Mosadegh Keshavarz | University of Perugia (original) (raw)

Mosadegh Keshavarz

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Papers by Mosadegh Keshavarz

Research paper thumbnail of Three-component One-pot Synthetic Route to Functionalized N -Phenyl- and N , N -(1,4-phenylene)-2-alkylimino-2,3-dihydrothiazoles under Mild, Solvent- and Catalyst-free Conditions

Journal of the Chinese Chemical Society, 2014

ABSTRACT A simple and efficient one-pot synthesis of Alkyl-2-(alkylimino)-4-methyl-3-phenyl-2,3-d... more ABSTRACT A simple and efficient one-pot synthesis of Alkyl-2-(alkylimino)-4-methyl-3-phenyl-2,3-dihydrothiazole-5-carboxylate and Dialkyl 3,3'-(1,4-phenylene)-bis-[2-(alkylimino)-4-methyl-2,3-dihydrothiazole-5-carboxylate] derivatives from the reaction of phenylisothiocyanate (and also 1,4-phenylene diisothiocyanate) and primary alkylamines in the presence of 2-chloro-1,3-dicarbonyl compounds is described. This new protocol has several advantages such as lack of necessity of the catalyst and solvent, good yields,mild conditions and short times for reaction.

Research paper thumbnail of Imidazol-1-yl-acetic acid as a novel green bifunctional organocatalyst for the synthesis of 1,8-dioxooctahydroxanthenes under solvent-free conditions

Chinese Chemical Letters, 2014

Research paper thumbnail of 中国化学快报 2014, 25 (02) 317-320 Doi: Issn: 1001-8417 CN: 11-2710/O6

Research paper thumbnail of Melamine trisulfonic acid: an efficient and recyclable solid acid catalyst for the green synthesis of Biscoumarin derivatives

A novel catalytic synthesis of 3,3'-(arylmethylene)-bis-(4-hydroxy-2H-chromene-2-one) derivatives... more A novel catalytic synthesis of 3,3'-(arylmethylene)-bis-(4-hydroxy-2H-chromene-2-one) derivatives from a tandem
condensation reaction of 4-hydroxycoumarin and aromatic aldehydes has been developed. The reaction occurs in water in the
presence of Melamine trisulfonic acid as catalyst to give the corresponding products in good to high yields. This green
approach has several advantages such as short reaction times, clean reaction profiles, and simple experimental and workup
procedures. Moreover, the catalyst can be easily recovered by filtration and used at least seven times with only slight reduction
in its catalytic activity. The results of the presented protocol in comparison with the different available catalysts in
condensation reaction of benzaldehyde with 4-Hydroxycoumarin show that MTSA presented better results due to the structure
of MTSA.

Research paper thumbnail of Three-component One-pot Synthetic Route to Functionalized N -Phenyl- and N , N -(1,4-phenylene)-2-alkylimino-2,3-dihydrothiazoles under Mild, Solvent- and Catalyst-free Conditions

Journal of the Chinese Chemical Society, 2014

ABSTRACT A simple and efficient one-pot synthesis of Alkyl-2-(alkylimino)-4-methyl-3-phenyl-2,3-d... more ABSTRACT A simple and efficient one-pot synthesis of Alkyl-2-(alkylimino)-4-methyl-3-phenyl-2,3-dihydrothiazole-5-carboxylate and Dialkyl 3,3'-(1,4-phenylene)-bis-[2-(alkylimino)-4-methyl-2,3-dihydrothiazole-5-carboxylate] derivatives from the reaction of phenylisothiocyanate (and also 1,4-phenylene diisothiocyanate) and primary alkylamines in the presence of 2-chloro-1,3-dicarbonyl compounds is described. This new protocol has several advantages such as lack of necessity of the catalyst and solvent, good yields,mild conditions and short times for reaction.

Research paper thumbnail of Imidazol-1-yl-acetic acid as a novel green bifunctional organocatalyst for the synthesis of 1,8-dioxooctahydroxanthenes under solvent-free conditions

Chinese Chemical Letters, 2014

Research paper thumbnail of 中国化学快报 2014, 25 (02) 317-320 Doi: Issn: 1001-8417 CN: 11-2710/O6

Research paper thumbnail of Melamine trisulfonic acid: an efficient and recyclable solid acid catalyst for the green synthesis of Biscoumarin derivatives

A novel catalytic synthesis of 3,3'-(arylmethylene)-bis-(4-hydroxy-2H-chromene-2-one) derivatives... more A novel catalytic synthesis of 3,3'-(arylmethylene)-bis-(4-hydroxy-2H-chromene-2-one) derivatives from a tandem
condensation reaction of 4-hydroxycoumarin and aromatic aldehydes has been developed. The reaction occurs in water in the
presence of Melamine trisulfonic acid as catalyst to give the corresponding products in good to high yields. This green
approach has several advantages such as short reaction times, clean reaction profiles, and simple experimental and workup
procedures. Moreover, the catalyst can be easily recovered by filtration and used at least seven times with only slight reduction
in its catalytic activity. The results of the presented protocol in comparison with the different available catalysts in
condensation reaction of benzaldehyde with 4-Hydroxycoumarin show that MTSA presented better results due to the structure
of MTSA.

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