Second Order Optical Nonlinearity of Polymers Induced by Charge Injection Asymmetry (original) (raw)

Molecular Crystals and Liquid Crystals, 1994

Abstract

A new mechanism for inducing bulk asymmetry and second order optical nonlinearity in polymer-dye systems is described. An anisotropic distribution of charges is established inside the medium resulting from the application of high voltage via an asymmetric electrode structure. The nonlinearity induced via this mechanism is perpendicular to the externally applied electric field. It is proven that the nonlinearity induced

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