Eileen Harkin-Jones | University of Ulster (original) (raw)
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Papers by Eileen Harkin-Jones
Polymer Engineering and Science, 1996
Rotational molding is used primarily for the manufacture of products from powdered plastics. Howe... more Rotational molding is used primarily for the manufacture of products from powdered plastics. However, there are many advantages to be gained from the use of a liquid plastic feedstock. This paper describes the results of an investigation to study the effect of process variables, such as mold temperature, on the morphology and mechanical properties of parts manufactured by the rotational molding of a reactive liquid nylon, caprolactam plus a diol. Initial mold temperature has a significant effect on the degree of crystallinity, levels drop off sharply at mold temperatures in excess of 140°C, while spherulite size increases after this point. Flexural properties improve with increasing degree of crystallinity while impact strength decreases. A similar trend is observed in moldings containing fillers. A brief study of water uptake and dimensional stability of molded parts is also described.
Composites Science and Technology, 2011
Polymer International, 2009
BACKGROUND: Poly(ethylene terephthalate) (PET) is widely used in the packaging industry. In order... more BACKGROUND: Poly(ethylene terephthalate) (PET) is widely used in the packaging industry. In order to enhance the mechanical and barrier properties, nanoscale fillers are added to PET matrices to form nanocomposites. In the work reported here, a melt-processed PET/synthetic mica nanocomposite sheet was characterised to determine the effect of the incorporation of synthetic mica on the sheet properties and also to see if these properties are an indicator of subsequent performance under high-speed, high-temperature biaxial deformation, typical of processes such as stretch blow moulding.RESULTS: The incorporation of synthetic mica was found to enhance the modulus, particularly above the glass transition temperature, and barrier properties of the extruded sheet and it significantly altered the deformation behaviour of PET under biaxial deformation. The plastic flow of PET during biaxial deformation was found to diminish for the nanocomposites, and strain hardening occurred earlier.CONCLUSION: The modulus and barrier properties of PET were enhanced by the incorporation of synthetic mica. Clay loading also altered the biaxial deformation behaviour of PET. Copyright © 2009 Society of Chemical Industry
Composites Science and Technology, 2009
Macromolecules, 2009
Solid-state NMR and TEM were used to quantitatively examine the evolution of clay morphology upon... more Solid-state NMR and TEM were used to quantitatively examine the evolution of clay morphology upon equibiaxial stretching of polypropylene/montmorillonite (PP−MMT) nanocomposites up to a stretch ratio (λ = final length/initial length) of 3.5. 1 H spin−lattice relaxation times ...
Materials Letters, 2010
This paper presents a novel method to describe the microstructure of polymer/clay nanocomposites ... more This paper presents a novel method to describe the microstructure of polymer/clay nanocomposites quantitatively. Based on the image analyses of transmission electron microscopy (TEM) and optical microscopy micrographs, two parameters, degree of dispersion (χ) and mean ...
Composites Science and Technology, 2010
Polymer Engineering and Science, 1996
Rotational molding is used primarily for the manufacture of products from powdered plastics. Howe... more Rotational molding is used primarily for the manufacture of products from powdered plastics. However, there are many advantages to be gained from the use of a liquid plastic feedstock. This paper describes the results of an investigation to study the effect of process variables, such as mold temperature, on the morphology and mechanical properties of parts manufactured by the rotational molding of a reactive liquid nylon, caprolactam plus a diol. Initial mold temperature has a significant effect on the degree of crystallinity, levels drop off sharply at mold temperatures in excess of 140°C, while spherulite size increases after this point. Flexural properties improve with increasing degree of crystallinity while impact strength decreases. A similar trend is observed in moldings containing fillers. A brief study of water uptake and dimensional stability of molded parts is also described.
Composites Science and Technology, 2011
Polymer International, 2009
BACKGROUND: Poly(ethylene terephthalate) (PET) is widely used in the packaging industry. In order... more BACKGROUND: Poly(ethylene terephthalate) (PET) is widely used in the packaging industry. In order to enhance the mechanical and barrier properties, nanoscale fillers are added to PET matrices to form nanocomposites. In the work reported here, a melt-processed PET/synthetic mica nanocomposite sheet was characterised to determine the effect of the incorporation of synthetic mica on the sheet properties and also to see if these properties are an indicator of subsequent performance under high-speed, high-temperature biaxial deformation, typical of processes such as stretch blow moulding.RESULTS: The incorporation of synthetic mica was found to enhance the modulus, particularly above the glass transition temperature, and barrier properties of the extruded sheet and it significantly altered the deformation behaviour of PET under biaxial deformation. The plastic flow of PET during biaxial deformation was found to diminish for the nanocomposites, and strain hardening occurred earlier.CONCLUSION: The modulus and barrier properties of PET were enhanced by the incorporation of synthetic mica. Clay loading also altered the biaxial deformation behaviour of PET. Copyright © 2009 Society of Chemical Industry
Composites Science and Technology, 2009
Macromolecules, 2009
Solid-state NMR and TEM were used to quantitatively examine the evolution of clay morphology upon... more Solid-state NMR and TEM were used to quantitatively examine the evolution of clay morphology upon equibiaxial stretching of polypropylene/montmorillonite (PP−MMT) nanocomposites up to a stretch ratio (λ = final length/initial length) of 3.5. 1 H spin−lattice relaxation times ...
Materials Letters, 2010
This paper presents a novel method to describe the microstructure of polymer/clay nanocomposites ... more This paper presents a novel method to describe the microstructure of polymer/clay nanocomposites quantitatively. Based on the image analyses of transmission electron microscopy (TEM) and optical microscopy micrographs, two parameters, degree of dispersion (χ) and mean ...
Composites Science and Technology, 2010