Atoms in ultra-intense laser fields (original) (raw)

1993, Journal of Physics B: Atomic, Molecular and Optical Physics

The interaction of an atom with an ultra-intense radiation field is characterized by the involvement of many photons in absorptions and emissions. Of course the word 'intense' has to be compared with some atomic reference: if the induced transition coupling between bound states exceeds inherent widths, then the dressed atom Rabi oscillations which dominate the atomic evolution are typical intense field effects, even though laser intensities may actually be quite modest. When laser intensities exceed IOi3 Wcm-', and infrared frequencies are employed, tben free electrons are dressed by interaction energies which exceed the photon energies. Non-perturbative continuum processes such as abovethreshold ionization then occur, combined with the emission of very high order harmonics ofthe pump laser frequency. At higher laser intensities, the optical electric field can exceed the Coulombic binding electric field and allow aver-the-barrier ionization. which defines a new regime of high intensity physics. In this region (or at higher intensities) the atomic electron charge cloud oscillates in the laser field with large amplitude excursions from the nucleus, during which time it is unable to absorb further photons. This stabilization regime is predicted to persist until the electron dressing energy approaches the restmass energy when wholly unexplored regions remain 10 be investigated. In this topical review, we examine theorelied models of atoms dressed by intense fields. We review the breakdown of lowest-order perturbation theory and those 'essential states' methods adopted to include Rabi frequencies, Stark shifts, induced widths and continuum dressing. Newer methods more suitable for super-svong fields are described, such as Floquet and Valkov methods and the direct numerical integration ofthe Schr6dinger equation. Such methods are used to provide completely non-perturbative strong field descriptions of atomic dynamics. We conclude with a brief examination of the relativistic effects expected to be important when new high intensity ultrashort pulse lasers currently under development are employed in strong field physics. photon absorption in a crystal [3] and Abella observed such absorption in caesium atoms in 1963 [4]. Multiphoton ionization (MPI) was first observed in the experiments

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Atoms and Di-Atoms in Intense Laser Fields

A series of experimental studies was carried out on diatomic molecules to understand how they interact with intense laser fields. These studies have mainly consisted of multiple photon excitation, ionization and dissociation of hydrogen, oxygen, and chlorine molecules using time of flight electron and ion spectroscopy. I took advantage of the similarities and differences in the molecular structure of these molecules in order to investigate whether differ ent molecules interact differently with the applied fields. Clear experimental evidence of molecular Bond Softening as an intensity dependent variation in the vibrational distribution of molecular ions is being reported for the first time in H2 and D2. The competition between different channels in the above threshold dissociation of molecules had been predicted recently using the dressed molecular states model. My results on these branching ratios are qualitatively consistent with the theoretical predictions. The study on oxygen concentrated mainly on the anomalous intensity dependence of the final state vibrational distribution. I have used a model similar to Smith's model to explain the role intermediate states play in the ionization of oxy gen. In a series of arguments, I have shown that this anomalous behavior can be explained as a pure intermediate state interplay in the first approxima tion. Finally, in the photoelectron spectroscopy of chlorine, I have observed the positive Ponderomotive shifts known for a long time but never directly observed before. Also observed in the spectra is a very low order above threshold ionization process of highly excited atoms. These observations in chlorine suggest an unexplored mechanism of exposing atoms to intense fields without the risk of their ionization in the rising part of the laser pulses.

Two-electron atoms in short intense laser pulses

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We discuss a method of solving the time dependent Schrödinger equation for atoms with two active electrons in a strong laser field, which we used in a previous paper [ A. Scrinzi and B. Piraux, Phys. Rev. A 56, R13 (1997) ] to calculate ionization, double excitation and harmonic generation in Helium by short laser pulses. The method employs complex scaling and an expansion in an explicitly correlated basis. Convergence of the calculations is documented and error estimates are provided. The results for Helium at peak intensities up to 10 15 W/cm 2 and wave length 248 nm are accurate to at least 10 %. Similarly accurate calculations are presented for electron detachment and double excitation of the negative hydrogen ion.

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Australian journal of physics, 1998

Laser assisted inelastic scattering of heavy ions by alkali atoms is studied theoretically. The non-perturbative quasi-energy method, generalised for many states, is used to describe the laser-atom interaction, and the close coupling method using the ...

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Journal of Modern Optics, 2003

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