Ultrafast Structural Dynamics of 1, 3-CYCLOHEXADIENE: Electronic State Dependence (original) (raw)

66th International …, 2011

Abstract

The ultrafast structural dynamics of 1,3-cyclohexadiene has been investigated using structurally sensitive Rydberg electron binding energies. Excitation to the 1B state and the 3p Rydberg state yielded different structural responses. In both experiments, the structural dynamics of the molecular core are reflected by time-dependent shifts of the Rydberg electron binding energy. Structural distortions associated with 3p-excitation cause a dynamical shift

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