infrared spectra. This approach allowed us to extract some significant parameters characteristic of the solvent water H bond network such as the probability of forming H bonds, the degree of cooperativity, the supercooling and superheating limit temperatures and the distribution of water molecules among the five species. The emerging picture suggests that alcohol acts upon the water H bond network as a structure maker in the normal temperature region and, probably, as a structure breaker in the supercooled one. Moreover, a progressive disappearance of the H bond network cooperativity is observed as the alcohol concentration is increased.
The Neuroradiology Journal, 2000
Physical review. E, Statistical physics, plasmas, fluids, and related interdisciplinary topics, 1995
The lifetime of the H bond network has been calculated as a function of temperature by a statisti... more The lifetime of the H bond network has been calculated as a function of temperature by a statistical five-species model for water in which the H bond cooperativity has been explicitly taken into account. While, on one hand, the Arrhenius behavior of the depolarized Rayleigh scattering data existing in an intermediate temperature region is well reproduced, the model predicts that
Physical review. E, Statistical physics, plasmas, fluids, and related interdisciplinary topics, 1994
Some thermodynamic and transport properties of normal and supercooled water have been interpreted... more Some thermodynamic and transport properties of normal and supercooled water have been interpreted in the framework of a dynamic extension of the polychromatic percolation model in which both the recently reported evidence for a temperature-dependent H-bond cooperativity and free-volume fluctuations within the percolative patches are included. The proposed model, which allowed us to fit the experimental self-diffusion data as a
Journal of Dairy Science, 2000
Triacylglycerols from cows and buffaloes' milk fat were investigated by 13 C nuclear magnetic res... more Triacylglycerols from cows and buffaloes' milk fat were investigated by 13 C nuclear magnetic resonance (NMR) spectroscopy. By the addition of pure triacylglycerols standards, we identified the resonances of both milk fats, and the peaks were used for qualitative and quantitative analysis of acyl groups. Multivariate analysis treatment of triacylglycerols distribution and composition parameters enabled us to identify milk. This study shows that NMR can safely be used to quantitate milk fatty acid content, providing unique information for milk identification of different animal species. (Key words: buffaloes' milk, milk fat, triacylglycerols, 13 C-nuclear magnetic resonance)
Physical Review E, 1994
The Stokes-Einstein equation is applied to the water self-diffusion coefficient D in human serum ... more The Stokes-Einstein equation is applied to the water self-diffusion coefficient D in human serum albumin protein solutions. A linear trend for D as a function of T/eta is found for all the protein concentrations investigated. However, the indication of a violation of the Stokes-Einstein equation is found in the protein concentration dependence of the effective hydrodynamic radius of water. The
Il Nuovo Cimento D, 1991
Summary Water proton spin-lattice relaxation and self-diffusion in aqueous solutions of human se... more Summary Water proton spin-lattice relaxation and self-diffusion in aqueous solutions of human serum albumin have been studied by1H NMR as a function of the protein concentration. Spin-lattice relaxation data, which display a nonlinear behaviour with the protein concentration, could be fitted with a two-phase model taking into account the experimentally determined hydration («bound») water values. Despite a similar trend is registered
International Journal of Pharmaceutics, 2009
Hydrogels have been widely used in tissue engineering as a support for tissue formation and/or to... more Hydrogels have been widely used in tissue engineering as a support for tissue formation and/or to deliver drug locally. A novel procedure for the in situ rapid chemical gelation of aqueous solutions of hyaluronan (HA) was employed. HA was functionalised with an arm bearing a terminal azido group (HAAA). When HAAA was mixed with a series of dialkyne reagents of different length, a 1,3-dipolar cycloaddition ("clickchemistry") reaction took place in the presence of catalytic amount of Cu(I) resulting in fast gelation at room temperature. The resulting gels were characterised in terms of degree of cross-linking by 1 H HR-MAS NMR. The kinetic of gelation and the determination of elastic moduli as well as the degree of swelling and the controlled release of a model drug, were studied as a function of chemical nature of the dialkyne group, catalyst concentration, HAAA concentration and temperature. All these variables allowed the swelling ratio and the extent of release of a drug, doxorubicin, entrapped within the gel, to be modulated. In all cases the kinetic of release reached the stationary state within 150 h. The height of the plateau was dependent on the overall (chemical and topological) degree of cross-linking.
Polymer, 2015
Hybrid foams based on polyurethane and polysiloxane-domains were designed in terms of chemical st... more Hybrid foams based on polyurethane and polysiloxane-domains were designed in terms of chemical structure and hierarchical morphology to improve the thermal insulation capability of conventional polyurethane foams. Polysiloxane-domains by solegel approach reacted with polyols to produce a polysiloxane-reactive-adduct, which completed its formation into polysiloxane aerogel-like structure during the polyurethane foaming process. Hybrids with 5wt% of the polysiloxane-domains exhibited a 22% reduction in thermal conductivity in comparison with pristine PUR. The chemical structure and the hierarchical morphology were studied by means of SAXS/WAXS and 29 Si and 13 C NMR. In particular the hybrid structure consisted of coarse polysiloxane-fractal-aggregates composed of silica nanoparticles embedded in the polyurethane matrix. Morphological analysis revealed a decrease of the cell size with the increase of the siloxane content ascribed to the nucleation effect of polysiloxane-domains during the foaming. The cell size reduction and the formation of hybrid-aerogel-like structures within the cell-walls are considered the key factors to reduce the thermal conductivity of hybrid foams.
Journal of Apicultural Research, 2013
ABSTRACT Freshness and authenticity of Chinese and Italian royal jelly samples were investigated ... more ABSTRACT Freshness and authenticity of Chinese and Italian royal jelly samples were investigated by means of HPLC determination of furosine and (E)-10-hydroxy-2-decenoic acid. In addition, High Resolution Magic Angle Spinning Nuclear Magnetic Resonance (HR-MAS NMR) spectroscopy was used to determine the metabolic profile of the same royal jelly samples. water-soluble metabolites such as amino acids and sugars as well as fatty acids were identified in the same experiment. A combined approach including NMR analytical profile together with HPLC measured markers was used to discriminate between Italian and Chinese samples by means of Principal Component Analysis.
Journal of Physical Chemistry C, 2008
ABSTRACT
Microporous and Mesoporous Materials, 2012
ABSTRACT A novel porous polyurethane (PU) hybrid foam was designed to improve the hydrophilicity ... more ABSTRACT A novel porous polyurethane (PU) hybrid foam was designed to improve the hydrophilicity of a conventional open pore PU foam, and to enhance the adsorption of carcinogenic compounds from tobacco smoke.The hybrid foam was prepared by interdispersing ultramilled alumina particles within PU precursors to realize a PU/Al2O3 hybrid porous material with well controlled microstructural properties and improved hydrophilicity. The capability of the as obtained hybrid foam to adsorb toxic compounds from the mainstream of tobacco smoke was investigated by using a cellulose-active carbon-cellulose triple filter model, and the results were compared to those obtained for neat PU foam and the standard cigarette filter tip.The results of this study showed that the ultramilled alumina particles enhanced both thermal stability and hydrophilicity of the neat PU foam. Furthermore, the as-obtained hybrid PU/Al2O3 foam was able to improve the adsorption of nitrosamines, acetamide, idroquinone, cresol and small aminic and aldehydic molecules, if compared to neat PU foam and standard cigarette filter tip, evidencing potential as tobacco smoke filter.
Measurement Science and Technology, 1991
ABSTRACT A crossed-coil probe for solid-state NMR with a recovery time of 5 mu s at 10 MHz has be... more ABSTRACT A crossed-coil probe for solid-state NMR with a recovery time of 5 mu s at 10 MHz has been constructed. The transitory Q damping performed on the transmitting coil, together with a simultaneous grounding of the receiving coil, provides a significant reduction in the probe ringing-down time without degradation of the signal-to-noise ratio. Since no particular isolation between the two sections is required, the system is very simple to produce.
Magnetic Resonance in Chemistry, 2006
Carotenoids are linear C 40 tetraterpenoid hydrocarbons and represent a wide category of natural ... more Carotenoids are linear C 40 tetraterpenoid hydrocarbons and represent a wide category of natural pigments. They are components of the pigment system of chloroplasts and are involved in the primary light absorption and the photon canalization of photosynthesis. Moreover, they also behave as quenchers of singlet oxygen, protecting cells and organisms against lipid peroxidation.
Magnetic Resonance in Chemistry, 2003
... of high-resolution 1H NMR spectroscopy to dis-criminate between numerous compounds in complex... more ... of high-resolution 1H NMR spectroscopy to dis-criminate between numerous compounds in complex solu-tions has found many new applications in food science.14 Recently, the potential usefulness of high-resolution1H NMR spectroscopy in the analysis of fruit juices and ...
Magnetic Resonance in Chemistry, 2008
This preliminary work deals with the influence of packaging on the degradation of an Italian soft... more This preliminary work deals with the influence of packaging on the degradation of an Italian soft cheese studied by NMR. The NMR profiles of aqueous cheese extracts were acquired as a function of time during storage of cheese inside and outside the original package. From the NMR spectra 15 metabolites are quantified and used in a kinetic degradation model and in a multivariate algorithm in order to evaluate the changes in the metabolic composition of cheese stored under different conditions.
IEEE Transactions on Applied Superconductivity, 2016
Annual Reports on NMR Spectroscopy, 2013
J Amer Oil Chem Soc, 2002
In order to differentiate milks from different species, we carried out a comparative analysis of ... more In order to differentiate milks from different species, we carried out a comparative analysis of TAG from cow, buffalo, goat, and sheep milk fat based on 13 C NMR experiments. NMR spectroscopy, although less sensitive than other techniques, does not require an extensive chemical manipulation of samples and can easily highlight the differences in the content of short-chain acyl groups in the four milk species. The resonances were assigned and quantified, and by using only three NMR parameters in data clustering with fuzzy logic analysis, we were able to distinguish goats' milk from sheep's milk, and both of these milks from cows' and buffaloes' milks. This appears to be an important result, considering the ease and rapidity with which milk identification can be obtained. From 13 C NMR spectra of TAG, the positional distribution of FA chains on the glycerol backbone can also be easily evaluated.
Chemical Physics, 1996
Density and water self-diffusion in ethanol-water mixtures are measured as a function of the temp... more Density and water self-diffusion in ethanol-water mixtures are measured as a function of the temperature and for several alcohol concentrations in the water rich region. An extension of the five species model for liquid water, in which H bond cooperativity is taken into account, is proposed to interpret the temperature and concentration trends of the mixture density, solvent self-diffusion and near infrared spectra. This approach allowed us to extract some significant parameters characteristic of the solvent water H bond network such as the probability of forming H bonds, the degree of cooperativity, the supercooling and superheating limit temperatures and the distribution of water molecules among the five species. The emerging picture suggests that alcohol acts upon the water H bond network as a structure maker in the normal temperature region and, probably, as a structure breaker in the supercooled one. Moreover, a progressive disappearance of the H bond network cooperativity is observed as the alcohol concentration is increased.
The Neuroradiology Journal, 2000
Physical review. E, Statistical physics, plasmas, fluids, and related interdisciplinary topics, 1995
The lifetime of the H bond network has been calculated as a function of temperature by a statisti... more The lifetime of the H bond network has been calculated as a function of temperature by a statistical five-species model for water in which the H bond cooperativity has been explicitly taken into account. While, on one hand, the Arrhenius behavior of the depolarized Rayleigh scattering data existing in an intermediate temperature region is well reproduced, the model predicts that
Physical review. E, Statistical physics, plasmas, fluids, and related interdisciplinary topics, 1994
Some thermodynamic and transport properties of normal and supercooled water have been interpreted... more Some thermodynamic and transport properties of normal and supercooled water have been interpreted in the framework of a dynamic extension of the polychromatic percolation model in which both the recently reported evidence for a temperature-dependent H-bond cooperativity and free-volume fluctuations within the percolative patches are included. The proposed model, which allowed us to fit the experimental self-diffusion data as a
Journal of Dairy Science, 2000
Triacylglycerols from cows and buffaloes' milk fat were investigated by 13 C nuclear magnetic res... more Triacylglycerols from cows and buffaloes' milk fat were investigated by 13 C nuclear magnetic resonance (NMR) spectroscopy. By the addition of pure triacylglycerols standards, we identified the resonances of both milk fats, and the peaks were used for qualitative and quantitative analysis of acyl groups. Multivariate analysis treatment of triacylglycerols distribution and composition parameters enabled us to identify milk. This study shows that NMR can safely be used to quantitate milk fatty acid content, providing unique information for milk identification of different animal species. (Key words: buffaloes' milk, milk fat, triacylglycerols, 13 C-nuclear magnetic resonance)
Physical Review E, 1994
The Stokes-Einstein equation is applied to the water self-diffusion coefficient D in human serum ... more The Stokes-Einstein equation is applied to the water self-diffusion coefficient D in human serum albumin protein solutions. A linear trend for D as a function of T/eta is found for all the protein concentrations investigated. However, the indication of a violation of the Stokes-Einstein equation is found in the protein concentration dependence of the effective hydrodynamic radius of water. The
Il Nuovo Cimento D, 1991
Summary Water proton spin-lattice relaxation and self-diffusion in aqueous solutions of human se... more Summary Water proton spin-lattice relaxation and self-diffusion in aqueous solutions of human serum albumin have been studied by1H NMR as a function of the protein concentration. Spin-lattice relaxation data, which display a nonlinear behaviour with the protein concentration, could be fitted with a two-phase model taking into account the experimentally determined hydration («bound») water values. Despite a similar trend is registered
International Journal of Pharmaceutics, 2009
Hydrogels have been widely used in tissue engineering as a support for tissue formation and/or to... more Hydrogels have been widely used in tissue engineering as a support for tissue formation and/or to deliver drug locally. A novel procedure for the in situ rapid chemical gelation of aqueous solutions of hyaluronan (HA) was employed. HA was functionalised with an arm bearing a terminal azido group (HAAA). When HAAA was mixed with a series of dialkyne reagents of different length, a 1,3-dipolar cycloaddition ("clickchemistry") reaction took place in the presence of catalytic amount of Cu(I) resulting in fast gelation at room temperature. The resulting gels were characterised in terms of degree of cross-linking by 1 H HR-MAS NMR. The kinetic of gelation and the determination of elastic moduli as well as the degree of swelling and the controlled release of a model drug, were studied as a function of chemical nature of the dialkyne group, catalyst concentration, HAAA concentration and temperature. All these variables allowed the swelling ratio and the extent of release of a drug, doxorubicin, entrapped within the gel, to be modulated. In all cases the kinetic of release reached the stationary state within 150 h. The height of the plateau was dependent on the overall (chemical and topological) degree of cross-linking.
Polymer, 2015
Hybrid foams based on polyurethane and polysiloxane-domains were designed in terms of chemical st... more Hybrid foams based on polyurethane and polysiloxane-domains were designed in terms of chemical structure and hierarchical morphology to improve the thermal insulation capability of conventional polyurethane foams. Polysiloxane-domains by solegel approach reacted with polyols to produce a polysiloxane-reactive-adduct, which completed its formation into polysiloxane aerogel-like structure during the polyurethane foaming process. Hybrids with 5wt% of the polysiloxane-domains exhibited a 22% reduction in thermal conductivity in comparison with pristine PUR. The chemical structure and the hierarchical morphology were studied by means of SAXS/WAXS and 29 Si and 13 C NMR. In particular the hybrid structure consisted of coarse polysiloxane-fractal-aggregates composed of silica nanoparticles embedded in the polyurethane matrix. Morphological analysis revealed a decrease of the cell size with the increase of the siloxane content ascribed to the nucleation effect of polysiloxane-domains during the foaming. The cell size reduction and the formation of hybrid-aerogel-like structures within the cell-walls are considered the key factors to reduce the thermal conductivity of hybrid foams.
Journal of Apicultural Research, 2013
ABSTRACT Freshness and authenticity of Chinese and Italian royal jelly samples were investigated ... more ABSTRACT Freshness and authenticity of Chinese and Italian royal jelly samples were investigated by means of HPLC determination of furosine and (E)-10-hydroxy-2-decenoic acid. In addition, High Resolution Magic Angle Spinning Nuclear Magnetic Resonance (HR-MAS NMR) spectroscopy was used to determine the metabolic profile of the same royal jelly samples. water-soluble metabolites such as amino acids and sugars as well as fatty acids were identified in the same experiment. A combined approach including NMR analytical profile together with HPLC measured markers was used to discriminate between Italian and Chinese samples by means of Principal Component Analysis.
Journal of Physical Chemistry C, 2008
ABSTRACT
Microporous and Mesoporous Materials, 2012
ABSTRACT A novel porous polyurethane (PU) hybrid foam was designed to improve the hydrophilicity ... more ABSTRACT A novel porous polyurethane (PU) hybrid foam was designed to improve the hydrophilicity of a conventional open pore PU foam, and to enhance the adsorption of carcinogenic compounds from tobacco smoke.The hybrid foam was prepared by interdispersing ultramilled alumina particles within PU precursors to realize a PU/Al2O3 hybrid porous material with well controlled microstructural properties and improved hydrophilicity. The capability of the as obtained hybrid foam to adsorb toxic compounds from the mainstream of tobacco smoke was investigated by using a cellulose-active carbon-cellulose triple filter model, and the results were compared to those obtained for neat PU foam and the standard cigarette filter tip.The results of this study showed that the ultramilled alumina particles enhanced both thermal stability and hydrophilicity of the neat PU foam. Furthermore, the as-obtained hybrid PU/Al2O3 foam was able to improve the adsorption of nitrosamines, acetamide, idroquinone, cresol and small aminic and aldehydic molecules, if compared to neat PU foam and standard cigarette filter tip, evidencing potential as tobacco smoke filter.
Measurement Science and Technology, 1991
ABSTRACT A crossed-coil probe for solid-state NMR with a recovery time of 5 mu s at 10 MHz has be... more ABSTRACT A crossed-coil probe for solid-state NMR with a recovery time of 5 mu s at 10 MHz has been constructed. The transitory Q damping performed on the transmitting coil, together with a simultaneous grounding of the receiving coil, provides a significant reduction in the probe ringing-down time without degradation of the signal-to-noise ratio. Since no particular isolation between the two sections is required, the system is very simple to produce.
Magnetic Resonance in Chemistry, 2006
Carotenoids are linear C 40 tetraterpenoid hydrocarbons and represent a wide category of natural ... more Carotenoids are linear C 40 tetraterpenoid hydrocarbons and represent a wide category of natural pigments. They are components of the pigment system of chloroplasts and are involved in the primary light absorption and the photon canalization of photosynthesis. Moreover, they also behave as quenchers of singlet oxygen, protecting cells and organisms against lipid peroxidation.
Magnetic Resonance in Chemistry, 2003
... of high-resolution 1H NMR spectroscopy to dis-criminate between numerous compounds in complex... more ... of high-resolution 1H NMR spectroscopy to dis-criminate between numerous compounds in complex solu-tions has found many new applications in food science.14 Recently, the potential usefulness of high-resolution1H NMR spectroscopy in the analysis of fruit juices and ...
Magnetic Resonance in Chemistry, 2008
This preliminary work deals with the influence of packaging on the degradation of an Italian soft... more This preliminary work deals with the influence of packaging on the degradation of an Italian soft cheese studied by NMR. The NMR profiles of aqueous cheese extracts were acquired as a function of time during storage of cheese inside and outside the original package. From the NMR spectra 15 metabolites are quantified and used in a kinetic degradation model and in a multivariate algorithm in order to evaluate the changes in the metabolic composition of cheese stored under different conditions.