Surface-Plasmon-Enhanced Photodriven CO2 Reduction Catalyzed by Metal-Organic-Framework-Derived Iron Nanoparticles Encapsulated by Ultrathin Carbon Layers (original) (raw)

Advanced materials (Deerfield Beach, Fla.), 2016

Abstract

Highly efficient utilization of solar light with an excellent reduction capacity has been achieved for plasmonic Fe@C nanostructures. By carbon layer coating, the optimized catalyst exhibits enhanced selectivity and stability applied to the solar-driven reduction of CO2 into CO. The surface-plasmon effect of iron particles has been proposed to excite CO2 molecules, and thereby facilitates the final reaction activity.

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