Proton beam writing: a tool for high-aspect ratio mask production (original) (raw)

2007, Microsystem Technologies

P-beam writing (proton beam writing), a direct write 3D nano lithographic technique has been employed for the production of X-ray masks in a single step fabrication process, with high aspect ratios and extremely smooth absorber edges. P-beam writing employs a focused MeV proton beam scanned in a predetermined pattern over a resist (e.g. PMMA or SU-8), which is subsequently chemically developed. P-beam writing in combination with electroplating appears ideally suited to directly write X-ray masks with nano sized features, high aspect ratios, small lateral feature sizes, and smooth and vertical sidewalls. Sub 100 nm resist structures with aspect ratios up 160 have been produced, as well as metallic (nickel) structures down to the 100 nm level. Preliminary tests on p-beam written X-ray test masks show that Ni stencils can be fabricated with a thickness of 2-20 lm, smooth side walls, feature details down to 1 lm, and aspect ratios up to 20.

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The fabrication of x-ray masks using proton beam writing

Journal of Micromechanics and Microengineering, 2008

We have developed a simplified method of fabricating x-ray masks for deep x-ray lithography by using proton beam writing (PBW) without subsequent soft x-ray copying steps. Combining direct PBW and subsequent electroplating, x-ray masks with gold absorber patterns of up to 11 µm height and with vertical and smooth sidewalls were fabricated. The smallest size in the absorber pattern is less than 0.5 µm in this work. The masks were used for x-ray lithography with synchrotron radiation, and 870 µm SU-8 structures with smooth sidewalls were produced. This fabrication method is promising to be an important alternative to conventional methods for x-ray mask making.

Fabrication of high aspect ratio 100 nm metallic stamps for nanoimprint lithography using proton beam writing

Applied Physics Letters, 2004

We report a way of fabricating high-quality void-free high-aspect-ratio metallic stamps of 100 nm width and 2 m depth, using the technique of proton beam writing coupled with electroplating using a nickel sulfamate solution. Proton beam writing is a one-step direct-write process with the ability to fabricate nanostructures with high-aspect-ratio vertical walls and smooth sides, and as such has ideal characteristics for three-dimensional (3D) stamp fabrication. Nanoindentation and atomic force microscopy measurements of the nickel surfaces of the fabricated stamp show a hardness and side-wall roughness of 5 GPa and 7 nm, respectively. The fabricated 100 nm 3D stamps have been used to transfer test patterns into poly(methylmethacrylate) films, spin coated onto a silicon substrate. Proton beam writing coupled with electroplating offers a process of high potential for the fabrication of high quality metallic 3D nanostamps.

Fabrication of X-Ray Masks Using the Silicon Direct Write Electron-Beam Lithography Process and Complementary Electron-Sensitive Resists

Japanese Journal of Applied Physics, 2002

In order to meet the long term goals of the International Technology Roadmap for Semiconductors, it is important to demonstrate that X-ray masks can be fabricated at resolutions well below the 100 nm barrier. This paper presents results on the use of conventional electron-sensitive resists and the silicide direct write electron beam lithography process (SiDWEL) for the fabrication of X-ray masks with sub-100 nm resolution. By optimizing the deposition of the thin films using conventional evaporators, the SiDWEL process was able to achieve linewidths of less than 40 nm and line spacing of less than 100 nm. The silicide patterns formed by the SiDWEL process are sufficiently resistant to plasma etching to directly transfer the patterns to the tantalum absorber. To improve the turnover time for mask fabrication, different writing schemes were studied, including combining the SiDWEL process with QSR-4, a novel negative resist designed specifically for this application.

Proton beam writing: a progress review

2004

A new direct write 3D nano lithographic technique has been developed at the Centre for Ion Beam Applications (CIBA) in the Physics Department of the National University of Singapore. This technique employs a focused MeV proton beam which is scanned in a predetermined pattern over a resist (e.g. PMMA or SU-8), which is subsequently chemically developed. The secondary electrons induced by the primary proton beam have low energy and therefore limited range, resulting in minimal proximity effects. Low proximity effects coupled with the straight trajectory and high penetration of the proton beam enables the production of 3D micro and nano structures with well-defined smooth side walls to be directly written into resist materials. In this review the current status of proton beam writing will be discussed; recent tests have shown this technique capable of writing high aspect ratio walls up to 160 and details down to 30 nm in width with sub-3 nm edge smoothness.

Fast prototyping of high-aspect ratio, high-resolution X-ray masks by gas-assisted focused ion beam

Microsystem Technologies, 2003

The capacity of chemically-assisted Focused Ion Beam (FIB) etching systems to undertake direct and highly anisotropic erosion of thin and thick gold (or other high atomic number (2)) coatings on X-ray mask membraneshbstrates provides new levels of precision, flexibility, simplification and rapidity in the manufacture of mask absorber patterns, allowing for fast prototyping of highaspect ratio, high-resolution masks for deep X-ray lithography. In preliminary demonstrations of an automated FIB system operating at 30 keV with a gallium liquid metal source and an iodine gas injection system illustrated the capability of the technique for direct milling into a few micrometer thick gold. Focused ion beam diameters as small as 7nm were obtained, enabling fabrication well into the sub-hundred nanometer regime.

Improvement in proton beam writing at the nano scale

2004

Here we report on the progress of 3D nano machining using MeV protons. In proton beam (p-beam) writing a proton beam is typically focused down to a sub 100 nm spot size and scanned over a resist material (e.g. Su-8 or PMMA). Currently the scanning is performed using a magnetic scan coil which has an intrinsically long settling time. A new scanning system is introduced which employs electrostatic scanning and allows an increase in writing speed up to 2 orders of magnitude.

Polymer-based X-ray masks patterned by direct laser writing

Review of Scientific Instruments, 2018

X-ray masks are indispensable tools in deep X-ray lithography (XRL). To date, hardly any fabrication technology can provide affordable and readily available masks with good structure quality. The bottleneck of adequate masks to a large extent limits the widespread use of XRL. In this article, an alternative XRL mask fabrication process is described to significantly improve availability and cost efficiency of XRL masks as key instruments in XRL processing: A 355 nm UV-laser is applied to expose SU-8 resist on an antireflective coating and a copper sacrificial substrate. The voids in this resist template are filled by a two-step electroplating process with sacrificial nickel and 3.6 μm thick gold absorbers. A second SU-8 coat embeds the absorbers, forming the 40 μm mask membrane. This configuration allows for XRL into resists of up to about 200 μm thickness at the SyLMAND beamline, Canada. The absorber structure accuracy is about 1 μm, at smallest tested lateral dimensions of 2 μm iso...

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