Somesh Chandra Ganguli | Aalto University, School of Science (original) (raw)

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Papers by Somesh Chandra Ganguli

Heavy fermion systems represent one of the paradigmatic strongly correlated states of matter. The... more Heavy fermion systems represent one of the paradigmatic strongly correlated states of matter. They have been used as a platform for investigating exotic behavior ranging from quantum criticality and non-Fermi liquid behavior to unconventional topological superconductivity. Heavy fermions arise from the exchange interaction between localized magnetic moments and conduction electrons that leads to the well-known Kondo effect. In a Kondo lattice, the interaction between the localized moments gives rise to a band with heavy effective mass. This intriguing phenomenology has so far only been realized in compounds containing rare-earth elements with 4f or 5f electrons. Here, we realize a designer van der Waals heterostructure where artificial heavy fermions emerge from the Kondo coupling between a lattice of localized magnetic moments and itinerant electrons in a 1T/1H-TaS_2 heterostructure. We study the heterostructure using scanning tunneling microscopy (STM) and spectroscopy (STS) and s...

We report the construction and performance of a low temperature, high field scanning tunneling mi... more We report the construction and performance of a low temperature, high field scanning tunneling microscope (STM) operating down to 350mK and in magnetic fields up to 9T, with thin film deposition and in-situ cleaving capabilities. The main focus lies on the simple design of STM head allowing top loading of the sample and innovative sample holder design that allows us to get spectroscopic data on superconducting thin films grown in-situ on insulating substrates. Other design details on sample transport, chamber and vibration isolation scheme are also described. We demonstrate the capability of our instrument through the atomic resolution imaging and spectroscopy on NbSe2 single crystal and spectroscopic maps obtained on homogeneously disordered NbN thin film.

The notion of spontaneous formation of an inhomogeneous superconducting state is at the heart of ... more The notion of spontaneous formation of an inhomogeneous superconducting state is at the heart of most theories attempting to understand the superconducting state in the presence of strong disorder. Using scanning tunneling spectroscopy and high resolution scanning transmission electron microscopy, we experimentally demonstrate that under the competing effects of strong homogeneous disorder and superconducting correlations, the superconducting state of a conventional superconductor, NbN, spontaneously segregates into domains. Tracking these domains as a function of temperature we observe that the superconducting domains persist across the bulk superconducting transition, Tc, and disappear close to the pseudogap temperature, T*, where signatures of superconducting correlations disappear from the tunneling spectrum and the superfluid response of the system.

The vortex lattice in a Type II superconductor provides a versatile model system to investigate t... more The vortex lattice in a Type II superconductor provides a versatile model system to investigate the order-disorder transition in a periodic medium in the presence of random pinning. Here, using scanning tunnelling spectroscopy in a weakly pinned Co0.0075NbSe2 single crystal, we show that at low temperatures, the vortex lattice in a 3-dimensional superconductor disorders in two steps across the peak effect. At the onset of the peak effect, the equilibrium Bragg glass transforms into an orientational glass through the proliferation of dislocations. At a higher field, the dislocations dissociate into isolated disclination giving rise to an amorphous vortex glass. We also show the existence of a variety of additional non-equilibrium metastable states, which can be accessed through different thermomagnetic cycling.

Disorder induced melting, where the increase in positional entropy created by random pinning site... more Disorder induced melting, where the increase in positional entropy created by random pinning sites drives the order-disorder transition in a periodic solid, provides an alternate route to the more conventional thermal melting. Here, using real space imaging of the vortex lattice through scanning tunneling spectroscopy, we show that in the presence of weak pinning, the vortex lattice in a type II superconductor disorders through two distinct topological transitions. Across each transition, we separately identify metastable states formed through superheating of the low temperature state or supercooling of the high temperature state. Comparing crystals with different levels of pinning we conclude that the two-step melting is fundamentally associated with the presence of random pinning which generates topological defects in the ordered vortex lattice.

Transition metal dichalcogenides (TMDC) are a rich family of two-dimensional materials displaying... more Transition metal dichalcogenides (TMDC) are a rich family of two-dimensional materials displaying a multitude of different quantum ground states. In particular, d^3 TMDCs are paradigmatic materials hosting a variety of symmetry broken states, including charge density waves, superconductivity, and magnetism. Among this family, NbSe_2 is one of the best-studied superconducting materials down to the monolayer limit. Despite its superconducting nature, a variety of results point towards strong electronic repulsions in NbSe_2. Here, we control the strength of the interactions experimentally via quantum confinement effects and use low-temperature scanning tunneling microscopy (STM) and spectroscopy (STS) to demonstrate that NbSe_2 is in strong proximity to a correlated insulating state. This reveals the coexistence of competing interactions in NbSe_2, creating a transition from a superconducting to an insulating quantum correlated state by confinement-controlled interactions. Our results ...

We report directional point contact Andreev reflection (PCAR) measurements on high-quality single... more We report directional point contact Andreev reflection (PCAR) measurements on high-quality single crystals of the non-centrosymmetric superconductor, BiPd. The PCAR spectra measured on different crystallographic faces of the single crystal clearly show the presence of multiple superconducting energy gaps. For point contacts with low resistance, in addition to the superconducting gap feature, a pronounced zero bias conductance peak is observed. These observations provide strong evidence of the presence of unconventional order parameter in this material.

Bulletin of the American Physical Society, 2018

Scientific Reports, 2013

We measure the frequency dependence of the complex ac conductivity of NbN films with different le... more We measure the frequency dependence of the complex ac conductivity of NbN films with different levels of disorder in frequency range 0.4-20 GHz. Films with low disorder exhibit a narrow dynamic fluctuation regime above T c as expected for a conventional superconductor. However, for strongly disordered samples, the fluctuation regime extends well above T c , with a strongly frequency-dependent superfluid stiffness which disappears only at a temperature * m T close to the pseudogap temperature obtained from scanning tunneling measurements. Such a finite-frequency response is associated to a marked slowing down of the superconducting fluctuations already below * m T. The corresponding large length-scale fluctuations suggest a scenario of thermal phase fluctuations between superconducting domains in a strongly disordered s-wave superconductor.

We report experimental evidence of strong orientational coupling between the crystal lattice and ... more We report experimental evidence of strong orientational coupling between the crystal lattice and the vortex lattice in a weakly pinned Co-doped NbSe2 single crystal through direct imaging using low temperature scanning tunneling microscopy/spectroscopy. At low fields, when the magnetic field is applied along the six-fold symmetric c-axis of the NbSe2 crystal, the equilibrium configuration of the vortex lattice is preferentially aligned along the basis vectors of the crystal lattice. The orientational coupling between the vortex lattice and crystal lattice becomes more pronounced as the magnetic field is increased. We show that this coupling enhances the stability of the orientational order of the vortex lattice, which persists even in the disordered state at high fields where dislocations and disclinations have destroyed the topological order.

arXiv: Mesoscale and Nanoscale Physics, 2020

Transition metal dichalcogenides (TMDC) are a rich family of two-dimensional materials displaying... more Transition metal dichalcogenides (TMDC) are a rich family of two-dimensional materials displaying a multitude of different quantum ground states. In particular, d$^3$ TMDCs are paradigmatic materials hosting a variety of symmetry broken states, including charge density waves, superconductivity, and magnetism. Among this family, NbSe$_2$ is one of the best-studied superconducting materials down to the monolayer limit. Despite its superconducting nature, a variety of results point towards strong electronic repulsions in NbSe$_2$. Here, we control the strength of the interactions experimentally via quantum confinement effects and use low-temperature scanning tunneling microscopy (STM) and spectroscopy (STS) to demonstrate that NbSe$_2$ is in strong proximity to a correlated insulating state. This reveals the coexistence of competing interactions in NbSe$_2$, creating a transition from a superconducting to an insulating quantum correlated state by confinement-controlled interactions. Ou...

Heavy fermion systems represent one of the paradigmatic strongly correlated states of matter. The... more Heavy fermion systems represent one of the paradigmatic strongly correlated states of matter. They have been used as a platform for investigating exotic behavior ranging from quantum criticality and non-Fermi liquid behavior to unconventional topological superconductivity. Heavy fermions arise from the exchange interaction between localized magnetic moments and conduction electrons that leads to the well-known Kondo effect. In a Kondo lattice, the interaction between the localized moments gives rise to a band with heavy effective mass. This intriguing phenomenology has so far only been realized in compounds containing rare-earth elements with 4f or 5f electrons. Here, we realize a designer van der Waals heterostructure where artificial heavy fermions emerge from the Kondo coupling between a lattice of localized magnetic moments and itinerant electrons in a 1T/1H-TaS2 heterostructure. We study the heterostructure using scanning tunneling microscopy (STM) and spectroscopy (STS) and sh...

arXiv: Superconductivity, 2015

We report experimental evidence of strong orientational coupling between the crystal lattice and ... more We report experimental evidence of strong orientational coupling between the crystal lattice and the vortex lattice in a weakly pinned Co-doped NbSe2 single crystal through direct imaging using low temperature scanning tunneling microscopy/spectroscopy. At low fields, when the magnetic field is applied along the six-fold symmetric c-axis of the NbSe2 crystal, the equilibrium configuration of the vortex lattice is preferentially aligned along the basis vectors of the crystal lattice. The orientational coupling between the vortex lattice and crystal lattice becomes more pronounced as the magnetic field is increased. We show that this coupling enhances the stability of the orientational order of the vortex lattice, which persists even in the disordered state at high fields where dislocations and disclinations have destroyed the topological order.

The breakdown of crystalline order in a disordered background connects to some of the most challe... more The breakdown of crystalline order in a disordered background connects to some of the most challenging problems in condensed matter physics. For a superconducting vortex lattice, the equilibrium state in the presence of impurities is predicted to be a "Bragg glass" (BG), where the local crystalline order is maintained everywhere and yet the global positional order decays algebraically. Here, using scanning tunnelling spectroscopy (STS) we image the vortex lattice in a weakly pinned NbSe2 single crystal. We present direct evidence that the ordered state of the VL is a BG, consisting of a large number of degenerate metastable states, which is a hallmark of a glassy state. These results are a significant step towards understanding the disordering of a lattice under the influence of quenched random disorder with a direct impact on various fields, including charge density waves, colloidal crystals and self-organised periodic structures on a substrate.

ABSTRACT Using low temperature scanning tunnelling spectroscopy down to 350 mK we study variety o... more ABSTRACT Using low temperature scanning tunnelling spectroscopy down to 350 mK we study variety of vortex lattice states that emerge in a weakly pinned NbSe2 single crystal. Using small magnetic field pulses, and temperature cycling protocols in magnetic field we access various vortex lattice configurations characterised by different degree of order: Quasi long range ordered states characterised by the absence of topological defects and vortex glass states characterised by the proliferation of dislocations. We explicitly show that the quasi long range ordered state comprises of several metastable states with different "local" configuration of the vortex lattice, consistent with predictions of a Bragg glass.

Bulletin of the American Physical Society, 2019

Heavy fermion systems represent one of the paradigmatic strongly correlated states of matter. The... more Heavy fermion systems represent one of the paradigmatic strongly correlated states of matter. They have been used as a platform for investigating exotic behavior ranging from quantum criticality and non-Fermi liquid behavior to unconventional topological superconductivity. Heavy fermions arise from the exchange interaction between localized magnetic moments and conduction electrons that leads to the well-known Kondo effect. In a Kondo lattice, the interaction between the localized moments gives rise to a band with heavy effective mass. This intriguing phenomenology has so far only been realized in compounds containing rare-earth elements with 4f or 5f electrons. Here, we realize a designer van der Waals heterostructure where artificial heavy fermions emerge from the Kondo coupling between a lattice of localized magnetic moments and itinerant electrons in a 1T/1H-TaS_2 heterostructure. We study the heterostructure using scanning tunneling microscopy (STM) and spectroscopy (STS) and s...

We report the construction and performance of a low temperature, high field scanning tunneling mi... more We report the construction and performance of a low temperature, high field scanning tunneling microscope (STM) operating down to 350mK and in magnetic fields up to 9T, with thin film deposition and in-situ cleaving capabilities. The main focus lies on the simple design of STM head allowing top loading of the sample and innovative sample holder design that allows us to get spectroscopic data on superconducting thin films grown in-situ on insulating substrates. Other design details on sample transport, chamber and vibration isolation scheme are also described. We demonstrate the capability of our instrument through the atomic resolution imaging and spectroscopy on NbSe2 single crystal and spectroscopic maps obtained on homogeneously disordered NbN thin film.

The notion of spontaneous formation of an inhomogeneous superconducting state is at the heart of ... more The notion of spontaneous formation of an inhomogeneous superconducting state is at the heart of most theories attempting to understand the superconducting state in the presence of strong disorder. Using scanning tunneling spectroscopy and high resolution scanning transmission electron microscopy, we experimentally demonstrate that under the competing effects of strong homogeneous disorder and superconducting correlations, the superconducting state of a conventional superconductor, NbN, spontaneously segregates into domains. Tracking these domains as a function of temperature we observe that the superconducting domains persist across the bulk superconducting transition, Tc, and disappear close to the pseudogap temperature, T*, where signatures of superconducting correlations disappear from the tunneling spectrum and the superfluid response of the system.

The vortex lattice in a Type II superconductor provides a versatile model system to investigate t... more The vortex lattice in a Type II superconductor provides a versatile model system to investigate the order-disorder transition in a periodic medium in the presence of random pinning. Here, using scanning tunnelling spectroscopy in a weakly pinned Co0.0075NbSe2 single crystal, we show that at low temperatures, the vortex lattice in a 3-dimensional superconductor disorders in two steps across the peak effect. At the onset of the peak effect, the equilibrium Bragg glass transforms into an orientational glass through the proliferation of dislocations. At a higher field, the dislocations dissociate into isolated disclination giving rise to an amorphous vortex glass. We also show the existence of a variety of additional non-equilibrium metastable states, which can be accessed through different thermomagnetic cycling.

Disorder induced melting, where the increase in positional entropy created by random pinning site... more Disorder induced melting, where the increase in positional entropy created by random pinning sites drives the order-disorder transition in a periodic solid, provides an alternate route to the more conventional thermal melting. Here, using real space imaging of the vortex lattice through scanning tunneling spectroscopy, we show that in the presence of weak pinning, the vortex lattice in a type II superconductor disorders through two distinct topological transitions. Across each transition, we separately identify metastable states formed through superheating of the low temperature state or supercooling of the high temperature state. Comparing crystals with different levels of pinning we conclude that the two-step melting is fundamentally associated with the presence of random pinning which generates topological defects in the ordered vortex lattice.

Transition metal dichalcogenides (TMDC) are a rich family of two-dimensional materials displaying... more Transition metal dichalcogenides (TMDC) are a rich family of two-dimensional materials displaying a multitude of different quantum ground states. In particular, d^3 TMDCs are paradigmatic materials hosting a variety of symmetry broken states, including charge density waves, superconductivity, and magnetism. Among this family, NbSe_2 is one of the best-studied superconducting materials down to the monolayer limit. Despite its superconducting nature, a variety of results point towards strong electronic repulsions in NbSe_2. Here, we control the strength of the interactions experimentally via quantum confinement effects and use low-temperature scanning tunneling microscopy (STM) and spectroscopy (STS) to demonstrate that NbSe_2 is in strong proximity to a correlated insulating state. This reveals the coexistence of competing interactions in NbSe_2, creating a transition from a superconducting to an insulating quantum correlated state by confinement-controlled interactions. Our results ...

We report directional point contact Andreev reflection (PCAR) measurements on high-quality single... more We report directional point contact Andreev reflection (PCAR) measurements on high-quality single crystals of the non-centrosymmetric superconductor, BiPd. The PCAR spectra measured on different crystallographic faces of the single crystal clearly show the presence of multiple superconducting energy gaps. For point contacts with low resistance, in addition to the superconducting gap feature, a pronounced zero bias conductance peak is observed. These observations provide strong evidence of the presence of unconventional order parameter in this material.

Bulletin of the American Physical Society, 2018

Scientific Reports, 2013

We measure the frequency dependence of the complex ac conductivity of NbN films with different le... more We measure the frequency dependence of the complex ac conductivity of NbN films with different levels of disorder in frequency range 0.4-20 GHz. Films with low disorder exhibit a narrow dynamic fluctuation regime above T c as expected for a conventional superconductor. However, for strongly disordered samples, the fluctuation regime extends well above T c , with a strongly frequency-dependent superfluid stiffness which disappears only at a temperature * m T close to the pseudogap temperature obtained from scanning tunneling measurements. Such a finite-frequency response is associated to a marked slowing down of the superconducting fluctuations already below * m T. The corresponding large length-scale fluctuations suggest a scenario of thermal phase fluctuations between superconducting domains in a strongly disordered s-wave superconductor.

We report experimental evidence of strong orientational coupling between the crystal lattice and ... more We report experimental evidence of strong orientational coupling between the crystal lattice and the vortex lattice in a weakly pinned Co-doped NbSe2 single crystal through direct imaging using low temperature scanning tunneling microscopy/spectroscopy. At low fields, when the magnetic field is applied along the six-fold symmetric c-axis of the NbSe2 crystal, the equilibrium configuration of the vortex lattice is preferentially aligned along the basis vectors of the crystal lattice. The orientational coupling between the vortex lattice and crystal lattice becomes more pronounced as the magnetic field is increased. We show that this coupling enhances the stability of the orientational order of the vortex lattice, which persists even in the disordered state at high fields where dislocations and disclinations have destroyed the topological order.

arXiv: Mesoscale and Nanoscale Physics, 2020

Transition metal dichalcogenides (TMDC) are a rich family of two-dimensional materials displaying... more Transition metal dichalcogenides (TMDC) are a rich family of two-dimensional materials displaying a multitude of different quantum ground states. In particular, d$^3$ TMDCs are paradigmatic materials hosting a variety of symmetry broken states, including charge density waves, superconductivity, and magnetism. Among this family, NbSe$_2$ is one of the best-studied superconducting materials down to the monolayer limit. Despite its superconducting nature, a variety of results point towards strong electronic repulsions in NbSe$_2$. Here, we control the strength of the interactions experimentally via quantum confinement effects and use low-temperature scanning tunneling microscopy (STM) and spectroscopy (STS) to demonstrate that NbSe$_2$ is in strong proximity to a correlated insulating state. This reveals the coexistence of competing interactions in NbSe$_2$, creating a transition from a superconducting to an insulating quantum correlated state by confinement-controlled interactions. Ou...

Heavy fermion systems represent one of the paradigmatic strongly correlated states of matter. The... more Heavy fermion systems represent one of the paradigmatic strongly correlated states of matter. They have been used as a platform for investigating exotic behavior ranging from quantum criticality and non-Fermi liquid behavior to unconventional topological superconductivity. Heavy fermions arise from the exchange interaction between localized magnetic moments and conduction electrons that leads to the well-known Kondo effect. In a Kondo lattice, the interaction between the localized moments gives rise to a band with heavy effective mass. This intriguing phenomenology has so far only been realized in compounds containing rare-earth elements with 4f or 5f electrons. Here, we realize a designer van der Waals heterostructure where artificial heavy fermions emerge from the Kondo coupling between a lattice of localized magnetic moments and itinerant electrons in a 1T/1H-TaS2 heterostructure. We study the heterostructure using scanning tunneling microscopy (STM) and spectroscopy (STS) and sh...

arXiv: Superconductivity, 2015

We report experimental evidence of strong orientational coupling between the crystal lattice and ... more We report experimental evidence of strong orientational coupling between the crystal lattice and the vortex lattice in a weakly pinned Co-doped NbSe2 single crystal through direct imaging using low temperature scanning tunneling microscopy/spectroscopy. At low fields, when the magnetic field is applied along the six-fold symmetric c-axis of the NbSe2 crystal, the equilibrium configuration of the vortex lattice is preferentially aligned along the basis vectors of the crystal lattice. The orientational coupling between the vortex lattice and crystal lattice becomes more pronounced as the magnetic field is increased. We show that this coupling enhances the stability of the orientational order of the vortex lattice, which persists even in the disordered state at high fields where dislocations and disclinations have destroyed the topological order.

The breakdown of crystalline order in a disordered background connects to some of the most challe... more The breakdown of crystalline order in a disordered background connects to some of the most challenging problems in condensed matter physics. For a superconducting vortex lattice, the equilibrium state in the presence of impurities is predicted to be a "Bragg glass" (BG), where the local crystalline order is maintained everywhere and yet the global positional order decays algebraically. Here, using scanning tunnelling spectroscopy (STS) we image the vortex lattice in a weakly pinned NbSe2 single crystal. We present direct evidence that the ordered state of the VL is a BG, consisting of a large number of degenerate metastable states, which is a hallmark of a glassy state. These results are a significant step towards understanding the disordering of a lattice under the influence of quenched random disorder with a direct impact on various fields, including charge density waves, colloidal crystals and self-organised periodic structures on a substrate.

ABSTRACT Using low temperature scanning tunnelling spectroscopy down to 350 mK we study variety o... more ABSTRACT Using low temperature scanning tunnelling spectroscopy down to 350 mK we study variety of vortex lattice states that emerge in a weakly pinned NbSe2 single crystal. Using small magnetic field pulses, and temperature cycling protocols in magnetic field we access various vortex lattice configurations characterised by different degree of order: Quasi long range ordered states characterised by the absence of topological defects and vortex glass states characterised by the proliferation of dislocations. We explicitly show that the quasi long range ordered state comprises of several metastable states with different "local" configuration of the vortex lattice, consistent with predictions of a Bragg glass.

Bulletin of the American Physical Society, 2019