Michel Fromm | Université de Franche-Comté (original) (raw)

Michel Fromm

I was born in Colmar, France in 1962. I received the Ph.D. degree in 1990 from the Université de Franche-Comté, France. After a three year position as Research Engineer in Electron Microscopy at the Faculty of Pharmacy and Medecine of Besançon I held an Assistant Professor position in Physical Chemistry at the University of Franche-Comté in 1993. In 2002, I was designated Director of the Laboratoire de Microanalyses Nucleaires-Alain Chambaudet of the same university. In 2003, I became Professor at the Université de Franche-Comté in Physical Chemistry and in the same year the laboratory became a Mix Unit of the French Atomic Agency (CEA). Today, this unit is integrated in the mixt unit of the French National Center for Scientific Research (CNRS)

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Papers by Michel Fromm

Research paper thumbnail of Distribution of radial dose in water at nanometer scale for ions of the same linear energy transfer: benefits of the concept of annular dose

Physica Scripta

Annular-dose AD is a new conception , based on the radial dose distribution, RDD, introduced by t... more Annular-dose AD is a new conception , based on the radial dose distribution, RDD, introduced by the present work. AD is the integrated dose for many shells around the ions and it is defined as the dose deposited in the shell volume perpendicular to the ion path of width ( r = 0.1 → R min ) , length equal 2 π and thickness equal unity (1 nm). Thus, it integrates and maps the deposited dose due to ion in any medium at nanometer scale better than the ordinary radial dose. Katz and Awad radial dose formulae plus Butts-Katz and Tabata electron range-energy relations are composing three different approaches. These approaches were used for studying the AD for 30 ions forming 4 different equal LET groups and have energy at Bragg peak region from 1.5 to 24 MeV n−1. The annular dose, AD as a function of the shell width for the ions under investigation showed that dose distributions around the ions of same LET are not the same and a clear peak at certain shell width called the ion’s maximum an...

Research paper thumbnail of A thorough examination of swift ion latent track formation and etching in PADC (Review)

Research paper thumbnail of revised version of Low energy electrons and swift ion track structure in PADC (RPC)

Research paper thumbnail of TECHNICAL ADVANCE Production and Validation of CR-39-Based Dishes for a-Particle Radiobiological Experiments

Research paper thumbnail of The contribution of hydrogen peroxide to the radiosensitizing effect of gold nanoparticles

Colloids and Surfaces B: Biointerfaces, 2018

Research paper thumbnail of Auto-assembly of nanometer thick, water soluble layers of plasmid DNA complexed with diamines and basic amino acids on graphite: Greatest DNA protection is obtained with arginine

Materials Science and Engineering: C, 2017

Research paper thumbnail of Complexation des acides aminés basiques arginine, histidine et lysine avec l’ADN plasmidique en solution aqueuse : participation à la capture de radicaux sous irradiation X à 1,5 keV

EPJ Web of Conferences, 2016

Research paper thumbnail of Low energy electrons and ultra-soft X-rays irradiation of plasmid DNA. Technical innovations

Radiation Physics and Chemistry, 2016

Research paper thumbnail of 19th International Conference on Nuclear Tracks in Solids (ICNTSs)

Research paper thumbnail of Ion-kill dosimetry

Physica medica : PM : an international journal devoted to the applications of physics to medicine and biology : official journal of the Italian Association of Biomedical Physics (AIFB), 2001

Unanticipated late effects in neutron and heavy ion therapy, not attributable to overdose, imply ... more Unanticipated late effects in neutron and heavy ion therapy, not attributable to overdose, imply a qualitative difference between low and high LET therapy. We identify that difference as 'ion kill', associated with the spectrum of z/beta in the radiation field, whose measurement we label 'ion-kill dosimetry'.

Research paper thumbnail of Le tritium de l'Ecosystème à l'Homme-Etude des mécanismes et des constantes qui régissent les équilibres et différentes voies de transfert

Research paper thumbnail of Etched track profiles for relativistic 7 GeV silicon and 17.48 GeV Nickel ions in PADC detector: The case study of convex track walls

Radiation Physics and Chemistry, 2021

Research paper thumbnail of Inter-comparison of geometrical track parameters and depth dependent track etch rates measured for Li-7 ions in two types of CR-39

Radiation Measurements, 2001

Research paper thumbnail of Role of intermediate species in the formation of an energetic ion latent track in PADC: A review

Polymer Degradation and Stability, 2019

Abstract This review paper intends at identifying the early processes arising during the formatio... more Abstract This review paper intends at identifying the early processes arising during the formation of a latent ion track in Poly Allyl Diglycol Carbonate (PADC). We briefly summarize the physical and chemical processes specific to the description of the interaction of ionizing radiation with matter. Then we gather published information in relation to PADC response regarding energy absorption and further transient species formation. Emphasis is given to the chemistry of radicals. Due to a lack of available data in relation with clearly identified unpaired electron carriers in PADC, we use data stemming from surrogate molecules. Based on such data we suggest mechanisms for the decomposition of PADC during the early times of ion track formation. The α-sites of ether functional groups in PADC appear undoubtedly as critical targets which during further decomposition behave as the most probable origin of Carbon dioxide release. All suggested mechanisms are multi-step processes. Combining different concepts and data in relation with the dynamics of transient species formed in the ion track of a polymer material, we propose that the effective track radius may be described as the radial extension of reactive species formed rather than the maximum distance at which δ-rays escape out of ion's trajectory. Lastly, generalization of the different processes collected allows two major pathways to be proposed for describing the fate of damaged ether moieties in PADC. This way, evidence is given for a higher sensitivity of ether functional groups compared to ester carbonate ones. The latter generally being destroyed as a consequence of prior damaging of the ether group. Discussion presented here is of interest to the nuclear track community.

Research paper thumbnail of Elucidation of the Two-Step Damage Formation Process of Latent Tracks in Poly(allyl diglycol carbonate), PADC: Role of Secondary Low-Energy Electrons

The Journal of Physical Chemistry C

Research paper thumbnail of Methionine oxidation by hydrogen peroxide in peptides and proteins: A theoretical and Raman spectroscopy study

Journal of photochemistry and photobiology. B, Biology, 2018

The oxidation of proteins results in their deterioration via the oxidation of reactive amino acid... more The oxidation of proteins results in their deterioration via the oxidation of reactive amino acids. Oxidation of the amino acid, methionine plays an important role during biological conditions of oxidative stress, and equally a role in protein stability. In this study the oxidation of the methionine residue using the tripeptide GlyMetGly with respect to hydrogen peroxide has been studied using both Raman spectroscopy and DFT calculations. Spectral modifications following the formation of methionine sulfoxide are shown with the appearance of the SO vibration whilst there is also the modification of the CS vibrations at approximately 700 cm. The changes in the intensity of the CS stretching band were used to calculate the kinetic rate constant as 7.9 ± 0.6 × 10 dm mol s. The energy barrier for the reaction. is determined both experimentally and using DFT calculations. The reaction of the dairy protein beta-lactoglobulin with hydrogen peroxide is equally studied using the same techniqu...

Research paper thumbnail of Propagation Distance of the alpha-Particle-Induced Bystander Effect: The Role of Nuclear Traversal and Gap Junction Communication

Radiation Research, Jun 1, 2009

Research paper thumbnail of Distance distribution of bystander effects in alpha-particle irradiated cell populations using a CR-39-based culture dish

Radiation Measurements, Aug 1, 2008

Research paper thumbnail of TDAB-induced DNA plasmid condensation on the surface of a reconstructed boron doped silicon substrate

Surface Science, Jan 7, 2013

Research paper thumbnail of Special issue - Proceedings of the 19th International Conference on Nuclear Tracks in Solids

Research paper thumbnail of Distribution of radial dose in water at nanometer scale for ions of the same linear energy transfer: benefits of the concept of annular dose

Physica Scripta

Annular-dose AD is a new conception , based on the radial dose distribution, RDD, introduced by t... more Annular-dose AD is a new conception , based on the radial dose distribution, RDD, introduced by the present work. AD is the integrated dose for many shells around the ions and it is defined as the dose deposited in the shell volume perpendicular to the ion path of width ( r = 0.1 → R min ) , length equal 2 π and thickness equal unity (1 nm). Thus, it integrates and maps the deposited dose due to ion in any medium at nanometer scale better than the ordinary radial dose. Katz and Awad radial dose formulae plus Butts-Katz and Tabata electron range-energy relations are composing three different approaches. These approaches were used for studying the AD for 30 ions forming 4 different equal LET groups and have energy at Bragg peak region from 1.5 to 24 MeV n−1. The annular dose, AD as a function of the shell width for the ions under investigation showed that dose distributions around the ions of same LET are not the same and a clear peak at certain shell width called the ion’s maximum an...

Research paper thumbnail of A thorough examination of swift ion latent track formation and etching in PADC (Review)

Research paper thumbnail of revised version of Low energy electrons and swift ion track structure in PADC (RPC)

Research paper thumbnail of TECHNICAL ADVANCE Production and Validation of CR-39-Based Dishes for a-Particle Radiobiological Experiments

Research paper thumbnail of The contribution of hydrogen peroxide to the radiosensitizing effect of gold nanoparticles

Colloids and Surfaces B: Biointerfaces, 2018

Research paper thumbnail of Auto-assembly of nanometer thick, water soluble layers of plasmid DNA complexed with diamines and basic amino acids on graphite: Greatest DNA protection is obtained with arginine

Materials Science and Engineering: C, 2017

Research paper thumbnail of Complexation des acides aminés basiques arginine, histidine et lysine avec l’ADN plasmidique en solution aqueuse : participation à la capture de radicaux sous irradiation X à 1,5 keV

EPJ Web of Conferences, 2016

Research paper thumbnail of Low energy electrons and ultra-soft X-rays irradiation of plasmid DNA. Technical innovations

Radiation Physics and Chemistry, 2016

Research paper thumbnail of 19th International Conference on Nuclear Tracks in Solids (ICNTSs)

Research paper thumbnail of Ion-kill dosimetry

Physica medica : PM : an international journal devoted to the applications of physics to medicine and biology : official journal of the Italian Association of Biomedical Physics (AIFB), 2001

Unanticipated late effects in neutron and heavy ion therapy, not attributable to overdose, imply ... more Unanticipated late effects in neutron and heavy ion therapy, not attributable to overdose, imply a qualitative difference between low and high LET therapy. We identify that difference as 'ion kill', associated with the spectrum of z/beta in the radiation field, whose measurement we label 'ion-kill dosimetry'.

Research paper thumbnail of Le tritium de l'Ecosystème à l'Homme-Etude des mécanismes et des constantes qui régissent les équilibres et différentes voies de transfert

Research paper thumbnail of Etched track profiles for relativistic 7 GeV silicon and 17.48 GeV Nickel ions in PADC detector: The case study of convex track walls

Radiation Physics and Chemistry, 2021

Research paper thumbnail of Inter-comparison of geometrical track parameters and depth dependent track etch rates measured for Li-7 ions in two types of CR-39

Radiation Measurements, 2001

Research paper thumbnail of Role of intermediate species in the formation of an energetic ion latent track in PADC: A review

Polymer Degradation and Stability, 2019

Abstract This review paper intends at identifying the early processes arising during the formatio... more Abstract This review paper intends at identifying the early processes arising during the formation of a latent ion track in Poly Allyl Diglycol Carbonate (PADC). We briefly summarize the physical and chemical processes specific to the description of the interaction of ionizing radiation with matter. Then we gather published information in relation to PADC response regarding energy absorption and further transient species formation. Emphasis is given to the chemistry of radicals. Due to a lack of available data in relation with clearly identified unpaired electron carriers in PADC, we use data stemming from surrogate molecules. Based on such data we suggest mechanisms for the decomposition of PADC during the early times of ion track formation. The α-sites of ether functional groups in PADC appear undoubtedly as critical targets which during further decomposition behave as the most probable origin of Carbon dioxide release. All suggested mechanisms are multi-step processes. Combining different concepts and data in relation with the dynamics of transient species formed in the ion track of a polymer material, we propose that the effective track radius may be described as the radial extension of reactive species formed rather than the maximum distance at which δ-rays escape out of ion's trajectory. Lastly, generalization of the different processes collected allows two major pathways to be proposed for describing the fate of damaged ether moieties in PADC. This way, evidence is given for a higher sensitivity of ether functional groups compared to ester carbonate ones. The latter generally being destroyed as a consequence of prior damaging of the ether group. Discussion presented here is of interest to the nuclear track community.

Research paper thumbnail of Elucidation of the Two-Step Damage Formation Process of Latent Tracks in Poly(allyl diglycol carbonate), PADC: Role of Secondary Low-Energy Electrons

The Journal of Physical Chemistry C

Research paper thumbnail of Methionine oxidation by hydrogen peroxide in peptides and proteins: A theoretical and Raman spectroscopy study

Journal of photochemistry and photobiology. B, Biology, 2018

The oxidation of proteins results in their deterioration via the oxidation of reactive amino acid... more The oxidation of proteins results in their deterioration via the oxidation of reactive amino acids. Oxidation of the amino acid, methionine plays an important role during biological conditions of oxidative stress, and equally a role in protein stability. In this study the oxidation of the methionine residue using the tripeptide GlyMetGly with respect to hydrogen peroxide has been studied using both Raman spectroscopy and DFT calculations. Spectral modifications following the formation of methionine sulfoxide are shown with the appearance of the SO vibration whilst there is also the modification of the CS vibrations at approximately 700 cm. The changes in the intensity of the CS stretching band were used to calculate the kinetic rate constant as 7.9 ± 0.6 × 10 dm mol s. The energy barrier for the reaction. is determined both experimentally and using DFT calculations. The reaction of the dairy protein beta-lactoglobulin with hydrogen peroxide is equally studied using the same techniqu...

Research paper thumbnail of Propagation Distance of the alpha-Particle-Induced Bystander Effect: The Role of Nuclear Traversal and Gap Junction Communication

Radiation Research, Jun 1, 2009

Research paper thumbnail of Distance distribution of bystander effects in alpha-particle irradiated cell populations using a CR-39-based culture dish

Radiation Measurements, Aug 1, 2008

Research paper thumbnail of TDAB-induced DNA plasmid condensation on the surface of a reconstructed boron doped silicon substrate

Surface Science, Jan 7, 2013

Research paper thumbnail of Special issue - Proceedings of the 19th International Conference on Nuclear Tracks in Solids

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