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Papers by Soma Chakrabarti
Journal of Pharmaceutical Sciences, Apr 1, 1997
The dissolution rate of a solid drug from the gastrointestinal (GI) tract is affected by the prop... more The dissolution rate of a solid drug from the gastrointestinal (GI) tract is affected by the properties and flow dynamics of the liquid medium surrounding the tablet, as well as by the chemical nature of the drug. In this study, naproxen was used as a poorly soluble model drug. The dissolution medium was buffered with acetate, citrate, or phosphate buffer of varied concentrations and pH. GI flow conditions around a stationary tablet were simulated in a laminar flow device by anchoring the tablet on the floor of its channel having a rectangular cross section. Fresh, buffered solution was passed across the tablet and the effluent was collected for analysis and calculation of the dissolution rate. The dissolution rate was found to vary nonlinearly with the exposed tablet height, reaching a maximum at a tablet height approximately half the channel height. This maximum rate was attributed to an optimal combination of (1) eddy mixing and local turbulence generated by the flow impingement on the bluff object (tablet) and (2) the exposed tablet surface area available for dissolution. This effect was further confirmed by using dye-enhanced visual analysis of flow patterns at varied flow rates and exposed tablet heights. Elevation of the tablet to approximately the channel half-height significantly magnified the dissolution rate increase observed on exposure to buffered medium. Thus, tablet height and exposed surface area are major factors in determining dissolution rate, especially in conditions where the dissolving species reacts with the solvent. These results suggest that standard in vitro dissolution rate methods do not qualitatively indicate incremental changes in rate with altered tablet geometry or dissolution medium.
Journal of Pharmaceutical Sciences, Mar 1, 1996
The dissolution rate of a solid drug from the gastrointestinal (GI) tract is affected by the prop... more The dissolution rate of a solid drug from the gastrointestinal (GI) tract is affected by the properties and flow dynamics of the liquid medium surrounding the tablet, as well as by the chemical nature of the drug. In this study, naproxen was used as a poorly soluble model drug. The dissolution medium was buffered with acetate, citrate, or phosphate buffer of varied concentrations and pH. GI flow conditions around a stationary tablet were simulated in a laminar flow device by anchoring the tablet on the floor of its channel having a rectangular cross section. Fresh, buffered solution was passed across the tablet and the effluent was collected for analysis and calculation of the dissolution rate. The dissolution rate was found to vary nonlinearly with the exposed tablet height, reaching a maximum at a tablet height approximately half the channel height. This maximum rate was attributed to an optimal combination of (1) eddy mixing and local turbulence generated by the flow impingement on the bluff object (tablet) and (2) the exposed tablet surface area available for dissolution. This effect was further confirmed by using dye-enhanced visual analysis of flow patterns at varied flow rates and exposed tablet heights. Elevation of the tablet to approximately the channel half-height significantly magnified the dissolution rate increase observed on exposure to buffered medium. Thus, tablet height and exposed surface area are major factors in determining dissolution rate, especially in conditions where the dissolving species reacts with the solvent. These results suggest that standard in vitro dissolution rate methods do not qualitatively indicate incremental changes in rate with altered tablet geometry or dissolution medium.
2021 World Engineering Education Forum/Global Engineering Deans Council (WEEF/GEDC)
Journal of Peptide Research, 1999
eucen Studies eJournal of University Lifelong Learning
2012 ASEE Annual Conference & Exposition Proceedings
2014 ASEE Annual Conference & Exposition Proceedings
2013 ASEE Annual Conference & Exposition Proceedings
2013 ASEE Annual Conference & Exposition Proceedings
Proceedings of the 12th World Conference on Continuing Engineering Education, 2010
International Journal of Peptide and Protein Research, 1994
RGD peptides are known as important ligands for integrin receptors in the cell adhesion process. ... more RGD peptides are known as important ligands for integrin receptors in the cell adhesion process. The selectivity of RGD peptides for a certain integrin receptor is partly dependent on the RGD conformation and the residues surrounding the RGD sequence. This paper investigates the effect of the addition of a phenylalanine residue on the RGD conformation in cyclo(1,6)Ac-Cys-Arg-Gly-Asp-Phe-Pen-NH2 (1) as compared to the previously studied cyclo(1,5)Ac-Pen-Arg-Gly-Asp-Cys-NH2 (2). The conformational study of peptide 1 was done in aqueous solution using nuclear magnetic resonance (NMR) spectroscopy and molecular dynamics simulations. This work will increase the understanding of the flanking residue's effect in RGD peptides.
Journal of Pharmaceutical Sciences, 1997
The dissolution rate of a solid drug from the gastrointestinal (GI) tract is affected by the prop... more The dissolution rate of a solid drug from the gastrointestinal (GI) tract is affected by the properties and flow dynamics of the liquid medium surrounding the tablet, as well as by the chemical nature of the drug. In this study, naproxen was used as a poorly soluble model drug. The dissolution medium was buffered with acetate, citrate, or phosphate buffer of varied concentrations and pH. GI flow conditions around a stationary tablet were simulated in a laminar flow device by anchoring the tablet on the floor of its channel having a rectangular cross section. Fresh, buffered solution was passed across the tablet and the effluent was collected for analysis and calculation of the dissolution rate. The dissolution rate was found to vary nonlinearly with the exposed tablet height, reaching a maximum at a tablet height approximately half the channel height. This maximum rate was attributed to an optimal combination of (1) eddy mixing and local turbulence generated by the flow impingement on the bluff object (tablet) and (2) the exposed tablet surface area available for dissolution. This effect was further confirmed by using dye-enhanced visual analysis of flow patterns at varied flow rates and exposed tablet heights. Elevation of the tablet to approximately the channel half-height significantly magnified the dissolution rate increase observed on exposure to buffered medium. Thus, tablet height and exposed surface area are major factors in determining dissolution rate, especially in conditions where the dissolving species reacts with the solvent. These results suggest that standard in vitro dissolution rate methods do not qualitatively indicate incremental changes in rate with altered tablet geometry or dissolution medium.
Journal of Biomolecular Structure and Dynamics, 1996
The Journal of Peptide Research, 2009
A 10 amino acid residue cyclic peptide, cyclo(2,9)-Ac-Glnl-Cys2-Arg3-Ser4-Val5-Glu6-Gly7-Ser8-Cys... more A 10 amino acid residue cyclic peptide, cyclo(2,9)-Ac-Glnl-Cys2-Arg3-Ser4-Val5-Glu6-Gly7-Ser8-Cys9-Glyl0, from the C-terminal region of human growth hormone (hGH) was synthesized and studied by 2D proton NMR and molecular dynamics (MD) simulations. The solubility of the peptide was low in water; hence, NMR studies were done in two solvent mixtures, water and deuterated dimethyl sulfoxide. NOE-constrained molecular dynamics and MD simulations resulted in major and minor conformers in solution. The major conformer has a type I p-turn at Glnl-Cys2-Arg3-Ser4 and a loop structure around Glu6-Gly7-Ser8. Comparison of the conformation of this peptide with the peptide fragment 181-190 in the intact hGH protein X-ray crystal structure indicated that the synthetic peptide retains some structural similarity to the intact protein. Since the C-terminal region is important in binding the hCH protein to its receptor, the conformation of the synthetic peptide could be useful in understanding the binding mechanism. 0 Munksgaard 1997.
Biochemical and Biophysical Research Communications, 1992
Cyclo(l,S)-Ac-Pen-Arg-Gly-Asp-Cys-NH2 (3) is a potent inhibitor of platelet aggregation. Nuclear ... more Cyclo(l,S)-Ac-Pen-Arg-Gly-Asp-Cys-NH2 (3) is a potent inhibitor of platelet aggregation. Nuclear magnetic resonance (NMR) and restrained molecular dynamics were used to study the conformations of 3. Elucidation of RGD conformations in 3 will increase the understanding of interaction between the RGD-sequence with GPIIb/IIIa.
The Journal of …, 1997
A 10 amino acid residue cyclic peptide, cyclo(2,9)-Ac-Glnl-Cys2-Arg3-Ser4-Val5-Glu6-Gly7-Ser8-Cys... more A 10 amino acid residue cyclic peptide, cyclo(2,9)-Ac-Glnl-Cys2-Arg3-Ser4-Val5-Glu6-Gly7-Ser8-Cys9-Glyl0, from the C-terminal region of human growth hormone (hGH) was synthesized and studied by 2D proton NMR and molecular dynamics (MD) simulations. The solubility of the peptide was low in water; hence, NMR studies were done in two solvent mixtures, water and deuterated dimethyl sulfoxide. NOE-constrained molecular dynamics and MD simulations resulted in major and minor conformers in solution. The major conformer has a type I p-turn at Glnl-Cys2-Arg3-Ser4 and a loop structure around Glu6-Gly7-Ser8. Comparison of the conformation of this peptide with the peptide fragment 181-190 in the intact hGH protein X-ray crystal structure indicated that the synthetic peptide retains some structural similarity to the intact protein. Since the C-terminal region is important in binding the hCH protein to its receptor, the conformation of the synthetic peptide could be useful in understanding the binding mechanism. 0 Munksgaard 1997.
… Journal of Peptide …, 1994
RGD peptides are known as important ligands for integrin receptors in the cell adhesion process. ... more RGD peptides are known as important ligands for integrin receptors in the cell adhesion process. The selectivity of RGD peptides for a certain integrin receptor is partly dependent on the RGD conformation and the residues surrounding the RGD sequence. This paper investigates the effect of the addition of a phenylalanine residue on the RGD conformation in cyclo(1,6)Ac-Cys-Arg-Gly-Asp-Phe-Pen-NH2 (1) as compared to the previously studied cyclo(1,5)Ac-Pen-Arg-Gly-Asp-Cys-NH2 (2). The conformational study of peptide 1 was done in aqueous solution using nuclear magnetic resonance (NMR) spectroscopy and molecular dynamics simulations. This work will increase the understanding of the flanking residue's effect in RGD peptides.
Journal of pharmaceutical …, 1997
The dissolution rate of a solid drug from the gastrointestinal (GI) tract is affected by the prop... more The dissolution rate of a solid drug from the gastrointestinal (GI) tract is affected by the properties and flow dynamics of the liquid medium surrounding the tablet, as well as by the chemical nature of the drug. In this study, naproxen was used as a poorly soluble model drug. The dissolution medium was buffered with acetate, citrate, or phosphate buffer of varied concentrations and pH. GI flow conditions around a stationary tablet were simulated in a laminar flow device by anchoring the tablet on the floor of its channel having a rectangular cross section. Fresh, buffered solution was passed across the tablet and the effluent was collected for analysis and calculation of the dissolution rate. The dissolution rate was found to vary nonlinearly with the exposed tablet height, reaching a maximum at a tablet height approximately half the channel height. This maximum rate was attributed to an optimal combination of (1) eddy mixing and local turbulence generated by the flow impingement on the bluff object (tablet) and (2) the exposed tablet surface area available for dissolution. This effect was further confirmed by using dye-enhanced visual analysis of flow patterns at varied flow rates and exposed tablet heights. Elevation of the tablet to approximately the channel half-height significantly magnified the dissolution rate increase observed on exposure to buffered medium. Thus, tablet height and exposed surface area are major factors in determining dissolution rate, especially in conditions where the dissolving species reacts with the solvent. These results suggest that standard in vitro dissolution rate methods do not qualitatively indicate incremental changes in rate with altered tablet geometry or dissolution medium.
Journal of Pharmaceutical Sciences, Apr 1, 1997
The dissolution rate of a solid drug from the gastrointestinal (GI) tract is affected by the prop... more The dissolution rate of a solid drug from the gastrointestinal (GI) tract is affected by the properties and flow dynamics of the liquid medium surrounding the tablet, as well as by the chemical nature of the drug. In this study, naproxen was used as a poorly soluble model drug. The dissolution medium was buffered with acetate, citrate, or phosphate buffer of varied concentrations and pH. GI flow conditions around a stationary tablet were simulated in a laminar flow device by anchoring the tablet on the floor of its channel having a rectangular cross section. Fresh, buffered solution was passed across the tablet and the effluent was collected for analysis and calculation of the dissolution rate. The dissolution rate was found to vary nonlinearly with the exposed tablet height, reaching a maximum at a tablet height approximately half the channel height. This maximum rate was attributed to an optimal combination of (1) eddy mixing and local turbulence generated by the flow impingement on the bluff object (tablet) and (2) the exposed tablet surface area available for dissolution. This effect was further confirmed by using dye-enhanced visual analysis of flow patterns at varied flow rates and exposed tablet heights. Elevation of the tablet to approximately the channel half-height significantly magnified the dissolution rate increase observed on exposure to buffered medium. Thus, tablet height and exposed surface area are major factors in determining dissolution rate, especially in conditions where the dissolving species reacts with the solvent. These results suggest that standard in vitro dissolution rate methods do not qualitatively indicate incremental changes in rate with altered tablet geometry or dissolution medium.
Journal of Pharmaceutical Sciences, Mar 1, 1996
The dissolution rate of a solid drug from the gastrointestinal (GI) tract is affected by the prop... more The dissolution rate of a solid drug from the gastrointestinal (GI) tract is affected by the properties and flow dynamics of the liquid medium surrounding the tablet, as well as by the chemical nature of the drug. In this study, naproxen was used as a poorly soluble model drug. The dissolution medium was buffered with acetate, citrate, or phosphate buffer of varied concentrations and pH. GI flow conditions around a stationary tablet were simulated in a laminar flow device by anchoring the tablet on the floor of its channel having a rectangular cross section. Fresh, buffered solution was passed across the tablet and the effluent was collected for analysis and calculation of the dissolution rate. The dissolution rate was found to vary nonlinearly with the exposed tablet height, reaching a maximum at a tablet height approximately half the channel height. This maximum rate was attributed to an optimal combination of (1) eddy mixing and local turbulence generated by the flow impingement on the bluff object (tablet) and (2) the exposed tablet surface area available for dissolution. This effect was further confirmed by using dye-enhanced visual analysis of flow patterns at varied flow rates and exposed tablet heights. Elevation of the tablet to approximately the channel half-height significantly magnified the dissolution rate increase observed on exposure to buffered medium. Thus, tablet height and exposed surface area are major factors in determining dissolution rate, especially in conditions where the dissolving species reacts with the solvent. These results suggest that standard in vitro dissolution rate methods do not qualitatively indicate incremental changes in rate with altered tablet geometry or dissolution medium.
2021 World Engineering Education Forum/Global Engineering Deans Council (WEEF/GEDC)
Journal of Peptide Research, 1999
eucen Studies eJournal of University Lifelong Learning
2012 ASEE Annual Conference & Exposition Proceedings
2014 ASEE Annual Conference & Exposition Proceedings
2013 ASEE Annual Conference & Exposition Proceedings
2013 ASEE Annual Conference & Exposition Proceedings
Proceedings of the 12th World Conference on Continuing Engineering Education, 2010
International Journal of Peptide and Protein Research, 1994
RGD peptides are known as important ligands for integrin receptors in the cell adhesion process. ... more RGD peptides are known as important ligands for integrin receptors in the cell adhesion process. The selectivity of RGD peptides for a certain integrin receptor is partly dependent on the RGD conformation and the residues surrounding the RGD sequence. This paper investigates the effect of the addition of a phenylalanine residue on the RGD conformation in cyclo(1,6)Ac-Cys-Arg-Gly-Asp-Phe-Pen-NH2 (1) as compared to the previously studied cyclo(1,5)Ac-Pen-Arg-Gly-Asp-Cys-NH2 (2). The conformational study of peptide 1 was done in aqueous solution using nuclear magnetic resonance (NMR) spectroscopy and molecular dynamics simulations. This work will increase the understanding of the flanking residue's effect in RGD peptides.
Journal of Pharmaceutical Sciences, 1997
The dissolution rate of a solid drug from the gastrointestinal (GI) tract is affected by the prop... more The dissolution rate of a solid drug from the gastrointestinal (GI) tract is affected by the properties and flow dynamics of the liquid medium surrounding the tablet, as well as by the chemical nature of the drug. In this study, naproxen was used as a poorly soluble model drug. The dissolution medium was buffered with acetate, citrate, or phosphate buffer of varied concentrations and pH. GI flow conditions around a stationary tablet were simulated in a laminar flow device by anchoring the tablet on the floor of its channel having a rectangular cross section. Fresh, buffered solution was passed across the tablet and the effluent was collected for analysis and calculation of the dissolution rate. The dissolution rate was found to vary nonlinearly with the exposed tablet height, reaching a maximum at a tablet height approximately half the channel height. This maximum rate was attributed to an optimal combination of (1) eddy mixing and local turbulence generated by the flow impingement on the bluff object (tablet) and (2) the exposed tablet surface area available for dissolution. This effect was further confirmed by using dye-enhanced visual analysis of flow patterns at varied flow rates and exposed tablet heights. Elevation of the tablet to approximately the channel half-height significantly magnified the dissolution rate increase observed on exposure to buffered medium. Thus, tablet height and exposed surface area are major factors in determining dissolution rate, especially in conditions where the dissolving species reacts with the solvent. These results suggest that standard in vitro dissolution rate methods do not qualitatively indicate incremental changes in rate with altered tablet geometry or dissolution medium.
Journal of Biomolecular Structure and Dynamics, 1996
The Journal of Peptide Research, 2009
A 10 amino acid residue cyclic peptide, cyclo(2,9)-Ac-Glnl-Cys2-Arg3-Ser4-Val5-Glu6-Gly7-Ser8-Cys... more A 10 amino acid residue cyclic peptide, cyclo(2,9)-Ac-Glnl-Cys2-Arg3-Ser4-Val5-Glu6-Gly7-Ser8-Cys9-Glyl0, from the C-terminal region of human growth hormone (hGH) was synthesized and studied by 2D proton NMR and molecular dynamics (MD) simulations. The solubility of the peptide was low in water; hence, NMR studies were done in two solvent mixtures, water and deuterated dimethyl sulfoxide. NOE-constrained molecular dynamics and MD simulations resulted in major and minor conformers in solution. The major conformer has a type I p-turn at Glnl-Cys2-Arg3-Ser4 and a loop structure around Glu6-Gly7-Ser8. Comparison of the conformation of this peptide with the peptide fragment 181-190 in the intact hGH protein X-ray crystal structure indicated that the synthetic peptide retains some structural similarity to the intact protein. Since the C-terminal region is important in binding the hCH protein to its receptor, the conformation of the synthetic peptide could be useful in understanding the binding mechanism. 0 Munksgaard 1997.
Biochemical and Biophysical Research Communications, 1992
Cyclo(l,S)-Ac-Pen-Arg-Gly-Asp-Cys-NH2 (3) is a potent inhibitor of platelet aggregation. Nuclear ... more Cyclo(l,S)-Ac-Pen-Arg-Gly-Asp-Cys-NH2 (3) is a potent inhibitor of platelet aggregation. Nuclear magnetic resonance (NMR) and restrained molecular dynamics were used to study the conformations of 3. Elucidation of RGD conformations in 3 will increase the understanding of interaction between the RGD-sequence with GPIIb/IIIa.
The Journal of …, 1997
A 10 amino acid residue cyclic peptide, cyclo(2,9)-Ac-Glnl-Cys2-Arg3-Ser4-Val5-Glu6-Gly7-Ser8-Cys... more A 10 amino acid residue cyclic peptide, cyclo(2,9)-Ac-Glnl-Cys2-Arg3-Ser4-Val5-Glu6-Gly7-Ser8-Cys9-Glyl0, from the C-terminal region of human growth hormone (hGH) was synthesized and studied by 2D proton NMR and molecular dynamics (MD) simulations. The solubility of the peptide was low in water; hence, NMR studies were done in two solvent mixtures, water and deuterated dimethyl sulfoxide. NOE-constrained molecular dynamics and MD simulations resulted in major and minor conformers in solution. The major conformer has a type I p-turn at Glnl-Cys2-Arg3-Ser4 and a loop structure around Glu6-Gly7-Ser8. Comparison of the conformation of this peptide with the peptide fragment 181-190 in the intact hGH protein X-ray crystal structure indicated that the synthetic peptide retains some structural similarity to the intact protein. Since the C-terminal region is important in binding the hCH protein to its receptor, the conformation of the synthetic peptide could be useful in understanding the binding mechanism. 0 Munksgaard 1997.
… Journal of Peptide …, 1994
RGD peptides are known as important ligands for integrin receptors in the cell adhesion process. ... more RGD peptides are known as important ligands for integrin receptors in the cell adhesion process. The selectivity of RGD peptides for a certain integrin receptor is partly dependent on the RGD conformation and the residues surrounding the RGD sequence. This paper investigates the effect of the addition of a phenylalanine residue on the RGD conformation in cyclo(1,6)Ac-Cys-Arg-Gly-Asp-Phe-Pen-NH2 (1) as compared to the previously studied cyclo(1,5)Ac-Pen-Arg-Gly-Asp-Cys-NH2 (2). The conformational study of peptide 1 was done in aqueous solution using nuclear magnetic resonance (NMR) spectroscopy and molecular dynamics simulations. This work will increase the understanding of the flanking residue's effect in RGD peptides.
Journal of pharmaceutical …, 1997
The dissolution rate of a solid drug from the gastrointestinal (GI) tract is affected by the prop... more The dissolution rate of a solid drug from the gastrointestinal (GI) tract is affected by the properties and flow dynamics of the liquid medium surrounding the tablet, as well as by the chemical nature of the drug. In this study, naproxen was used as a poorly soluble model drug. The dissolution medium was buffered with acetate, citrate, or phosphate buffer of varied concentrations and pH. GI flow conditions around a stationary tablet were simulated in a laminar flow device by anchoring the tablet on the floor of its channel having a rectangular cross section. Fresh, buffered solution was passed across the tablet and the effluent was collected for analysis and calculation of the dissolution rate. The dissolution rate was found to vary nonlinearly with the exposed tablet height, reaching a maximum at a tablet height approximately half the channel height. This maximum rate was attributed to an optimal combination of (1) eddy mixing and local turbulence generated by the flow impingement on the bluff object (tablet) and (2) the exposed tablet surface area available for dissolution. This effect was further confirmed by using dye-enhanced visual analysis of flow patterns at varied flow rates and exposed tablet heights. Elevation of the tablet to approximately the channel half-height significantly magnified the dissolution rate increase observed on exposure to buffered medium. Thus, tablet height and exposed surface area are major factors in determining dissolution rate, especially in conditions where the dissolving species reacts with the solvent. These results suggest that standard in vitro dissolution rate methods do not qualitatively indicate incremental changes in rate with altered tablet geometry or dissolution medium.