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Papers by Gianluigi Zanardo
XXII CONGRESSO NAZIONALE DELLA S.C. I., 2006
Journal of Organometallic Chemistry
Trichlorostannyl complexes [Ru(SnCl 3) (Cp')L] (2a-c) were prepared by treatment of optically act... more Trichlorostannyl complexes [Ru(SnCl 3) (Cp')L] (2a-c) were prepared by treatment of optically active halfsandwich chlorocomplexes [RuCl(Cp')L] (1a-c) with an excess of SnCl 2 .2H 2 O in ethanol. Treatment of trichlorostannyl complexes 2a-c with NaBH 4 afforded trihydridostannyl derivatives [Ru(SnH 3) (Cp')L] (3a-c) in moderated yields. Treatment of 2a-c with MgBrMe gave the trimethylstannyl complexes Ru(SnMe 3) (Cp')L (4a-c). Alkynylstannyl derivatives [Ru{Sn(C≡CPh) 3 }(Cp')L] (5a-c) were prepared by treatment of trichlorostannyl compounds 2a-c with an excess of LiC≡CPh in thf. All the complexes present optical activity. The complexes were characterized spectroscopically and by X-ray crystal structure determination of [RuCl(h 5-C 5 Me 5)L] (1b), [Ru(SnCl 3) (h 5-C 5 Me 5)L] (2b), and [Ru(SnCl 3) (h 5-C 9 H 7)L] (2c). The influence of different ligands on the RueP interaction in several complexes 1a-c, 2a-c and 3a-c was evaluated by DFT calculations. These calculations indicate that [SnCl 3 ]has a stronger stabilization effect than [Cl]and the same occurs between eC 9 H 7 and eC 5 Me 5. These relative stabilities combined with the distortion energies of the fragments produce a stabilizing effect in the RueP bonds of complex 2c that is twice as strong as in the 1b complex.
Organometallics, 2006
ABSTRACT
Organometallics, 2013
ABSTRACT Trichlorostannyl complexes Ru(SnCl3)(η5-C9H7)(PPh3)L (1; L = P(OMe)3, P(OEt)3) were prep... more ABSTRACT Trichlorostannyl complexes Ru(SnCl3)(η5-C9H7)(PPh3)L (1; L = P(OMe)3, P(OEt)3) were prepared by allowing chloro compounds RuCl(η5-C9H7)(PPh3)L to react with SnCl2·2H2O in ethanol. Treatment of compounds 1 with NaBH4 in ethanol yielded the tin trihydride derivatives Ru(SnH3)(η5-C9H7)(PPh3)L (2). The reaction of trichlorostannyl complexes 1 with MgBrMe in diethyl ether afforded the chlorodimethylstannyl derivatives Ru(SnClMe2)(η5-C9H7)(PPh3)L (3), whereas reaction with Li+C≡CPh– in THF yielded the trialkynylstannyl compounds Ru[Sn(C≡CPh)3](η5-C9H7)(PPh3)L (4). Treatment of the trihydridostannyl complexes 2 with the alkyl propiolate HC≡CCOOR led to the trivinylstannyl derivatives Ru[Sn{C(COOR)═CH2}3](η5-C9H7)(PPh3)L (5, 6; R = Me, Et). However, the reaction of [Ru]–SnH3 (2) with the propargylic alcohol HC≡CCPh2OH yielded the alkene H2C═C(H)CPh2OH and the hydride RuH(η5-C9H7)(PPh3)L (7). Treatment of tin trihydride complexes 2 with H2O led to the trihydroxostannyl derivatives Ru[Sn(OH)3](η5-C9H7)(PPh3)L (8). Protonation of [Ru]–SnH3 (2) with triflic acid (HOTf) produced the very unstable dihydridostannyl compound Ru[SnH2(OTf)](η5-C9H7)(PPh3)L (9). Stabilization of SnH2 species was achieved by protonation with HOTf at −30 °C of the cyclopentadienyl compound Ru(SnH3)(η5-C5H5)(PPh3)[P(OMe)3], which yielded the complex Ru[SnH2(OTf)](η5-C5H5)(PPh3)[P(OMe)3] (10a). The complexes were characterized by spectroscopy (IR and 1H, 31P, 13C, and 119Sn NMR data) and by X-ray crystal structure determinations of Ru[Sn(C≡CPh)3](η5-C9H7)(PPh3)[P(OEt)3] (4b) and Ru[Sn(OH)3](η5-C9H7)(PPh3)[P(OEt)3] (8b).
Organometallics, 2008
ABSTRACT Trichlorostannyl complexes M(SnCl3)(Tp)L(PPh3) (1, 2) and M(SnCl3)(Cp)L(PPh3) (5, 6) [M ... more ABSTRACT Trichlorostannyl complexes M(SnCl3)(Tp)L(PPh3) (1, 2) and M(SnCl3)(Cp)L(PPh3) (5, 6) [M = Ru, Os; L = P(OMe)3 (a), P(OEt)3 (b), PPh(OEt)2 (c), PPh3 (d)] were prepared by allowing chloro complexes MCl(Tp)L(PPh3) and MCl(Cp)L(PPh3) to react with an excess of SnCl2·2H2O in ethanol. Treatment of trichlorostannyl complexes 1, 2, 5, and 6 with NaBH4 in ethanol yielded tin trihydride derivatives M(SnH3)(Tp)L(PPh3) (3, 4) and M(SnH3)(Cp)L(PPh3) (7, 8). Reaction of these complexes with CCl4 gave the trichlorostannyl precursors 1, 2, 5, and 6. Hydridochlorostannyl intermediates Os(SnH2Cl)(Tp)[P(OMe)3](PPh3) (9a) and Os(SnHCl2)(Tp)[P(OMe)3](PPh3) (10a) were also obtained. Reaction of trihydridostannyl complexes M(SnH3)(Tp)L(PPh3) (3, 4) with CO2 (1 atm) led to hydridobis(formate) derivatives M[SnH{OC(H)O}2](Tp)L(PPh3) (11). In contrast, reaction of the related complexes M(SnH3)(Cp)L(PPh3) (7, 8) with CO2 (1 atm) led to the binuclear OH-bridging bis(formate) derivatives [M[Sn{OC(H)O}2(μ-OH)](Cp)L(PPh3)]2 (12, 13). A reaction path for the formation of 12 and 13, involving the mononuclear tin hydride complex M[SnH{OC(H)O}2](Cp)L(PPh3), is discussed. The X-ray crystal structure of 12b is reported. Chlorobis(methyl)stannyl Ru(SnClMe2)(Cp)[P(OEt)3](PPh3) (15b) and trimethylstannyl complexes M(SnMe3)(Tp)[P(OMe)3](PPh3) (14a) and M(SnMe3)(Cp)[P(OEt)3](PPh3) (16b, 17b) were prepared by allowing trichlorostannyl compounds 1, 2, 5, and 6 to react with MgBrMe in diethyl ether. Trialkynylstannyl derivatives M[Sn(CCR)3}(Tp)L(PPh3) (18, 19) and Ru[Sn(CCR)3}(Cp)[P(OEt)3](PPh3) (20b) (R = Ph, p-tolyl) were also prepared from the reaction of trichlorostannyl complexes 1, 2, 5, and 6 with Li+(CCR)− in thf. The complexes were characterized by spectroscopy and by X-ray crystal structure determination of Ru(SnClMe2)(Cp)[P(OEt)3](PPh3) (15b).
Materials and Structures, 2001
ABSTRACT The technical aspects and the notable outcomes of an experiment on a reduced scale build... more ABSTRACT The technical aspects and the notable outcomes of an experiment on a reduced scale building, aimed to determine the seismic performances of an advanced reinforced masonry construction technique, are presented. The testing program includes 33 shaking table tests (characterised by a design PGA varying from 0.02 g up to 0.6 g), alternated with sequences of low intensity dynamic characterisations, based on shock tests. The damage evolution is analysed by modelling the structure as a non-linear SDOF oscillator, where the input is the ground motion and the output is the top floor response. The analysis results high-light a very satisfactory seismic behaviour of the tested construction technique, in terms of the response to low-medium intensity earthquakes, and the performance at the ultimate limit state (ductility and reduction factor equal to 7.5 and 3.6, respectively). These outcomes are discussed with reference to the current Eurocode provisions. Des essais sur table vibrante ont été effectués afin d'observer la réponse sismique d'un bâtiment en briques, à échelle réduite, renforcé selon une nouvelle méthode. Le programme d'essais inclut 33 séismes, caractérisés par une valeur maximale d'accélération au sol variant entre 0,02 g et 0,6 g, alternés avec des séquences de caractérisations dynamiques à basse intensité. L'évolution des dommages a été analysée en modélisant la structure comme un oscillateur non linéaire à un degré de liberté, sollicité à la base par le mouvement au sol. La réponse de l'oscillateur correspond à celle du bâtiment mesurée au sommet. Les résultats analytiques mettent en évidence le comportement sismique satisfaisant des bâtiments renforcés selon la technique r.m., tant pour des séismes à basse-moyenne intensité que pour des séismes où les états limites sont atteints (ductilité de 7,5 et facteur de comportement équivalant à 3,6). Les résultats sont comparés aux recommandations de L'Eurocode.
Journal of Organometallic Chemistry, 2005
ABSTRACT
Journal of Organometallic Chemistry, 2007
Mixed-ligand OsCl(Tp)L(PPh 3 ) complexes 1 [Tp = hydridotris(pyrazolyl)borate; L = P(OMe) 3 , P(O... more Mixed-ligand OsCl(Tp)L(PPh 3 ) complexes 1 [Tp = hydridotris(pyrazolyl)borate; L = P(OMe) 3 , P(OEt) 3 and PPh(OEt) 2 ] were prepared by allowing OsCl(Tp)(PPh 3 ) 2 to react with an excess of phosphite. Treatment of chlorocomplexes 1 with NaBH 4 in ethanol afforded hydride OsH(Tp)L(PPh 3 ) derivatives 2. Stable dihydrogen [Os(g 2 -H 2 )(Tp)L(PPh 3 )]BPh 4 derivatives 3 were prepared by protonation of hydrides 2 with HBF 4 AE Et 2 O at À80°C. The presence of the g 2 -H 2 ligand is supported by short T 1 min values and J HD measurements on the partially deuterated derivatives. Treatment of the hydride OsH(Tp)[P(OEt) 3 ](PPh 3 ) complex with the aryldiazonium salt [4-CH 3 C 6 H 4 N 2 ]BF 4 afforded aryldiazene [Os(4-CH 3 C 6 H 4 N@NH)(Tp){P(OEt) 3 }(PPh 3 )]BPh 4 derivative 4. Instead, aryldiazenido [Os(4-CH 3 C 6 H 4 N 2 )(Tp)[P(OEt) 3 ](PPh 3 )](BF 4 ) 2 derivative 5 was obtained by reacting the hydride OsH(Tp)[P(OEt) 3 ](PPh 3 ) first with methyltriflate and then with aryldiazonium [4-CH 3 C 6 H 4 N 2 ]BF 4 salt. Spectroscopic characterisation (IR, 15 N NMR) by the 15 N-labelled derivative strongly supports the presence of a near-linear Os-N"N-Ar aryldiazenido group. Imine [Os{g 1 -NH@C(H)Ar}(Tp)-{P(OEt) 3 }(PPh 3 )]BPh 4 complexes 6 and 7 (Ar = C 6 H 5 , 4-CH 3 C 6 H 4 ) were also prepared by allowing the hydride OsH(Tp)[P(OEt) 3 ](PPh 3 ) to react first with methyltriflate and then with alkylazides.
Inorganica Chimica Acta, 2010
Mixed-ligand complexes [ReBr (CO) 2 (CNR) nL3− n](14)[R= 4-CH3OC6H4, 4-CH3C6H4, C (CH3) 3; L= P ... more Mixed-ligand complexes [ReBr (CO) 2 (CNR) nL3− n](14)[R= 4-CH3OC6H4, 4-CH3C6H4, C (CH3) 3; L= P (OEt) 3, PPh (OEt) 2; n= 1, 2] were prepared by allowing carbonyl compounds [ReBr (CO) 4L] and [ReBr (CO) 3L2] to react with an excess of isocyanide. ...
European Journal of Inorganic Chemistry, 2008
Vinyl complexes [Ru{η 2 -C(=CH 2 )CPh(R)OH(Ru-O)}P 4 ]BPh 4 (1) [P = P(OEt) 3 ; R = Ph, Me] were ... more Vinyl complexes [Ru{η 2 -C(=CH 2 )CPh(R)OH(Ru-O)}P 4 ]BPh 4 (1) [P = P(OEt) 3 ; R = Ph, Me] were prepared by allowing the RuH 2 P 4 hydride to react first with HBF 4 ·Et 2 O and then with propargylic alcohol HCϵCCPh(R)OH at low temperature. The complexes were characterised spectroscopically (IR, NMR) and by X-ray crystal structure determination of the [Ru{η 2 -C(=CH 2 )CPh 2 OH(Ru-O)}{P(OEt) 3 } 4 ]BPh 4 (1a) derivative. Related osmium complexes [Os{η 2 -C(=CH 2 )CPh(R)-OH(Os-O)}P 4 ]BPh 4 (2) and [Os{η 2 -CH=C(H)CPh(R)OH(Os-O)}P 4 ]BPh 4 (3) [P = P(OEt) 3 ; R = Ph, Me] were obtained by treating the OsH 2 P 4 hydride first with methyl triflate Eur.
Dalton Transactions, 2007
Azide complexes [M(RN(3))(CO)(3)P(2)]BPh(4)[M = Mn, Re; R = C(6)H(5)CH(2), 4-CH(3)C(6)H(4)CH(2), ... more Azide complexes [M(RN(3))(CO)(3)P(2)]BPh(4)[M = Mn, Re; R = C(6)H(5)CH(2), 4-CH(3)C(6)H(4)CH(2), C(6)H(5), 4-CH(3)C(6)H(4), C(5)H(9); P = PPh(OEt)(2), PPh(2)(OEt)] were prepared by allowing tricarbonyl MH(CO)(3)P(2) hydride complexes to react first with Brønsted acid (HBF(4), CF(3)SO(3)H) and then with organic azide in the dark. In sunlight the reaction yielded tetraazabutadiene [M(eta(2)-1,4-R(2)N(4))(CO)(2)P(2)]BPh(4) complexes or, with benzyl azide, imine [M{eta(1)-NH[double bond, length as m-dash]C(H)Ar}(CO)(3)P(2)]BPh(4)(Ar = C(6)H(5), 4-CH(3)C(6)H(4)) derivatives. Tetraazabutadiene [M(eta(2)-1,4-R(2)N(4))(CO)(2)P(2)]BPh(4) complexes were also prepared by reacting dicarbonyl MH(CO)(2)P(3) species first with Brønsted acid and then with an excess of organic azide. Complexes were characterised spectroscopically (IR, (1)H, (31)P, (13)C, (15)N NMR data) and by the X-ray crystal structure determination of complex [Re{eta(2)-1,4-(C(6)H(5)CH(2))(2)N(4)}(CO)(2){PPh(OEt)(2)}(2)]BPh(4)(). Strong evidence for coordination of the organic azide was obtained from the (15)N NMR spectra of labelled [M(C(6)H(5)CH(2)(15)NN(15)N)(CO)(3)P(2)]BPh(4) derivatives.
XXII CONGRESSO NAZIONALE DELLA S.C. I., 2006
Journal of Organometallic Chemistry
Trichlorostannyl complexes [Ru(SnCl 3) (Cp')L] (2a-c) were prepared by treatment of optically act... more Trichlorostannyl complexes [Ru(SnCl 3) (Cp')L] (2a-c) were prepared by treatment of optically active halfsandwich chlorocomplexes [RuCl(Cp')L] (1a-c) with an excess of SnCl 2 .2H 2 O in ethanol. Treatment of trichlorostannyl complexes 2a-c with NaBH 4 afforded trihydridostannyl derivatives [Ru(SnH 3) (Cp')L] (3a-c) in moderated yields. Treatment of 2a-c with MgBrMe gave the trimethylstannyl complexes Ru(SnMe 3) (Cp')L (4a-c). Alkynylstannyl derivatives [Ru{Sn(C≡CPh) 3 }(Cp')L] (5a-c) were prepared by treatment of trichlorostannyl compounds 2a-c with an excess of LiC≡CPh in thf. All the complexes present optical activity. The complexes were characterized spectroscopically and by X-ray crystal structure determination of [RuCl(h 5-C 5 Me 5)L] (1b), [Ru(SnCl 3) (h 5-C 5 Me 5)L] (2b), and [Ru(SnCl 3) (h 5-C 9 H 7)L] (2c). The influence of different ligands on the RueP interaction in several complexes 1a-c, 2a-c and 3a-c was evaluated by DFT calculations. These calculations indicate that [SnCl 3 ]has a stronger stabilization effect than [Cl]and the same occurs between eC 9 H 7 and eC 5 Me 5. These relative stabilities combined with the distortion energies of the fragments produce a stabilizing effect in the RueP bonds of complex 2c that is twice as strong as in the 1b complex.
Organometallics, 2006
ABSTRACT
Organometallics, 2013
ABSTRACT Trichlorostannyl complexes Ru(SnCl3)(η5-C9H7)(PPh3)L (1; L = P(OMe)3, P(OEt)3) were prep... more ABSTRACT Trichlorostannyl complexes Ru(SnCl3)(η5-C9H7)(PPh3)L (1; L = P(OMe)3, P(OEt)3) were prepared by allowing chloro compounds RuCl(η5-C9H7)(PPh3)L to react with SnCl2·2H2O in ethanol. Treatment of compounds 1 with NaBH4 in ethanol yielded the tin trihydride derivatives Ru(SnH3)(η5-C9H7)(PPh3)L (2). The reaction of trichlorostannyl complexes 1 with MgBrMe in diethyl ether afforded the chlorodimethylstannyl derivatives Ru(SnClMe2)(η5-C9H7)(PPh3)L (3), whereas reaction with Li+C≡CPh– in THF yielded the trialkynylstannyl compounds Ru[Sn(C≡CPh)3](η5-C9H7)(PPh3)L (4). Treatment of the trihydridostannyl complexes 2 with the alkyl propiolate HC≡CCOOR led to the trivinylstannyl derivatives Ru[Sn{C(COOR)═CH2}3](η5-C9H7)(PPh3)L (5, 6; R = Me, Et). However, the reaction of [Ru]–SnH3 (2) with the propargylic alcohol HC≡CCPh2OH yielded the alkene H2C═C(H)CPh2OH and the hydride RuH(η5-C9H7)(PPh3)L (7). Treatment of tin trihydride complexes 2 with H2O led to the trihydroxostannyl derivatives Ru[Sn(OH)3](η5-C9H7)(PPh3)L (8). Protonation of [Ru]–SnH3 (2) with triflic acid (HOTf) produced the very unstable dihydridostannyl compound Ru[SnH2(OTf)](η5-C9H7)(PPh3)L (9). Stabilization of SnH2 species was achieved by protonation with HOTf at −30 °C of the cyclopentadienyl compound Ru(SnH3)(η5-C5H5)(PPh3)[P(OMe)3], which yielded the complex Ru[SnH2(OTf)](η5-C5H5)(PPh3)[P(OMe)3] (10a). The complexes were characterized by spectroscopy (IR and 1H, 31P, 13C, and 119Sn NMR data) and by X-ray crystal structure determinations of Ru[Sn(C≡CPh)3](η5-C9H7)(PPh3)[P(OEt)3] (4b) and Ru[Sn(OH)3](η5-C9H7)(PPh3)[P(OEt)3] (8b).
Organometallics, 2008
ABSTRACT Trichlorostannyl complexes M(SnCl3)(Tp)L(PPh3) (1, 2) and M(SnCl3)(Cp)L(PPh3) (5, 6) [M ... more ABSTRACT Trichlorostannyl complexes M(SnCl3)(Tp)L(PPh3) (1, 2) and M(SnCl3)(Cp)L(PPh3) (5, 6) [M = Ru, Os; L = P(OMe)3 (a), P(OEt)3 (b), PPh(OEt)2 (c), PPh3 (d)] were prepared by allowing chloro complexes MCl(Tp)L(PPh3) and MCl(Cp)L(PPh3) to react with an excess of SnCl2·2H2O in ethanol. Treatment of trichlorostannyl complexes 1, 2, 5, and 6 with NaBH4 in ethanol yielded tin trihydride derivatives M(SnH3)(Tp)L(PPh3) (3, 4) and M(SnH3)(Cp)L(PPh3) (7, 8). Reaction of these complexes with CCl4 gave the trichlorostannyl precursors 1, 2, 5, and 6. Hydridochlorostannyl intermediates Os(SnH2Cl)(Tp)[P(OMe)3](PPh3) (9a) and Os(SnHCl2)(Tp)[P(OMe)3](PPh3) (10a) were also obtained. Reaction of trihydridostannyl complexes M(SnH3)(Tp)L(PPh3) (3, 4) with CO2 (1 atm) led to hydridobis(formate) derivatives M[SnH{OC(H)O}2](Tp)L(PPh3) (11). In contrast, reaction of the related complexes M(SnH3)(Cp)L(PPh3) (7, 8) with CO2 (1 atm) led to the binuclear OH-bridging bis(formate) derivatives [M[Sn{OC(H)O}2(μ-OH)](Cp)L(PPh3)]2 (12, 13). A reaction path for the formation of 12 and 13, involving the mononuclear tin hydride complex M[SnH{OC(H)O}2](Cp)L(PPh3), is discussed. The X-ray crystal structure of 12b is reported. Chlorobis(methyl)stannyl Ru(SnClMe2)(Cp)[P(OEt)3](PPh3) (15b) and trimethylstannyl complexes M(SnMe3)(Tp)[P(OMe)3](PPh3) (14a) and M(SnMe3)(Cp)[P(OEt)3](PPh3) (16b, 17b) were prepared by allowing trichlorostannyl compounds 1, 2, 5, and 6 to react with MgBrMe in diethyl ether. Trialkynylstannyl derivatives M[Sn(CCR)3}(Tp)L(PPh3) (18, 19) and Ru[Sn(CCR)3}(Cp)[P(OEt)3](PPh3) (20b) (R = Ph, p-tolyl) were also prepared from the reaction of trichlorostannyl complexes 1, 2, 5, and 6 with Li+(CCR)− in thf. The complexes were characterized by spectroscopy and by X-ray crystal structure determination of Ru(SnClMe2)(Cp)[P(OEt)3](PPh3) (15b).
Materials and Structures, 2001
ABSTRACT The technical aspects and the notable outcomes of an experiment on a reduced scale build... more ABSTRACT The technical aspects and the notable outcomes of an experiment on a reduced scale building, aimed to determine the seismic performances of an advanced reinforced masonry construction technique, are presented. The testing program includes 33 shaking table tests (characterised by a design PGA varying from 0.02 g up to 0.6 g), alternated with sequences of low intensity dynamic characterisations, based on shock tests. The damage evolution is analysed by modelling the structure as a non-linear SDOF oscillator, where the input is the ground motion and the output is the top floor response. The analysis results high-light a very satisfactory seismic behaviour of the tested construction technique, in terms of the response to low-medium intensity earthquakes, and the performance at the ultimate limit state (ductility and reduction factor equal to 7.5 and 3.6, respectively). These outcomes are discussed with reference to the current Eurocode provisions. Des essais sur table vibrante ont été effectués afin d'observer la réponse sismique d'un bâtiment en briques, à échelle réduite, renforcé selon une nouvelle méthode. Le programme d'essais inclut 33 séismes, caractérisés par une valeur maximale d'accélération au sol variant entre 0,02 g et 0,6 g, alternés avec des séquences de caractérisations dynamiques à basse intensité. L'évolution des dommages a été analysée en modélisant la structure comme un oscillateur non linéaire à un degré de liberté, sollicité à la base par le mouvement au sol. La réponse de l'oscillateur correspond à celle du bâtiment mesurée au sommet. Les résultats analytiques mettent en évidence le comportement sismique satisfaisant des bâtiments renforcés selon la technique r.m., tant pour des séismes à basse-moyenne intensité que pour des séismes où les états limites sont atteints (ductilité de 7,5 et facteur de comportement équivalant à 3,6). Les résultats sont comparés aux recommandations de L'Eurocode.
Journal of Organometallic Chemistry, 2005
ABSTRACT
Journal of Organometallic Chemistry, 2007
Mixed-ligand OsCl(Tp)L(PPh 3 ) complexes 1 [Tp = hydridotris(pyrazolyl)borate; L = P(OMe) 3 , P(O... more Mixed-ligand OsCl(Tp)L(PPh 3 ) complexes 1 [Tp = hydridotris(pyrazolyl)borate; L = P(OMe) 3 , P(OEt) 3 and PPh(OEt) 2 ] were prepared by allowing OsCl(Tp)(PPh 3 ) 2 to react with an excess of phosphite. Treatment of chlorocomplexes 1 with NaBH 4 in ethanol afforded hydride OsH(Tp)L(PPh 3 ) derivatives 2. Stable dihydrogen [Os(g 2 -H 2 )(Tp)L(PPh 3 )]BPh 4 derivatives 3 were prepared by protonation of hydrides 2 with HBF 4 AE Et 2 O at À80°C. The presence of the g 2 -H 2 ligand is supported by short T 1 min values and J HD measurements on the partially deuterated derivatives. Treatment of the hydride OsH(Tp)[P(OEt) 3 ](PPh 3 ) complex with the aryldiazonium salt [4-CH 3 C 6 H 4 N 2 ]BF 4 afforded aryldiazene [Os(4-CH 3 C 6 H 4 N@NH)(Tp){P(OEt) 3 }(PPh 3 )]BPh 4 derivative 4. Instead, aryldiazenido [Os(4-CH 3 C 6 H 4 N 2 )(Tp)[P(OEt) 3 ](PPh 3 )](BF 4 ) 2 derivative 5 was obtained by reacting the hydride OsH(Tp)[P(OEt) 3 ](PPh 3 ) first with methyltriflate and then with aryldiazonium [4-CH 3 C 6 H 4 N 2 ]BF 4 salt. Spectroscopic characterisation (IR, 15 N NMR) by the 15 N-labelled derivative strongly supports the presence of a near-linear Os-N"N-Ar aryldiazenido group. Imine [Os{g 1 -NH@C(H)Ar}(Tp)-{P(OEt) 3 }(PPh 3 )]BPh 4 complexes 6 and 7 (Ar = C 6 H 5 , 4-CH 3 C 6 H 4 ) were also prepared by allowing the hydride OsH(Tp)[P(OEt) 3 ](PPh 3 ) to react first with methyltriflate and then with alkylazides.
Inorganica Chimica Acta, 2010
Mixed-ligand complexes [ReBr (CO) 2 (CNR) nL3− n](14)[R= 4-CH3OC6H4, 4-CH3C6H4, C (CH3) 3; L= P ... more Mixed-ligand complexes [ReBr (CO) 2 (CNR) nL3− n](14)[R= 4-CH3OC6H4, 4-CH3C6H4, C (CH3) 3; L= P (OEt) 3, PPh (OEt) 2; n= 1, 2] were prepared by allowing carbonyl compounds [ReBr (CO) 4L] and [ReBr (CO) 3L2] to react with an excess of isocyanide. ...
European Journal of Inorganic Chemistry, 2008
Vinyl complexes [Ru{η 2 -C(=CH 2 )CPh(R)OH(Ru-O)}P 4 ]BPh 4 (1) [P = P(OEt) 3 ; R = Ph, Me] were ... more Vinyl complexes [Ru{η 2 -C(=CH 2 )CPh(R)OH(Ru-O)}P 4 ]BPh 4 (1) [P = P(OEt) 3 ; R = Ph, Me] were prepared by allowing the RuH 2 P 4 hydride to react first with HBF 4 ·Et 2 O and then with propargylic alcohol HCϵCCPh(R)OH at low temperature. The complexes were characterised spectroscopically (IR, NMR) and by X-ray crystal structure determination of the [Ru{η 2 -C(=CH 2 )CPh 2 OH(Ru-O)}{P(OEt) 3 } 4 ]BPh 4 (1a) derivative. Related osmium complexes [Os{η 2 -C(=CH 2 )CPh(R)-OH(Os-O)}P 4 ]BPh 4 (2) and [Os{η 2 -CH=C(H)CPh(R)OH(Os-O)}P 4 ]BPh 4 (3) [P = P(OEt) 3 ; R = Ph, Me] were obtained by treating the OsH 2 P 4 hydride first with methyl triflate Eur.
Dalton Transactions, 2007
Azide complexes [M(RN(3))(CO)(3)P(2)]BPh(4)[M = Mn, Re; R = C(6)H(5)CH(2), 4-CH(3)C(6)H(4)CH(2), ... more Azide complexes [M(RN(3))(CO)(3)P(2)]BPh(4)[M = Mn, Re; R = C(6)H(5)CH(2), 4-CH(3)C(6)H(4)CH(2), C(6)H(5), 4-CH(3)C(6)H(4), C(5)H(9); P = PPh(OEt)(2), PPh(2)(OEt)] were prepared by allowing tricarbonyl MH(CO)(3)P(2) hydride complexes to react first with Brønsted acid (HBF(4), CF(3)SO(3)H) and then with organic azide in the dark. In sunlight the reaction yielded tetraazabutadiene [M(eta(2)-1,4-R(2)N(4))(CO)(2)P(2)]BPh(4) complexes or, with benzyl azide, imine [M{eta(1)-NH[double bond, length as m-dash]C(H)Ar}(CO)(3)P(2)]BPh(4)(Ar = C(6)H(5), 4-CH(3)C(6)H(4)) derivatives. Tetraazabutadiene [M(eta(2)-1,4-R(2)N(4))(CO)(2)P(2)]BPh(4) complexes were also prepared by reacting dicarbonyl MH(CO)(2)P(3) species first with Brønsted acid and then with an excess of organic azide. Complexes were characterised spectroscopically (IR, (1)H, (31)P, (13)C, (15)N NMR data) and by the X-ray crystal structure determination of complex [Re{eta(2)-1,4-(C(6)H(5)CH(2))(2)N(4)}(CO)(2){PPh(OEt)(2)}(2)]BPh(4)(). Strong evidence for coordination of the organic azide was obtained from the (15)N NMR spectra of labelled [M(C(6)H(5)CH(2)(15)NN(15)N)(CO)(3)P(2)]BPh(4) derivatives.