Ziyun WANG - Academia.edu (original) (raw)
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Dr. Ram Manohar Lohiya Avadh University Faizabad
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Papers by Ziyun WANG
Journal of Vacuum Science & Technology A
Cerium oxide thin films were deposited on fused silica using atomic layer deposition (ALD). The n... more Cerium oxide thin films were deposited on fused silica using atomic layer deposition (ALD). The novel Ce precursor, Ce(iPrCp)2(N-iPr-amd) [bis-isopropylcyclopentadienyl-diisopropylacetamidinate-cerium] is a room-temperature liquid with good thermal stability and evaporate cleanly. Water vapor was used as the oxygen source. The growth characteristics and film properties of ALD CeO2 were investigated. A relatively broad ALD window of 165-285 °C resulted in a constant growth rate of 1.9 Å/cycle and good thickness uniformity. The films deposited at 240 °C were found to be polycrystalline with cubic structure without a preferential 17 direction in as-deposited condition. However, films grown at 335°C slightly favored a (200) 18 preferred orientation. XPS analysis showed that films are free from contamination, and the Ce:O 19 stoichiometry analysis revealed the existence of oxygen vacancies in the films with composition 20 CeO1.74. I. Introduction Thin-film cerium oxide (CeO2) is an attractive material because of its wide range of useful properties. It has a high dielectric constant (k>26), moderate band gap (3.0-3.6 eV), and high
ECS Transactions, 2007
ABSTRACT Ruthenium films have been deposited via a pulsed CVD process using tris(2,2,6,6-tetramet... more ABSTRACT Ruthenium films have been deposited via a pulsed CVD process using tris(2,2,6,6-tetramethyl-3,5-heptanedionato) ruthenium (i.e., Ru(thd)3) , oxygen, and hydrogen at 280 and 300{degree sign}C. Film resistivity near theoretical values (16 μΩ-cm at 3 nm) was achieved with repeatability. Films were smooth and continuous down to 2 nm; a low density of pinholes could be observed on films with 1 nm thickness. Adhesive tape tests indicated good adhesion. Carbon content is low.
ECS Transactions, 2009
ABSTRACT In this work, we evaluated novel Sr and Ti precursors for atomic layer deposition applic... more ABSTRACT In this work, we evaluated novel Sr and Ti precursors for atomic layer deposition application. Traditional Sr precursor Sr(thd)2 is a solid with very low vapor pressure, high melting point, and requires high temperature oxidation for efficient carbon removal.. In comparison, bulky cyclopentadienyl based Sr compounds display high vapor pressures, low melting points, reactivity with water and high ALD growth rates. We also evaluated the effect of various stabilizing adducts on the properties of Sr cyclopentadienyl precursors and on the SrO ALD process. Sr precursors studied include AbsoluteSr Sr(iPr3Cp)2, HyperSr.THF Sr(iPr3Cp)2.2THF, HyperSr.DME Sr(iPr3Cp)2.DME, StarSr.THF Sr(Me5Cp)2.THF and StarSr.DME Sr(iPr3Cp)2.DME. Novel Ti precursors like PrimeTi (Ti(MeCp)(OMe)3), StarTi (Ti(Me5Cp)(OMe)3), TyALD (TiCp(NMe2)3) and StarTyALD (TiMe5Cp(NMe2)3) developed using heteroleptic chemistry are evaluated for TiO2 ALD. Finally, compatibility of the novel HyperSr.THF along with Ti precursors such as PrimeTi and StarTi in terms of composition tunability and material properties for STO ALD are studied.
Journal of Vacuum Science & Technology A
Cerium oxide thin films were deposited on fused silica using atomic layer deposition (ALD). The n... more Cerium oxide thin films were deposited on fused silica using atomic layer deposition (ALD). The novel Ce precursor, Ce(iPrCp)2(N-iPr-amd) [bis-isopropylcyclopentadienyl-diisopropylacetamidinate-cerium] is a room-temperature liquid with good thermal stability and evaporate cleanly. Water vapor was used as the oxygen source. The growth characteristics and film properties of ALD CeO2 were investigated. A relatively broad ALD window of 165-285 °C resulted in a constant growth rate of 1.9 Å/cycle and good thickness uniformity. The films deposited at 240 °C were found to be polycrystalline with cubic structure without a preferential 17 direction in as-deposited condition. However, films grown at 335°C slightly favored a (200) 18 preferred orientation. XPS analysis showed that films are free from contamination, and the Ce:O 19 stoichiometry analysis revealed the existence of oxygen vacancies in the films with composition 20 CeO1.74. I. Introduction Thin-film cerium oxide (CeO2) is an attractive material because of its wide range of useful properties. It has a high dielectric constant (k>26), moderate band gap (3.0-3.6 eV), and high
ECS Transactions, 2007
ABSTRACT Ruthenium films have been deposited via a pulsed CVD process using tris(2,2,6,6-tetramet... more ABSTRACT Ruthenium films have been deposited via a pulsed CVD process using tris(2,2,6,6-tetramethyl-3,5-heptanedionato) ruthenium (i.e., Ru(thd)3) , oxygen, and hydrogen at 280 and 300{degree sign}C. Film resistivity near theoretical values (16 μΩ-cm at 3 nm) was achieved with repeatability. Films were smooth and continuous down to 2 nm; a low density of pinholes could be observed on films with 1 nm thickness. Adhesive tape tests indicated good adhesion. Carbon content is low.
ECS Transactions, 2009
ABSTRACT In this work, we evaluated novel Sr and Ti precursors for atomic layer deposition applic... more ABSTRACT In this work, we evaluated novel Sr and Ti precursors for atomic layer deposition application. Traditional Sr precursor Sr(thd)2 is a solid with very low vapor pressure, high melting point, and requires high temperature oxidation for efficient carbon removal.. In comparison, bulky cyclopentadienyl based Sr compounds display high vapor pressures, low melting points, reactivity with water and high ALD growth rates. We also evaluated the effect of various stabilizing adducts on the properties of Sr cyclopentadienyl precursors and on the SrO ALD process. Sr precursors studied include AbsoluteSr Sr(iPr3Cp)2, HyperSr.THF Sr(iPr3Cp)2.2THF, HyperSr.DME Sr(iPr3Cp)2.DME, StarSr.THF Sr(Me5Cp)2.THF and StarSr.DME Sr(iPr3Cp)2.DME. Novel Ti precursors like PrimeTi (Ti(MeCp)(OMe)3), StarTi (Ti(Me5Cp)(OMe)3), TyALD (TiCp(NMe2)3) and StarTyALD (TiMe5Cp(NMe2)3) developed using heteroleptic chemistry are evaluated for TiO2 ALD. Finally, compatibility of the novel HyperSr.THF along with Ti precursors such as PrimeTi and StarTi in terms of composition tunability and material properties for STO ALD are studied.