Irregular sesquiterpenoids from Ligusticum grayi roots (original) (raw)
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Sesquiterpene lactones from the Yugoslavian wild growing plant families asteraceae and apiaceae
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Tetrahedron, 1968
+ f+Eudesmol (I) has been synthesized in a highly stereoselective. lO-stage route from the octalone 2 Several of the synthetic intermediates are potentially useful compounds for the synthesis of other eudesmane sesquiterpenoids. ~EUDESMOL * A search of Chemical Abstracts indices through June, 1965, reveals that this compound, usually admixed with the a-and y-isomers (i and ii) has been isolated from more than thirty sources. pvO" gho. t Throughout this paper. x£s will be numbered as derivatl!:es of naphthalene, in keeping with current Chemical Abstracts practice. The traditional numbering system for eudesmane sesquiterpenoids is given in Fig. iii.
Atypical Lindenane-Type Sesquiterpenes from Lindera myrrha
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Two new lindenane sesquiterpenes were obtained from the roots of Lindera myrrha. These compounds were structurally elucidated by HRMS data, extensive NMR analyses, and comparison between experimental and theoretical 13C-NMR data. Myrrhalindenane A is the first monomeric seco-d lindenane displaying a non-rearranged, cyclohexanic C-ring. Myrrhalindenane B is the second occurrence of an angular lindenane-sesquiterpene related to a C6-C7 lactonization.
Sesquiterpenes from southern Magnolia virginiana
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Composition of the essential oil and the hydrosol of the roots of Ligusticum porteri
Monoterpenes and monoterpenes derivatives constitute the main part of the essential oil of the roots of Ligusticum porteri. Sabinene (9.0-15.5%) and p-cymene (6.5-9.7%) are the main compounds of monoterpene hydrocarbons along with a rather unusual compound: viridene (19.4%). trans-Sabinyl acetate (22.6%) is by far the most important oxygenated monoterpene. Several compounds are observed among the sesquiterpene group with percentage generally lower than 1%. The most important compound in one sample is thapsadiene (0.6%) and in the second sample is -selinene (0.7%). Finally, several recently described oxygenated sesquiterpenoids are among the minor compounds. The most important are: -prethapsenol (1.7-3.3%), -preisothapsenol (0.8-1.6%) and β-isoligustigrenol (0.6-1.3%) along with (Z)-ligustilide (0.7%). The hydrosol does not show the presence of hydrocarbon compounds. However, oxygenated compounds such as terpinen-4-ol (16.5 mg/L), including some compounds not observed in the oil such as hexanal (2.5 mg/L), furfural (2.0 mg/L) and p-cymen-8ol (2.5 mg/L), are observed in the hydrosol.