E. Gil-Santos - Academia.edu (original) (raw)

Papers by E. Gil-Santos

Journal of Applied Physics, 2020

In the last two decades, nano-mechanical resonators have risen as highly promising devices for ma... more In the last two decades, nano-mechanical resonators have risen as highly promising devices for mass sensing due to their ultrahigh sensitivity. They can be used to measure the mass and stiffness of single particles like small pollution particles, viruses, bacteria, or even proteins. These capabilities of the nano-mechanical resonators have allowed the birth of a new type of mass spectrometry with no need of fragmentation or ionization of the sample and therefore ideal to measure big masses, where conventional mass spectrometers have important problems. The shape and modes of vibration of a nano-mechanical resonator can be very different and the advantages and drawbacks of one respect to another is still a hot topic. A unified theoretical framework to describe the effect of particle adsorption on a mechanical resonator is fundamental but still lacks in the literature. In this work, we present such a framework and examine the particular case of a rod-like particle adsorbed on a cantil...

Proceedings, 2017

Cavity optomechanics have become a promising route towards the development of ultrasensitive sens... more Cavity optomechanics have become a promising route towards the development of ultrasensitive sensors for a wide range of applications including mass, chemical and biological sensing. We demonstrate the potential of Very Large Scale Integration (VLSI) with state-of-the-art low-loss performance silicon optomechanical microdisks for real-world applications. We report microdisks exhibiting optical Whispering Gallery Modes (WGM) with 1 million quality factors. These high-Q microdisks allow their Brownian motion to be resolved at few 100 MHz in ambient air. Such performance shows our VLSI process is a viable approach for the next generation of highend sensors operating in vacuum, gas or liquid phase.

Nature communications, Jan 11, 2016

The identification of species is a fundamental problem in analytical chemistry and biology. Mass ... more The identification of species is a fundamental problem in analytical chemistry and biology. Mass spectrometers identify species by their molecular mass with extremely high sensitivity (<10(-24) g). However, its application is usually limited to light analytes (<10(-19) g). Here we demonstrate that by using nanomechanical resonators, heavier analytes can be identified by their mass and stiffness. The method is demonstrated with spherical gold nanoparticles and whole intact E. coli bacteria delivered by electrospray ionization to microcantilever resonators placed in low vacuum at 0.1 torr. We develop a theoretical procedure for obtaining the mass, position and stiffness of the analytes arriving the resonator from the adsorption-induced eigenfrequency jumps. These results demonstrate the enormous potential of this technology for identification of large biological complexes near their native conformation, a goal that is beyond the capabilities of conventional mass spectrometers.

Physical Review Letters, 2017

Collective phenomena emerging from non-linear interactions between multiple oscillators, such as ... more Collective phenomena emerging from non-linear interactions between multiple oscillators, such as synchronization and frequency locking, find applications in a wide variety of fields. Optomechanical resonators, which are intrinsically non-linear, combine the scientific assets of mechanical devices with the possibility of long distance controlled interactions enabled by travelling light. Here we demonstrate light-mediated frequency locking of three distant nano-optomechanical oscillators positioned in a cascaded configuration. The oscillators, integrated on a chip along a coupling waveguide, are optically driven with a single laser and oscillate at gigahertz frequency. Despite an initial frequency disorder of hundreds of kilohertz, the guided light locks them all with a clear transition in the optical output. The experimental results are described by Langevin equations, paving the way to scalable cascaded optomechanical configurations.

In the last years, a large variety of ultrasensitive nanomechanical sensors have been developed a... more In the last years, a large variety of ultrasensitive nanomechanical sensors have been developed and used as biological sensors. The results demonstrate that rapid detection of biomolecules with high sensitivity and specificity without need of sample pre-treatment and labeling with fluorescent dyes is attainable(1). This technology has the potential to revolutionize the fields of molecular biology and preventive medicine. Here,

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The development of ultrasensitive protein spectrometers and ultrasensitive biological sensors wil... more The development of ultrasensitive protein spectrometers and ultrasensitive biological sensors will speed up the identification of disease biomarkers and their rapid detection [1, 2]. Nanomechanical resonators have emerged as promising candidates for ultrasensitive ...

Applied Physics Letters, 2013

Physical review letters, 2018

We report on a systematic study of nanomechanical dissipation in high-frequency (≈300 MHz) galli... more We report on a systematic study of nanomechanical dissipation in high-frequency (≈300 MHz) gallium arsenide optomechanical disk resonators, in conditions where clamping and fluidic losses are negligible. Phonon-phonon interactions are shown to contribute with a loss background fading away at cryogenic temperatures (3 K). Atomic layer deposition of alumina at the surface modifies the quality factor of resonators, pointing towards the importance of surface dissipation. The temperature evolution is accurately fitted by two-level systems models, showing that nanomechanical dissipation in gallium arsenide resonators directly connects to their microscopic properties. Two-level systems, notably at surfaces, appear to rule the damping and fluctuations of such high-quality crystalline nanomechanical devices, at all temperatures from 3 to 300 K.

Nature Nanotechnology, 2015

New Journal of Physics, 2015

We experimentally demonstrate the controlled enhancement of the mechanical quality factor Q of Ga... more We experimentally demonstrate the controlled enhancement of the mechanical quality factor Q of GaAs disk optomechanical resonators. Disks vibrating at 1.3 GHz with a mechanical shield integrated in their pedestal show a Q improvement by a factor 10 to 16. The structure is modeled numerically and different modes of vibration are observed, which shed light on the Q enhancement mechanism. An optimized double-disk geometry is presented that promises Q above the million for a large parameter range. Fig. 1: Scanning Electron Microscope (SEM) image of a fabricated shielded optomechanical disk resonator with its suspended optical coupling waveguide.

New Journal of Physics, 2013

We study optical back-action effects associated with confined electromagnetic modes in silicon na... more We study optical back-action effects associated with confined electromagnetic modes in silicon nanowire resonators interacting with a laser beam used for interferometric read-out of the nanowire vibrations. Our analysis describes the resonance frequency shift produced in the nanowires by two different mechanisms: the temperature dependence of the nanowire's Young's modulus and the effect of radiation pressure. We find different regimes in which each effect dominates depending on the nanowire morphology and dimensions, resulting in either positive or negative frequency shifts. Our results also show that in some cases bolometric and radiation pressure effects can have opposite contributions so that their overall effect is greatly reduced. We conclude that Si nanowire resonators can be engineered for harnessing back-action effects for either optimizing frequency stability or exploiting dynamic phenomena such as parametric amplification.

Nature Nanotechnology, 2010

One-dimensional nanomechanical resonators based on nanowires and nanotubes have emerged as promis... more One-dimensional nanomechanical resonators based on nanowires and nanotubes have emerged as promising candidates for mass sensors 1-6 . When the resonator is clamped at one end and the atoms or molecules being measured land on the other end (which is free to vibrate), the resonance frequency of the device decreases by an amount that is proportional to the mass of the atoms or molecules. However, atoms and molecules can land at any position along the resonator, and many biomolecules have sizes that are comparable to the size of the resonator, so the relationship between the added mass and the frequency shift breaks down 7-10 . Moreover, whereas resonators fabricated by top-down methods tend to vibrate in just one dimension because they are usually shaped like diving boards, perfectly axisymmetric one-dimensional nanoresonators can support flexural vibrations with the same amplitude and frequency in two dimensions 11 . Here, we propose a new approach to mass sensing and stiffness spectroscopy based on the fact that the nanoresonator will enter a superposition state of two orthogonal vibrations with different frequencies when this symmetry is broken. Measuring these frequencies allows the mass, stiffness and azimuthal arrival direction of the adsorbate to be determined.

Nanotechnology, 2013

We report a method to pattern horizontal vapor-liquid-solid growth of Si nanowires at vertical si... more We report a method to pattern horizontal vapor-liquid-solid growth of Si nanowires at vertical sidewalls of Si microstructures. The method allows one to produce either single nanowire structures or well-ordered nanowire arrays with predefined growth positions, thus enabling a practical development of nanomechanical devices that exploit the singular properties of Si nanowires. In particular, we demonstrate the fabrication of doubly clamped nanowire resonators and resonator arrays whose mechanical resonances can be measured by optical or electrical readout. We also show that the fabrication method enables the electrical readout of the resonant mode splitting of nanowire resonators in the VHF range, which allows the application of such an effect for enhanced nanomechanical sensing with nanowire resonators.

Nano Letters, 2012

The optomechanical coupling that emerges in an optical cavity in which one of the mirrors is a me... more The optomechanical coupling that emerges in an optical cavity in which one of the mirrors is a mechanical resonator has allowed sub-Kelvin cooling with the prospect of observing quantum phenomena and self-sustained oscillators with very high spectral purity. Both applications clearly benefit from the use of the smallest possible mechanical resonator. Unfortunately, the optomechanical coupling largely decays when the size of the mechanical system is below the light wavelength. Here, we propose to exploit the optical resonances associated to the light confinement in subwavelength structures to circumvent this limitation, efficiently extending optomechanics to nanoscale objects. We demonstrate this mechanism with suspended silicon nanowires. We are able to optically cool the mechanical vibration of the nanowires from room temperature to 30-40 K or to obtain regenerative mechanical oscillation with a frequency stability of about one part per million. The reported optomechanical phenomena can be exploited for developing cost-optimized mass sensors with sensitivities in the zeptogram range.

Nano Letters, 2009

Coupled nanomechanical systems and their entangled eigenstates offer unique opportunities for the... more Coupled nanomechanical systems and their entangled eigenstates offer unique opportunities for the detection of ultrasmall masses. In this paper we show theoretically and experimentally that the stochastic and deterministic responses of a pair of coupled nanocantilevers provide different and complementary information about the added mass of an analyte and its location. This method allows the sensitive detection of minute quantities of mass even in the presence of large initial differences in the active masses of the two cantilevers. Finally, we show the fundamental limits in mass detection of this sensing paradigm.