CO2-Activation by size-selected tantalum cluster cations (Ta1–16+): thermalization governing reaction selectivity (original) (raw)

CO2-Activation by size-selected tantalum cluster cations (Ta1–16+): thermalization governing reaction selectivity

Physical Chemistry Chemical Physics, 2022

Abstract

Tantalum cluster cations react with CO2 either via transfer of oxygen atoms to the clusters or the adsorption of an entire molecule. The released energy and vibrational heat capacities are assigned to determine the branching ratios of the pathways.

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