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Papers by Raffaele Molinari

Research paper thumbnail of Acetophenone hydrogenation in photocatalytic membrane reactor under UV and visible light

Research paper thumbnail of Membrane Operation in Biochemical Processing

Topics in molecular organization and engineering, 1994

The scientific and technological progresses in membrane processes during the past two decades hav... more The scientific and technological progresses in membrane processes during the past two decades have been huge. The existing and potential industrial applications of membrane operations are the widest if compared with any other available separation technology. Pressure driven membrane operations by themselves have already been successfully applied practically in all industrial sectors: from textile to pharmaceutical industry, from leather to agrofood, from automobile to water industry. Biomedical and biotechnological applications, membrane sensors, artificial organs, advanced components in analytical instruments, are other examples of well established membrane systems.

Research paper thumbnail of Studies of Stability of Supported Liquid Membranes for Chiral Separations

Research paper thumbnail of Selective precipitation of calcium ion from seawater desalination reverse osmosis brine

Journal of Cleaner Production, Dec 1, 2021

Research paper thumbnail of Processi a membrana per il trattamento degli effluenti esausti dell’industria conciaria

Research paper thumbnail of Integration of ultrafiltration into unhairing and degreasing operations

Membrane Technology, Nov 1, 1998

Research paper thumbnail of Selective Precipitation of Calcium Ion at Near-Ambient Temperature as a Pretreatment of Seawater Reverse Osmosis Brine and Ex-Ante Lca Assessment

Research paper thumbnail of Upgrade of a Slurry Photocatalytic Membrane Reactor Based on a Vertical Filter and an External Membrane and Testing in the Photodegradation of a Model Pollutant in Water

Research paper thumbnail of Behaviour of RO and NF membranes in the separation of some pollutants in water

Agencja Wydawnicza “ARGI”, 2001

Research paper thumbnail of PMRs Utilizing Pressure-Driven Membrane Techniques

Current Trends and Future Developments on (Bio-) Membranes, 2018

Abstract A brief overview of photocatalytic membrane reactors (PMRs) utilizing pressure-driven me... more Abstract A brief overview of photocatalytic membrane reactors (PMRs) utilizing pressure-driven membrane techniques such as microfiltration, ultrafiltration, and nanofiltration is presented and discussed. Possible strategies of mitigation of membrane fouling in PMRs, including backwashing, air sparging, intermittent permeation, control of hydraulic conditions, etc., are explained in detail. The problem of membrane stability in PMRs in terms of their resistance to UV irradiation, action of reactive oxygen species, and abrasion by photocatalyst particles is explicated. Moreover, an overview of factors affecting the permeate quality is presented. Finally, examples of various configurations of PMRs, including pressurized PMR and submerged PMR systems with photocatalyst in a slurry or photocatalytic membranes are described and compared.

Research paper thumbnail of Supported Liquid Membranes Stability by Chemically and Physically Modified Membranes

Research paper thumbnail of Photocatalytic CO2 Valorization by Using TiO2, ZrO2 and Graphitic Based Semiconductors

2018 IEEE 4th International Forum on Research and Technology for Society and Industry (RTSI), 2018

Research paper thumbnail of Graphitic C3N4 for CO2 reduction: a photoactivity and stability study

Research paper thumbnail of A Study on Neodymium Recovery from Aqueous Solutions for Designing a New Generation of Sandwich Liquid Membrane

Journal of Membrane Science and Research, 2019

Liquid Membrane (LM) based processes, as Supported Liquid Membranes (SLMs), have been proposed, f... more Liquid Membrane (LM) based processes, as Supported Liquid Membranes (SLMs), have been proposed, for over 30 years, as effective methods for the selective separation of inorganic/organic species from different water streams. The industrial use of SLMs has been limited mainly by their insufcient stability. To investigate on the main cause of system destabilization and the optimal conditions for mass transport, a good reference system is the traditional SLM. To this aim the recovery of neodymium (Nd) from acidic media by a traditional SLM has been studied, giving particular attention to permeation and stability. The results clearly evidenced that system stability was strongly influenced by the solubilization of the carrier in the aqueous phases. The consideration and the experimental results reported in this work give useful information to shift the next research step versus the development of a 2nd generation of SwLM able to give satisfactory system performance in view of industrial appl...

Research paper thumbnail of Ultrafiltrazione Combinata con Complessazione nella Rimozione di Metalli da Acque di Lavaggio di Suoli Contaminati

Research paper thumbnail of Arsenic removal from water by coupling photocatalysis and complexation-ultrafiltration processes: A preliminary study

Research paper thumbnail of Which Configuration of Photocatalytic Membrane Reactors Has a Major Potential to Be Used at an Industrial Level in Tertiary Sewage Wastewater Treatment?

Catalysts

Photocatalytic membrane reactors (PMRs) have been found to be very effective in the removal of or... more Photocatalytic membrane reactors (PMRs) have been found to be very effective in the removal of organic pollutants (particularly recalcitrant compounds) from wastewater because they allow for the mineralization of organic pollutants to innocuous by-products, thus achieving high-quality treated water. Owing to the very high volumes of water involved, treated sewage wastewater could be reused if a very efficient tertiary stage, like a PMR, can be foreseen. In this review, the two main PMR configurations (photocatalytic membranes and slurry PMRs) were analyzed as requirements of a tertiary treatment of sewage wastewater considering six design and operational parameters of such plants: (i) continuous wastewater flow rate from the secondary stage; (ii) the self-control of the photodegradation rate related to wastewater chemical–physical parameters; (iii) ability to handle variations of wastewater concentration and flow rate; (iv) the control of the quality of treated wastewater; (v) low p...

Research paper thumbnail of TiO2-Zeolite photocatalysts for acetophenone reduction in a photocatalytic membrane reactor

Research paper thumbnail of Removal of Copper(II)-Citric Acid Chelates from Aqueous Media by Polymer Assisted Ultrafiltration

Research paper thumbnail of Polymer-Assisted Ultrafiltration for metal ions removal from aqueous systems

Research paper thumbnail of Acetophenone hydrogenation in photocatalytic membrane reactor under UV and visible light

Research paper thumbnail of Membrane Operation in Biochemical Processing

Topics in molecular organization and engineering, 1994

The scientific and technological progresses in membrane processes during the past two decades hav... more The scientific and technological progresses in membrane processes during the past two decades have been huge. The existing and potential industrial applications of membrane operations are the widest if compared with any other available separation technology. Pressure driven membrane operations by themselves have already been successfully applied practically in all industrial sectors: from textile to pharmaceutical industry, from leather to agrofood, from automobile to water industry. Biomedical and biotechnological applications, membrane sensors, artificial organs, advanced components in analytical instruments, are other examples of well established membrane systems.

Research paper thumbnail of Studies of Stability of Supported Liquid Membranes for Chiral Separations

Research paper thumbnail of Selective precipitation of calcium ion from seawater desalination reverse osmosis brine

Journal of Cleaner Production, Dec 1, 2021

Research paper thumbnail of Processi a membrana per il trattamento degli effluenti esausti dell’industria conciaria

Research paper thumbnail of Integration of ultrafiltration into unhairing and degreasing operations

Membrane Technology, Nov 1, 1998

Research paper thumbnail of Selective Precipitation of Calcium Ion at Near-Ambient Temperature as a Pretreatment of Seawater Reverse Osmosis Brine and Ex-Ante Lca Assessment

Research paper thumbnail of Upgrade of a Slurry Photocatalytic Membrane Reactor Based on a Vertical Filter and an External Membrane and Testing in the Photodegradation of a Model Pollutant in Water

Research paper thumbnail of Behaviour of RO and NF membranes in the separation of some pollutants in water

Agencja Wydawnicza “ARGI”, 2001

Research paper thumbnail of PMRs Utilizing Pressure-Driven Membrane Techniques

Current Trends and Future Developments on (Bio-) Membranes, 2018

Abstract A brief overview of photocatalytic membrane reactors (PMRs) utilizing pressure-driven me... more Abstract A brief overview of photocatalytic membrane reactors (PMRs) utilizing pressure-driven membrane techniques such as microfiltration, ultrafiltration, and nanofiltration is presented and discussed. Possible strategies of mitigation of membrane fouling in PMRs, including backwashing, air sparging, intermittent permeation, control of hydraulic conditions, etc., are explained in detail. The problem of membrane stability in PMRs in terms of their resistance to UV irradiation, action of reactive oxygen species, and abrasion by photocatalyst particles is explicated. Moreover, an overview of factors affecting the permeate quality is presented. Finally, examples of various configurations of PMRs, including pressurized PMR and submerged PMR systems with photocatalyst in a slurry or photocatalytic membranes are described and compared.

Research paper thumbnail of Supported Liquid Membranes Stability by Chemically and Physically Modified Membranes

Research paper thumbnail of Photocatalytic CO2 Valorization by Using TiO2, ZrO2 and Graphitic Based Semiconductors

2018 IEEE 4th International Forum on Research and Technology for Society and Industry (RTSI), 2018

Research paper thumbnail of Graphitic C3N4 for CO2 reduction: a photoactivity and stability study

Research paper thumbnail of A Study on Neodymium Recovery from Aqueous Solutions for Designing a New Generation of Sandwich Liquid Membrane

Journal of Membrane Science and Research, 2019

Liquid Membrane (LM) based processes, as Supported Liquid Membranes (SLMs), have been proposed, f... more Liquid Membrane (LM) based processes, as Supported Liquid Membranes (SLMs), have been proposed, for over 30 years, as effective methods for the selective separation of inorganic/organic species from different water streams. The industrial use of SLMs has been limited mainly by their insufcient stability. To investigate on the main cause of system destabilization and the optimal conditions for mass transport, a good reference system is the traditional SLM. To this aim the recovery of neodymium (Nd) from acidic media by a traditional SLM has been studied, giving particular attention to permeation and stability. The results clearly evidenced that system stability was strongly influenced by the solubilization of the carrier in the aqueous phases. The consideration and the experimental results reported in this work give useful information to shift the next research step versus the development of a 2nd generation of SwLM able to give satisfactory system performance in view of industrial appl...

Research paper thumbnail of Ultrafiltrazione Combinata con Complessazione nella Rimozione di Metalli da Acque di Lavaggio di Suoli Contaminati

Research paper thumbnail of Arsenic removal from water by coupling photocatalysis and complexation-ultrafiltration processes: A preliminary study

Research paper thumbnail of Which Configuration of Photocatalytic Membrane Reactors Has a Major Potential to Be Used at an Industrial Level in Tertiary Sewage Wastewater Treatment?

Catalysts

Photocatalytic membrane reactors (PMRs) have been found to be very effective in the removal of or... more Photocatalytic membrane reactors (PMRs) have been found to be very effective in the removal of organic pollutants (particularly recalcitrant compounds) from wastewater because they allow for the mineralization of organic pollutants to innocuous by-products, thus achieving high-quality treated water. Owing to the very high volumes of water involved, treated sewage wastewater could be reused if a very efficient tertiary stage, like a PMR, can be foreseen. In this review, the two main PMR configurations (photocatalytic membranes and slurry PMRs) were analyzed as requirements of a tertiary treatment of sewage wastewater considering six design and operational parameters of such plants: (i) continuous wastewater flow rate from the secondary stage; (ii) the self-control of the photodegradation rate related to wastewater chemical–physical parameters; (iii) ability to handle variations of wastewater concentration and flow rate; (iv) the control of the quality of treated wastewater; (v) low p...

Research paper thumbnail of TiO2-Zeolite photocatalysts for acetophenone reduction in a photocatalytic membrane reactor

Research paper thumbnail of Removal of Copper(II)-Citric Acid Chelates from Aqueous Media by Polymer Assisted Ultrafiltration

Research paper thumbnail of Polymer-Assisted Ultrafiltration for metal ions removal from aqueous systems

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