Two-beam spin noise spectroscopy (original) (raw)
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Theory of Spin Noise in Nanowires
Physical Review Letters, 2011
We develop a theory of spin noise in semiconductor nanowires considered as prospective elements for spintronics applications. In these structures spin-orbit coupling can be realized as a random function of coordinate correlated on the spatial scale of the order of 10 nm. By analyzing different regimes of electron transport and spin dynamics, we demonstrate that the spin relaxation can be very slow and the resulting noise power spectrum demonstrates at low frequencies the "1/f " flicker noise. This effect brings semiconductor nanowires into a broad variety of systems demonstrating this very general phenomenon, making it best suitable for studies by rapidly developing spin-noise spectroscopy.
Spatiotemporal Spin Noise Spectroscopy
Physical Review Letters, 2019
We report on the potential of a new spin noise spectroscopy approach by demonstrating all-optical probing of spatiotemporal spin fluctuations. This is achieved by homodyne mixing of a spatially phasemodulated local oscillator with spin-flip scattered light, from which the frequency and wave vector dependence of the spin noise power is unveiled. As a first application of the method we measure the spatiotemporal spin noise in weakly n-doped CdTe layers, from which the electron spin diffusion constant and spin relaxation rates are determined. The absence of spatial spin correlations is also shown for this particular system.
Spin noise explores local magnetic fields in a semiconductor
Scientific reports, 2016
Rapid development of spin noise spectroscopy of the last decade has led to a number of remarkable achievements in the fields of both magnetic resonance and optical spectroscopy. In this report, we demonstrate a new - magnetometric - potential of the spin noise spectroscopy and use it to study magnetic fields acting upon electron spin-system of an n-GaAs layer in a high-Q microcavity probed by elliptically polarized light. Along with the external magnetic field, applied to the sample, the spin noise spectrum revealed the Overhauser field created by optically oriented nuclei and an additional, previously unobserved, field arising in the presence of circularly polarized light. This "optical field" is directed along the light propagation axis, with its sign determined by sign of the light helicity. We show that this field results from the optical Stark effect in the field of the elliptically polarized light. This conclusion is supported by theoretical estimates.
Optical Spectroscopy of Spin Noise
Physical Review Letters, 2013
Spontaneous fluctuations of the magnetization of a spin system in thermodynamic equilibrium (spin noise) manifest themselves as noise in the Faraday rotation of probe light. We show that the correlation properties of this noise over the optical spectrum can provide clear information about the composition of the spin system that is largely inaccessible for conventional linear optics. Such optical spectroscopy of spin noise, e.g., allows us to clearly distinguish between optical transitions associated with different spin subsystems, to resolve optical transitions that are unresolvable in the usual optical spectra, to unambiguously distinguish between homogeneously and inhomogeneously broadened optical bands, and to evaluate the degree of inhomogeneous broadening. These new possibilities are illustrated by theoretical calculations and by experiments on paramagnets with different degrees of inhomogeneous broadening of optical transitions [atomic vapors of 41 K and singly charged (In,Ga)As quantum dots].
New insights into electron spin dynamics in the presence of correlated noise
Journal of Physics: Condensed Matter, 2012
The changes of the spin depolarization length in zinc-blende semiconductors when an external component of correlated noise is added to a static driving electric field are analyzed for different values of field strength, noise amplitude and correlation time. Electron dynamics is simulated by a Monte Carlo procedure which keeps into account all the possible scattering phenomena of the hot electrons in the medium and includes the evolution of spin polarization. Spin depolarization is studied by examinating the decay of the initial spin polarization of the conduction electrons through the D'yakonov-Perel process, the only relevant relaxation mechanism in III-V crystals. Our results show that, for electric field amplitude lower than the Gunn field, the dephasing length shortens with the increasing of the noise intensity. Moreover, a nonmonotonic behavior of spin depolarization length with the noise correlation time is found, characterized by a maximum variation for values of noise correlation time comparable with the dephasing time. Instead, in high field conditions, we find that, critically depending on the noise correlation time, external fluctuations can positively affect the relaxation length. The influence of the inclusion of the electron-electron scattering mechanism is also shown and discussed.
Spin Fluctuations and "Spin Noise
Clusters and Nano-Assemblies - Physical and Biological Systems, 2005
We have theoretically studied the temporal fluctuations and the resulting kinetic noise in the average spin polarization of an electron ensemble drifting in a quantum wire under a high electric field. Electrons are initially injected in the wire from a ferromagnetic contact with all their spins polarized along the wire axis. The average spin polarization of the ensemble decays during transport because of D'yakonov-Perel' relaxation caused by both Rashba and Dresselhaus interactions. Once steady state is reached, the average spin fluctuates randomly around zero. The time average of this fluctuation is zero. The autocorrelation function of this fluctuation approximates a Lorentzian and so does the spectral density. To our knowledge, this is the first study of spin fluctuations and "spin noise" in a nanostructure.
Spin noise spectroscopy beyond thermal equilibrium and linear response
Physical review letters, 2014
Per the fluctuation-dissipation theorem, the information obtained from spin fluctuation studies in thermal equilibrium is necessarily constrained by the system's linear response functions. However, by including weak radio frequency magnetic fields, we demonstrate that intrinsic and random spin fluctuations even in strictly unpolarized ensembles can reveal underlying patterns of correlation and coupling beyond linear response, and can be used to study nonequilibrium and even multiphoton coherent spin phenomena. We demonstrate this capability in a classical vapor of (41)K alkali atoms, where spin fluctuations alone directly reveal Rabi splittings, the formation of Mollow triplets and Autler-Townes doublets, ac Zeeman shifts, and even nonlinear multiphoton coherences.
Spin noise of itinerant fermions
Physical Review B, 2010
We develop a theory of spin noise spectroscopy of itinerant, noninteracting, spin-carrying fermions in different regimes of temperature and disorder. We use kinetic equations for the density matrix in spin variables. We find a general result with a clear physical interpretation, and discuss its dependence on temperature, the size of the system, and applied magnetic field. We consider two classes of experimental probes: 1. electron-spin-resonance (ESR)-type measurements, in which the probe response to a uniform magnetization increases linearly with the volume sampled, and 2. optical Kerr/Faraday rotation-type measurements, in which the probe response to a uniform magnetization increases linearly with the length of the light propagation in the sample, but is independent of the cross section of the light beam. Our theory provides a framework for interpreting recent experiments on atomic gases and conduction electrons in semiconductors and provides a baseline for identifying the effects of interactions on spin noise spectroscopy.