Time-resolved electron spin resonance spectra of linked radical pairs on laser excitation of zinc tetraphenylporphyrin-viologen systems (original) (raw)

The Journal of Physical Chemistry, 1993

Abstract

Photoinduced electron transfer from the zinc tetraphenylporphyrin moiety to the viologen unit in linked compounds in reversed micelles generated radical pairs, which afforded chemically induced dynamic electron polarization (CIDEP) spectra at room temperature. The CIDEP spectra varied with the number of methylene groups (n) in the alkyl spacer of the linked compounds. In the case of longer spacers (n =

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