Tunable Superconducting Phase Transition in Metal-Decorated Graphene Sheets (original) (raw)
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Gate-Tunable Superconducting-Insulating Transition in Tin-Decorated Graphene
2012
Graphene 1 is a sturdy and chemically inert material exhibiting an exposed two-dimensional electron gas of high mobility. These combined properties enable the design of graphene composites, based either on covalent 2 or non-covalent 3 coupling of adsorbates, or on stacked and multilayered heterostructures 4 . These systems have shown tunable electronic properties such as bandgap engineering 3 , reversible metal-insulating transition 2,4 or supramolecular spintronics 5 . Tunable superconductivity is expected as well 6 , but experimental realization is lacking. Here, we show experiments based on metal-graphene hybrid composites, enabling the tunable proximity coupling of an array of superconducting nanoparticles of tin onto a macroscopic graphene sheet. This material allows full electrical control of the superconductivity down to a strongly insulating state at low temperature. The observed gate control of superconductivity results from the combination of a proximity-induced superconductivity generated by the metallic nanoparticle array with the two-dimensional and tunable metallicity of graphene. The resulting hybrid material behaves, as a whole, like a granular superconductor showing universal transition threshold and localization of Cooper pairs in the insulating phase. This experiment sheds light on the emergence of superconductivity in inhomogeneous superconductors, and more generally, it demonstrates the potential of graphene as a versatile building block for the realization of superconducting materials.
Tuning Superconductivity in Two Dimensions with a Novel Metal-Graphene Hybrid Material
2010
Using typical experimental techniques, such as chemical doping, it is difficult to isolate the effects of carrier density from disorder on a two-dimensional superconducting transition. To circumvent this problem, we have produced graphene sheets covered with a non-percolating network of nanoscale tin clusters. This network of disordered metal clusters efficiently dopes the graphene substrate and induces long-range superconducting correlations by
Scientific reports, 2015
The influence of static disorder on a quantum phase transition (QPT) is a fundamental issue in condensed matter physics. As a prototypical example of a disorder-tuned QPT, the superconductor-insulator transition (SIT) has been investigated intensively over the past three decades, but as yet without a general consensus on its nature. A key element is good control of disorder. Here, we present an experimental study of the SIT based on precise in-situ tuning of disorder in dual-gated bilayer graphene proximity-coupled to two superconducting electrodes through electrical and reversible control of the band gap and the charge carrier density. In the presence of a static disorder potential, Andreev-paired carriers formed close to the Fermi level in bilayer graphene constitute a randomly distributed network of proximity-induced superconducting puddles. The landscape of the network was easily tuned by electrical gating to induce percolative clusters at the onset of superconductivity. This is...
Electrical control of the superconducting-to-insulating transition in graphene–metal hybrids
Nature Materials, 2012
Graphene is a sturdy and chemically inert material exhibiting an exposed two-dimensional electron gas of high mobility. These combined properties enable the design of graphene composites, based either on covalent or non-covalent coupling of adsorbates, or on stacked and multilayered heterostructures. These systems have shown tunable electronic properties such as bandgap engineering, reversible metal-insulating transition or supramolecular spintronics. Tunable superconductivity is expected as well, but experimental realization is lacking. Here, we show experiments based on metal-graphene hybrid composites, enabling the tunable proximity coupling of an array of superconducting nanoparticles of tin onto a macroscopic graphene sheet. This material allows full electrical control of the superconductivity down to a strongly insulating state at low temperature. The observed gate control of superconductivity results from the combination of a proximity-induced superconductivity generated by the metallic nanoparticle array with the two-dimensional and tunable metallicity of graphene. The resulting hybrid material behaves, as a whole, like a granular superconductor showing universal transition threshold and localization of Cooper pairs in the insulating phase. This experiment sheds light on the emergence of superconductivity in inhomogeneous superconductors, and more generally, it demonstrates the potential of graphene as a versatile building block for the realization of superconducting materials.
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Unconventional superconductivity featuring large pairing energies has attracted immense interest, yet tractable microscopic theories have proven elusive. A major breakthrough has been the advent of twisted bilayer graphene (TBG), which serves as a simple model system to 'look under the hood' of unconventional superconductivity. We propose a new model, within current experimental reach, to investigate the microscopics of strong-binding superconductivity. Our proposed device is semiconductor artificial graphene (AG), a two dimensional electron gas overlaid with a periodic potential (superlattice). We demonstrate a new mechanism for superconductivity that originates solely from the repulsive Coulomb interaction. The superlattice promotes certain interactions, which are antiscreened, cause attractive ppp-wave pairing and - in contrast to graphene - can be strongly enhanced through device engineering. The strength of the pairing energy is similar to TBG, and we find within the ac...
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The superconducting transition temperature (Tc) of a single layer graphene coupled to an Indium oxide (InO) film, a low carrier-density superconductor, is found to increase with decreasing carrier density and is largest close to the average charge neutrality point in graphene. Such an effect is very surprising in conventional BCS superconductors. We study this phenomenon both experimentally and theoretically. Our analysis suggests that the InO film induces random electron and hole-doped puddles in the graphene. The Josephson effect across these regions of opposite polarity enhances the Josephson coupling between the superconducting clusters in InO, along with the overall Tc of the bilayer heterostructure. This enhancement is most effective when the chemical potential of the system is tuned between the charge neutrality points of the electron and hole-doped regions.
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We study graphene ferromagnet/superconductor/ferromagnet (F/S/F) nanostructures via a microscopic selfconsistent Dirac Bogoliubov-de Gennes formalism. We show that as a result of proximity effects, experimentally accessible spin switching phenomena can occur as one tunes the Fermi level µF of the F regions or varies the angle θ between exchange field orientations. Superconductivity can then be switched on and off by varying either θ or µF (a spin-controlled superconducting graphene switch). The induced equal-spin triplet correlations in S can be controlled by tuning µF , effectively making a graphene based two-dimensional spin-triplet valve.
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a Josephson junction array is built with hybrid superconductor/metal/superconductor junctions, a quantum phase transition from a superconducting to a two-dimensional (2D) metallic ground state is predicted to happen upon increasing the junction normal state resistance. Owing to its surface-exposed 2D electron gas and its gate-tunable charge carrier density, graphene coupled to superconductors is the ideal platform to study the above-mentioned transition between ground states. Here we show that decorating graphene with a sparse and regular array of superconducting nanodisks enables to continuously gate-tune the quantum superconductor-to-metal transition of the Josephson junction array into a zero-temperature metallic state. The suppression of proximity-induced superconductivity is a direct consequence of the emergence of quantum fluctuations of the superconducting phase of the disks. Under perpendicular magnetic field, the competition between quantum fluctuations and disorder is responsible for the resilience at the lowest temperatures of a superconducting glassy state that persists above the upper critical field. Our results provide the entire phase diagram of the disorder and magnetic field-tuned transition and unveil the fundamental impact of quantum phase fluctuations in 2D superconducting systems.
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Artificial lattices have served as a platform to study the physics of unconventional superconductivity. We study semiconductor artificial graphene-a honeycomb superlattice imposed on a semiconductor heterostructure-which hosts the Dirac physics of graphene but with a tunable periodic potential strength and lattice spacing, allowing control of the strength of the electron-electron interactions. We demonstrate a new mechanism for superconductivity due to repulsive interactions which requires a strong lattice potential and a minimum doping away from the Dirac points. The mechanism relies on the Berry phase of the emergent Dirac fermions, which causes oppositely moving electron pairs near the Dirac points to interfere destructively, reducing the Coulomb repulsion and thereby giving rise to an effective attraction. The attractive component of the interaction is enhanced by a novel antiscreening effect which, in turn, increases with doping; as a result there is a minimum doping beyond which superconducting order generically ensues. The dominant superconducting state exhibits a spatially modulated gap with chiral p-wave symmetry. Microscopic calculations suggest that the possible critical temperatures are large relative to the low carrier densities, for a range of experimentally realistic parameters.