Present-day Saharan dust deposition in the Atlantic Ocean and its marine-environmental consequences (original) (raw)

2019, EGUGA

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Abstract

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Mineral dust influences the carbon cycle in the ocean by providing nutrients and metals that can enhance phytoplankton growth and facilitate the sinking of organic matter. This study presents a two-year assessment of dust deposition in the Atlantic, using a network of dust-collecting instruments. The research reveals that summer rains significantly enhance dust nutrient release compared to dry conditions, which may improve surface-ocean productivity and affect broader ecological systems.

Particle size traces modern Saharan dust transport and deposition across the equatorial North Atlantic

Atmospheric Chemistry and Physics Discussions, 2016

Mineral dust has a large impact on regional and global climate, depending on its particle size. Especially in the Atlantic Ocean downwind of the Sahara, the largest dust source on earth, the effects can be substantial but are poorly understood. This study focuses on seasonal and spatial variations in particle size of Saharan dust deposition across the Atlantic Ocean, using an array of submarine sediment traps moored along a transect at 12˚ N. We show that the particle size decreases downwind with increased distance from the Saharan source, due to higher gravitational settling velocities of coarse particles in the atmosphere. Modal grain sizes vary between 4 and 33 μm throughout the different seasons and at five locations along the transect. This is much coarser than previously suggested and incorporated into climate models. In addition, seasonal changes are prominent, with coarser dust in summer, and finer dust in winter and spring. Such seasonal changes are caused by transport at h...

Compositional changes of present-day transatlantic Saharan dust deposition

Atmospheric Chemistry and Physics Discussions, 2016

Massive amounts of Saharan dust are blown from the African coast across the Atlantic Ocean towards the Americas each year. This dust has, depending on its chemistry, direct and indirect effects on global climate including reflection and absorption of solar radiation as well as transport and deposition of nutrients and metals fertilizing both ocean and land. To determine the temporal and spatial variability of Saharan dust transport and deposition and their marine environmental effects across the equatorial North Atlantic Ocean, we have set up a monitoring experiment using deep-ocean sediment traps as well as land-based dust collectors. The sediment traps were deployed at five ocean sites along a transatlantic transect between northwest Africa and the Caribbean along 12⁰ N, in a down-wind extension of the land-based dust collectors placed at 19⁰ N on the Mauritanian coast in Iwik. In this paper, we lay out the setup of the monitoring experiment and present the particle ...

Atmospheric Transport and Deposition of Mineral Dust to the Ocean: Implications for Research Needs

Environmental Science & Technology, 2012

This paper reviews our knowledge of the measurement and modeling of mineral dust emissions to the atmosphere, its transport and deposition to the ocean, the release of iron from the dust into seawater, and the possible impact of that nutrient on marine biogeochemistry and climate. Of particular concern is our poor understanding of the mechanisms and quantities of dust deposition as well as the extent of iron solubilization from the dust once it enters the ocean. Model estimates of dust deposition in remote oceanic regions vary by more than a factor of 10. The fraction of the iron in dust that is available for use by marine phytoplankton is still highly uncertain. There is an urgent need for a long-term marine atmospheric surface measurement network, spread across all oceans. Because the southern ocean is characterized by large areas with high nitrate but low chlorophyll surface concentrations, that region is particularly sensitive to the input of dust and iron. Data from this region would be valuable, particularly at sites downwind from known dust source areas in South America, Australia, and South Africa. Coordinated field experiments involving both atmospheric and marine measurements are recommended to address the complex and interlinked processes and role of dust/Fe fertilization on marine biogeochemistry and climate.

Mass deposition fluxes of Saharan mineral dust to the tropical northeast Atlantic Ocean: an intercomparison of methods

Atmospheric Chemistry and Physics, 2014

Mass deposition fluxes of mineral dust to the tropical northeast Atlantic Ocean were determined within this study. In the framework of SOPRAN (Surface Ocean Processes in the Anthropocene), the interaction between the atmosphere and the ocean in terms of material exchange were investigated at the Cape Verde atmospheric observatory (CVAO) on the island Sao Vicente for January 2009. Five different methods were applied to estimate the deposition flux, using different meteorological and physical measurements, remote sensing, and regional dust transport simulations. The set of observations comprises micrometeorological measurements with an ultra-sonic anemometer and profile measurements using 2-D anemometers at two different heights, and microphysical measurements of the sizeresolved mass concentrations of mineral dust. In addition, the total mass concentration of mineral dust was derived from absorption photometer observations and passive sampling. The regional dust model COSMO-MUSCAT was used for simulations of dust emission and transport, including dry and wet deposition processes. This model was used as it describes the AOD's and mass concentrations realistic compared to the measurements and because it was run for the time period of the measurements. The four observation-based methods yield a monthly average deposition flux of mineral dust of 12-29 ng m -2 s -1 . The simulation results come close to the upper range of the measurements with an average value of 47 ng m -2 s -1 . It is shown that the mass deposition flux of mineral dust obtained by the combination of micrometeorological (ultra-sonic anemometer) and microphysical measurements (particle mass size distribution of mineral dust) is difficult to compare to modeled mass deposition fluxes when the mineral dust is inhomogeneously distributed over the investigated area.

Seasonal impact of mineral dust on deep-ocean particle flux in the eastern subtropical Atlantic Ocean

Marine Geology, 1999

Seasonal lithogenic particle and Al fluxes were obtained from a deep-ocean sediment trap deployment during 1992 and 1993 off NW Africa, and were compared concurrently with atmospheric Al concentrations and two-dimensional backward trajectories of windfields from two barometric levels in the lower and mid troposphere. Marine Al fluxes, lithogenic particle fluxes and grain size distributions in the area were found to be directly linked to airmass pathways and surface mineral Ž found in the sediment traps. The comparison of marine, atmospheric and model derived data used within this study highlights the close temporal coupling between atmospheric dust transport and the deep-ocean particle stock. q

Vertical and areal distribution of Saharan dust over the western equatorial north Atlantic Ocean

Journal of Geophysical Research, 1972

Aerosol measurements were made as a part of the Barbados Oceanographic and Meteorological Experiment (Bomex) during May, June, and July 1969. Maximum dust concentrations occurred between the altitudes of 1.5 km and 3.7 km, a region which we call the Saharan air layer. The average concentration of mineral aerosol within this layer was 61 t•g m-a; in contrast, the average concentration in the low-level air was 22 t•g m -a. These dust concentrations are comparable to those found in continental surface air. Because of the presence of a strong inversion at the base of the Saharan layer, sea. salt was confined to te lower altitudes where the average concentration was 10 tzg m -8. Thus, sea salt appears to be a relatively minor constituent of the trade wind aerosol during much of the year. On the basis of these measurements and of a model describing the movement of Sararan air outbreaks, we estimate that 25 to 37 million tons of dust are transported through the longitude of Barbados each year. This quantity of dust is sufficient to supply all the material required to maintain the present rate of pelagic sedimentation across the entire northern equatorial Atlantic Ocean. The mineral aerosol concentration in sealevel, trade wind air at Barbados, West Indies (13øN, 59øW), has been measured from the fall of 1965 to the present [Delany et al., 1967; Prospero, 1968; Prospero et al., 1970; Carlson and Prospero, 1972]. During the first four years of this program, the air sampling was essentially continuous. These measurements have shown that large quantities of dust are transported across the northern equatorial Atlantic from the deserts of North Africa during the late spring, summer, and early fall. The average surface air concentration of mineral aerosol at Barbados during the dusty season varies from year to year but generally is of the order of 10/•g m -8 of air; the concentration during the rest of the year is more than an order of magnitude less [Prospero, 1968; Carlson and Prospero, 1972]. equatorial North Atlantic and of the relationship of the aerosol distribution to meteorological parameters. The meteorological aspects of this work, a study of the large-scale movement of Sararan air outbreaks over the northern equatorial Atlantic, are presented by us elsewhere [Carlson and Prospero., 1972]

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Tropical Rains Controlling Deposition of Saharan Dust Across the North Atlantic Ocean

Geophysical Research Letters, 2020

Mineral dust plays an important role in the atmospheric radiation budget as well as in the ocean carbon cycle through fertilization and by ballasting of settling organic matter. However, observational records of open‐ocean dust deposition are sparse. Here, we present the spatial and temporal evolution of Saharan dust deposition over 2 years from marine sediment traps across the North Atlantic, directly below the core of the Saharan dust plume, with highest dust fluxes observed in summer. We combined the observed deposition fluxes with model simulations and satellite observations and argue that dust deposition in the Atlantic is predominantly controlled by summer rains. The dominant depositional pathway changes from wet deposition in summer to dry deposition in winter. Wet deposition has previously been suggested to increase the release of dust‐derived nutrients and their bioavailability, which may be a key contributor to surface‐ocean productivity in remote and oligotrophic parts of...

Effects of dry and wet Saharan dust deposition in the tropical North Atlantic Ocean

Biogeosciences Discussions

Incubation experiments comprising Saharan dust additions were conducted in the tropical North Atlantic Ocean along an east-west transect at 12°N to study the phytoplankton response to nutrient release in oligotrophic seawater conditions. Experiments were performed at three stations (M1, M3, M4), mimicking wet and dry deposition of low and high amounts of Saharan dust deposition from two different dust sources (paleo-lake and sand dune). Dust particle sizes were adjusted to resemble dust that is naturally deposited over the ocean at the experiment sites. For wet dust deposition, the dust was pre-20 leached in acidified 'artificial rainwater' (H2SO4) for 16 to 24 hours, mimicking acid cloud processing at different pH values. Experiments were run up to eight days. Daily nutrient measurements of phosphate (PO4 3-), silicate (SiO4 4-), nitrate (NO3-) and cell abundances were performed in addition to measurements of concentrations of total dissolved iron (DFe), particulate organic carbon (POC), and dissolved inorganic carbon (DIC) at the start and at the end of the experiments. A significant initial increase and subsequent gradual decrease in PO4 3-, SiO4 4and DFe concentrations were observed after wet 25 dust deposition using high amounts of dust previously leached in low pH rain (H2SO4, pH=2). Remarkably, the experiments showed no nutrient release (PO4 3-, SiO4 4and DFe) from dry-dust addition and the NO3concentrations remained unaffected in all (dry and wet) experiments. The prokaryotic cyanobacterium Synechococcus spp. was the most prominent picophytoplankton in all mixed layer experiments. After an initial increase in cell abundance, a subsequent decrease (at M1) or a slight increase (at M3) with similar temporal dynamics was observed for dry-and wet-dust deposition experiments. The 30 POC concentrations increased in all experiments and showed similar high values after both dry and wet dust deposition treatments, even though wet dust deposition is considered to have a higher potential to introduce bioavailable nutrients (i.e. PO4 3-, SiO4 4and DFe) into the otherwise nutrient-starved oligotrophic ocean. Our observations suggest that such nutrients may be more likely to favor the growth of the phytoplankton community when an additional N-source is also available. In addition to acting as a fertilizer, our results from both dry and wet dust deposition experiments suggest that Saharan dust 35 particles might be incorporated into marine snow aggregates leading to similar high POC concentrations.

Carbon sequestration in the deep Atlantic enhanced by Saharan dust

Nature Geoscience, 2017

Enhanced atmospheric input of dust-borne nutrients and minerals to the remote surface ocean can potentially increase carbon uptake and sequestration at depth. Nutrients can enhance primary productivity, and mineral particles act as ballast, increasing sinking rates of particulate organic matter. Here we present a unique 2-year time-series of sediment-trap observations of particulate organic carbon flux to 3000 m depth, measured directly in two locations: the dust-rich central North Atlantic gyre and the dust-poor South Atlantic gyre. We find that carbon fluxes are twice as high and a higher proportion of primary production is exported to depth in the dust-rich North Atlantic gyre. Low stable nitrogen isotope ratios suggest that high fluxes result from the stimulation of nitrogen fixation and productivity following the deposition of dust-borne nutrients. Sediment traps in the northern gyre also collected intact colonies of nitrogen-fixing Trichodesmium species. Whereas ballast in the southern gyre is predominantly biogenic, dust-derived mineral particles constitute the dominant ballast element during the enhanced carbon fluxes in the northern gyre. We conclude that dust deposition increases

Atmospheric and oceanic dust fluxes in the northeastern tropical Atlantic Ocean: how close a coupling?

Annales Geophysicae, 2002

Atmospheric inputs to the ocean of dust originating from Africa are compared with downward dust flux in the oceanic water column. Atmospheric fluxes were estimated using remote-sensing-derived dust optical thickness and parameters from a transport/deposition model (TM2z). Oceanic fluxes were measured directly over/in two regions of contrasting primary productivity of the northeastern tropical Atlantic (one mesotrophic and one oligotrophic, located at about 500 and 1500 km off Mauritania) underlying the offshore dust plume. In both regions, estimates of annual atmospheric dust inputs to the ocean surface are lower than, but of the same order of magnitude as, oceanic fluxes (49.5 and 8.8 mg.m −2 .d −1 in the mesotrophic and oligotrophic regions). Part of this mismatch may reflect both a general flaw in the dust grain size distribution used in transport models, which likely underestimates large particles, and/or lateral advection to each region of dustier surface waters from upstream, where dust deposition is higher. Higher-frequency temporal coupling between atmospheric and oceanic fluxes seems to be primary-productivity dependent, as hypothesized in previously reported studies.

Revisiting atmospheric dust export to the Southern Hemisphere ocean: Biogeochemical implications

Global Biogeochemical Cycles, 2008

1] Aerosol concentrations in the Southern Hemisphere are largely undersampled. This study presents a chemical and physical description of dust particles collected on board research vessels in the southeast Pacific (SEPS) and the Southern Ocean (SOKS). Concentrations of dust were 6.1 ± 2.4 ng m À3 for SEPS and 13.0 ± 6.3 ng m À3 for SOKS. Dust fluxes, derived from those concentrations, were 9.9 ± 3.7 mg m À2 d À1 for SEPS and 38 ± 14 mg m À2 d À1 for SOKS and are shown to be representative of actual fluxes in those areas. Dust and iron deposition are up to 2 orders of magnitude lower than former predictions. A map of dust deposition on the Southern Hemisphere is proposed by incorporating those in situ measurements into a dust model. This study confirms that dust deposition is not the dominant source of iron to the large high-nutrient low-chlorophyll Southern Ocean.

Estimates of African Dust Deposition Along the Trans‐Atlantic Transit Using the Decadelong Record of Aerosol Measurements from CALIOP, MODIS, MISR, and IASI

Journal Of Geophysical Research: Atmospheres, 2019

Deposition of mineral dust into ocean fertilizes ecosystems and influences biogeochemical cycles and climate. In-situ observations of dust deposition are scarce, and model simulations depend on the highly parameterized representations of dust processes with few constraints. By taking advantage of satellites' routine sampling on global and decadal scales, we estimate African dust deposition flux and loss frequency (LF, a ratio of deposition flux to mass loading) along the transAtlantic transit using the three-dimensional distributions of aerosol retrieved by spaceborne lidar (CALIOP) and radiometers (MODIS, MISR, and IASI). On the basis of a ten-year (2007-2016) and basin scale average, the amount of dust deposition into the tropical Atlantic Ocean is estimated at 136-222 Tg yr-1. The 65-83% of satellite-based estimates agree with the in-situ climatology within a factor of 2. The magnitudes of dust deposition are highest in boreal summer and lowest in fall, whereas the interannual variability as measured by the normalized standard deviation with mean is largest in spring (28-41%) and smallest (7-15%) in summer. The dust deposition displays high spatial heterogeneity, revealing that the meridional shifts of major dust deposition belts are modulated by the seasonal migration of the intertropical convergence zone (ITCZ). On the basis of the annual and basin mean, the dust LF derived from the satellite observations ranges from 0.078 to 0.100 d −1 , which is lower than model simulations by up to