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Papers by Michael Man

Research paper thumbnail of Imaging electron motion in 2D semiconductor heterojunctions

Conference on Lasers and Electro-Optics, 2017

Transfer of electrons through semiconductor heterojunctions is the key process in all electronics... more Transfer of electrons through semiconductor heterojunctions is the key process in all electronics. Here we make movies of electron dynamics in InSe/GaAs through time and spectrally-resolved photoemission electron microscopy, bringing insights to this fundamental process.

Research paper thumbnail of Dynamics of momentum-resolved excitons in a 2D semiconductor using TR-µARPES

Bulletin of the American Physical Society, 2021

Research paper thumbnail of Step Permeability on the Pt(111) Surface

Bulletin of the American Physical Society, 2005

Research paper thumbnail of Investigation of local nanoscale electronic variation and photo excited carrier dynamics in hybrid organic-inorganic mixed cation perovskite films

Research paper thumbnail of Nanoscale Heterogeneities Limit Optoelectronic Performance in Halide Perovskites

Proceedings of the International Conference on Perovskite Thin Film Photovoltaics and Perovskite Photonics and Optoelectronics, 2019

Research paper thumbnail of Enhanced terahertz emission from a femtosecond-laser-ablated photoconductor

Bulletin of the American Physical Society, Mar 6, 2015

hertz (THz) emission properties from bow-tie antennas fabricated on a femtosecondlaser-ablated, s... more hertz (THz) emission properties from bow-tie antennas fabricated on a femtosecondlaser-ablated, semi-insulating gallium arsenide (SI-GaAs) photoconductor are investigated. The ablated material demonstrates increased photoabsorption resulting in increased photocurrent leading to a more efficient optical to THz efficiency. We use THz time-domain spectroscopy (THz-TDS) in order to compare the relative efficiency of the two fabricated devices. The influence of the excitation power and applied bias on the antennas electrodes for both ablated and non-ablated substrates is studied, highlighting the better performances of the ablated devices. A 60% enhancement in THz emission amplitude is observed in the frequency range 0.5-4 THz of the ablated SI-GaAs antenna, compared to untreated SI-GaAs. Our experimental results are in agreement with Drude-Lorentz numerical simulations using previously reported absorption and photocurrent properties of femtosecond laser ablated SI-GaAs based photoconductors. This material treatment provides a new way to achieve THz-TDS systems based on SI-GaAs antennas with an improved signal-to-noise ratio.

Research paper thumbnail of Observing the interplay between surface and bulk optical nonlinearities in thin van der Waals crystals

Research paper thumbnail of Protecting the properties of monolayer MoS2 on silicon based substrates with an atomically thin buffer

Research paper thumbnail of Chemical Vapor Deposition Synthesized Atomically Thin Molybdenum Disulfide with Optoelectronic-Grade Crystalline Quality

ACS nano, Jan 13, 2015

The ability to synthesize high-quality samples over large areas and at low cost is one of the big... more The ability to synthesize high-quality samples over large areas and at low cost is one of the biggest challenges during the developmental stage of any novel material. While chemical vapor deposition (CVD) methods provide a promising low-cost route for CMOS compatible, large-scale growth of materials, it often falls short of the high-quality demands in nanoelectronics and optoelectronics. We present large-scale CVD synthesis of single- and few-layered MoS2 using direct vapor-phase sulfurization of MoO2, which enables us to obtain extremely high-quality single-crystal monolayer MoS2 samples with field-effect mobility exceeding 30 cm(2)/(V s) in monolayers. These samples can be readily synthesized on a variety of substrates, and demonstrate a high-degree of optoelectronic uniformity in Raman and photoluminescence mapping over entire crystals with areas exceeding hundreds of square micrometers. Because of their high crystalline quality, Raman spectroscopy on these samples reveal a range...

Research paper thumbnail of Control of Nanoscale Surface Defects and the Relation to Local Structural Properties in Halide Perovskite Films

Proceedings of the International Conference on Perovskite Thin Film Photovoltaics and Perovskite Photonics and Optoelectronics, 2019

Research paper thumbnail of Imaging electron motion in 2D semiconductor heterojunctions

Conference on Lasers and Electro-Optics, 2017

Transfer of electrons through semiconductor heterojunctions is the key process in all electronics... more Transfer of electrons through semiconductor heterojunctions is the key process in all electronics. Here we make movies of electron dynamics in InSe/GaAs through time and spectrally-resolved photoemission electron microscopy, bringing insights to this fundamental process.

Research paper thumbnail of Dynamics of momentum-resolved excitons in a 2D semiconductor using TR-µARPES

Bulletin of the American Physical Society, 2021

Research paper thumbnail of Step Permeability on the Pt(111) Surface

Bulletin of the American Physical Society, 2005

Research paper thumbnail of Investigation of local nanoscale electronic variation and photo excited carrier dynamics in hybrid organic-inorganic mixed cation perovskite films

Research paper thumbnail of Nanoscale Heterogeneities Limit Optoelectronic Performance in Halide Perovskites

Proceedings of the International Conference on Perovskite Thin Film Photovoltaics and Perovskite Photonics and Optoelectronics, 2019

Research paper thumbnail of Enhanced terahertz emission from a femtosecond-laser-ablated photoconductor

Bulletin of the American Physical Society, Mar 6, 2015

hertz (THz) emission properties from bow-tie antennas fabricated on a femtosecondlaser-ablated, s... more hertz (THz) emission properties from bow-tie antennas fabricated on a femtosecondlaser-ablated, semi-insulating gallium arsenide (SI-GaAs) photoconductor are investigated. The ablated material demonstrates increased photoabsorption resulting in increased photocurrent leading to a more efficient optical to THz efficiency. We use THz time-domain spectroscopy (THz-TDS) in order to compare the relative efficiency of the two fabricated devices. The influence of the excitation power and applied bias on the antennas electrodes for both ablated and non-ablated substrates is studied, highlighting the better performances of the ablated devices. A 60% enhancement in THz emission amplitude is observed in the frequency range 0.5-4 THz of the ablated SI-GaAs antenna, compared to untreated SI-GaAs. Our experimental results are in agreement with Drude-Lorentz numerical simulations using previously reported absorption and photocurrent properties of femtosecond laser ablated SI-GaAs based photoconductors. This material treatment provides a new way to achieve THz-TDS systems based on SI-GaAs antennas with an improved signal-to-noise ratio.

Research paper thumbnail of Observing the interplay between surface and bulk optical nonlinearities in thin van der Waals crystals

Research paper thumbnail of Protecting the properties of monolayer MoS2 on silicon based substrates with an atomically thin buffer

Research paper thumbnail of Chemical Vapor Deposition Synthesized Atomically Thin Molybdenum Disulfide with Optoelectronic-Grade Crystalline Quality

ACS nano, Jan 13, 2015

The ability to synthesize high-quality samples over large areas and at low cost is one of the big... more The ability to synthesize high-quality samples over large areas and at low cost is one of the biggest challenges during the developmental stage of any novel material. While chemical vapor deposition (CVD) methods provide a promising low-cost route for CMOS compatible, large-scale growth of materials, it often falls short of the high-quality demands in nanoelectronics and optoelectronics. We present large-scale CVD synthesis of single- and few-layered MoS2 using direct vapor-phase sulfurization of MoO2, which enables us to obtain extremely high-quality single-crystal monolayer MoS2 samples with field-effect mobility exceeding 30 cm(2)/(V s) in monolayers. These samples can be readily synthesized on a variety of substrates, and demonstrate a high-degree of optoelectronic uniformity in Raman and photoluminescence mapping over entire crystals with areas exceeding hundreds of square micrometers. Because of their high crystalline quality, Raman spectroscopy on these samples reveal a range...

Research paper thumbnail of Control of Nanoscale Surface Defects and the Relation to Local Structural Properties in Halide Perovskite Films

Proceedings of the International Conference on Perovskite Thin Film Photovoltaics and Perovskite Photonics and Optoelectronics, 2019

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