Fluidic vortices generated from optical vortices in a microdroplet cavity (original) (raw)

Laser microfluidics: fluid actuation by light

Journal of Optics A: Pure and Applied Optics, 2009

The development of microfluidic devices is still hindered by the lack of robust fundamental building blocks that constitute any fluidic system. An attractive approach is optical actuation because light field interaction is contactless and dynamically reconfigurable, and solutions have been anticipated through the use of optical forces to manipulate microparticles in flows. Following the concept of "optical chip" advanced from the optical actuation of suspensions, we propose in this survey new routes to extend this concept to microfluidic two-phase flows. First, we investigate the destabilization of fluid interfaces by the optical radiation pressure and the formation of liquid jets. We analyze the droplet shedding from the jet tip and the continuous transport in laser-sustained liquid channels. In a second part, we investigate a dissipative light-flow interaction mechanism consisting in heating locally two immiscible fluids to produce thermocapillary stresses along their interface. This opto-capillary coupling is implemented in adequate microchannel geometries to manipulate two-phase flows and propose a contactless optical toolbox including valves, droplet sorters and switches, droplet dividers or droplet mergers. Finally, we discuss radiation pressure and opto-capillary effects in the context of the "optical-chip" where flows, channels and operating functions would all be performed optically on the same device.

Microscale solute flow probed with rotating microbead trapped in optical vortex

Experiments in Fluids, 2021

The dynamics of solute flow in the microscopic chamber can be studied with optical tweezers. A method based on the metallic microbeads trapped in the focused optical vortex beam is proposed. This annular beam of a twisted wavefront exerts torque on a reflective object placed inside the dark core of the vortex. The induced rotational movement of the bead is sensitive to local viscosity changes in the surrounding medium, for example, during the ongoing dissolution process. Two experimental configurations are described, both relying on tracing the angular velocity of the bead in time. In one-bead configuration, the dynamics of local solute concentration can be studied. In two-bead case, the direction and speed of solute flow can be probed with a spatial resolution of single micrometers. We approach the elementary problem of sucrose dissolution and diffusion in water. The surprising impression of the reverse solute flow was observed. Further experimental investigation led to the discovery that this phenomenon originates from the sucrose stream-like diffusion in the mid-depth of the measurement chamber. The rotating microbead method applies for various solid and liquid substances and may become a useful technique for microfluidics research.

Optical manipulation of a dielectric particle along polygonal closed-loop geometries within a single water droplet

Scientific Reports, 2021

We report a new method to optically manipulate a single dielectric particle along closed-loop polygonal trajectories by crossing a suite of all-fiber Bessel-like beams within a single water droplet. Exploiting optical radiation pressure, this method demonstrates the circulation of a single polystyrene bead in both a triangular and a rectangle geometry enabling the trapped particle to undergo multiple circulations successfully. The crossing of the Bessel-like beams creates polygonal corners where the trapped particles successfully make abrupt turns with acute angles, which is a novel capability in microfluidics. This offers an optofluidic paradigm for particle transport overcoming turbulences in conventional microfluidic chips.

Optical Fluid Pump: Generation of Directional Flow via Microphase Segregation/Homogenization

Journal of Physical Chemistry Letters, 2018

We report the successful generation of directional liquid-flow under stationary laser irradiation at a fixed position in a chamber. We adopt a homogeneous solution consisting of a mixture of water and triethylamine (TEA), with a composition near the critical point for phase segregation. When geometrical asymmetry is introduced around the laser focus in the chamber, continuous directional flow is generated, accompanied by the emergence of water-rich microdroplets at the laser focus. The emerging microdroplets tend to escape toward the surrounding bulk solution and then merge/annihilate into the homogeneous solution. The essential features of the directional flow are reproduced through a simple numerical simulation using fluid dynamic equations.

Observation of whispering gallery modes in elastic light scattering from microdroplets optically trapped in a microfluidic channel

Journal of the Optical Society of America B, 2016

Optical whispering gallery modes (WGMs) were observed in elastic scattering spectra recorded from oil-in-water emulsion droplets in a microfluidic channel. Droplets with diameters ranging between 15 and 50 μm were trapped by optical tweezers near the tip of a single mode fiber that enabled the excitation of the WGMs using a tunable laser. Quality factors of the WGMs were observed to increase with droplet size. WGMs with quality factors of more than 10 4 were observed for droplets with diameters around 45 μm. In some cases, recorded WGMs drifted monotonically to the blue end of the spectrum due to droplet dissolution in the host liquid. Fluctuating spectral shifts to both blue and red ends of the spectrum were also observed. These were attributed to the presence of randomly diffusing particulate contaminants in the droplet liquid, indicating the potential of optically trapped droplet resonators for optical sensing applications.

Water-Walled Microfluidics Makes an Ultimate Optical Finesse

arXiv: Optics, 2015

Liquids serve microcavity research ever since Ashkins studies on optical resonances in levitating droplets to recent optofluidic resonators. Droplets can provide optical quality factor (Q) in proximity to the limit restricted by water absorption and radiation loss. However, water micro-drops vaporize quickly due to their large area to volume ratio. Here we fabricate a water-air interface that almost entirely surrounds our device, allowing for more than 1,000,000 recirculations of light (finesse). We sustain the droplets for longer than 16 hours using a nano-water-bridge that extends from the droplet to a practically-unlimited distant-reservoir that compensates for evaporation. Our device exhibits surface tension 8000-times stronger than gravity that self-stabilizes its shape to a degree sufficient to maintain critical coupling as well as to resolve split modes. Our device has 98 percents of their surrounding walls made strictly of water-air interfaces with concave, convex or saddle ...

High-Throughput Optofluidic Acquisition of Microdroplets in Microfluidic Systems

Micromachines, 2018

Droplet optofluidics technology aims at manipulating the tiny volume of fluids confined in micro-droplets with light, while exploiting their interaction to create "digital" micro-systems with highly significant scientific and technological interests. Manipulating droplets with light is particularly attractive since the latter provides wavelength and intensity tunability, as well as high temporal and spatial resolution. In this review study, we focus mainly on recent methods developed in order to monitor real-time analysis of droplet size and size distribution, active merging of microdroplets using light, or to use microdroplets as optical probes.

Direct Measurement of Unsteady Microscale Stokes Flow Using Optically Driven Microspheres

2020

A growing body of work on the dynamics of eukaryotic flagella has noted that their oscillation frequencies are sufficiently high that the viscous penetration depth of unsteady Stokes flow is comparable to the scales over which flagella synchronize. Incorporating these effects into theories of synchronization requires an understanding of the global unsteady flows around oscillating bodies. Yet, there has been no precise experimental test on the microscale of the most basic aspects of such unsteady Stokes flow: the orbits of passive tracers and the position-dependent phase lag between the oscillating response of the fluid at a distant point and that of the driving particle. Here, we report the first such direct Lagrangian measurement of this unsteady flow. The method uses an array of 30 submicron tracer particles positioned by a time-shared optical trap at a range of distances and angular positions with respect to a larger, central particle, which is then driven by an oscillating opti...

Water-walled microfluidics for high-optical finesse cavities

In submerged microcavities there is a tradeoff between resonant enhancement for spatial water and light overlap. Why not transform the continuously resonating optical mode to be fully contained in a water microdroplet per se? Here we demonstrate a sustainable 30-mm-pure water device, bounded almost completely by free surfaces, enabling 41,000,000 re-circulations of light. The droplets survive for 416 h using a technique that is based on a nano-water bridge from the droplet to a distant reservoir to compensate for evaporation. More than enabling a nearly-perfect optical overlap with water, atomic-level surface smoothness that minimizes scattering loss, and B99% coupling efficiency from a standard fibre. Surface tension in our droplet is 8,000 times stronger than gravity, suggesting a new class of devices with water-made walls, for new fields of study including opto-capillaries.